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Metal photocathodes are an important source of high-brightness electron beams, ubiquitous in the operation of both large-scale accelerators and table-top microscopes. When the surface of a metal is nano-engineered with patterns on the order…
We investigate the fluorescence properties of colloidal quantum dots attached to gold rod nanoantennas. These structures are fabricated by a two step electron beam lithography process in combination with a chemical linking method. By…
We investigate optical nonlinearities that are induced and enhanced due to the strong phonon resonance in hexagonal boron nitride. We predict and observe large sub-picosecond duration signals due to four-wave mixing (FWM) during resonant…
Plasmon oscillations have been intensively studied for more than forty years in conventional two-dimensional electron gas systems in order to find new alternatives to the vacuum devices based on the Smith-Purcell effect in the far-infrared…
We investigate surface plasmon amplification in a silver nanoparticle coupled to an externally driven three-level gain medium, and show that quantum coherence significantly enhances the generation of surface plasmons. Surface plasmon…
We demonstrate that the surface second-harmonic generation can lead to the formation of nonlinear plasmonic whispering-gallery modes (WGMs) in microcavities made of metallic nanowires. Since these WGMs are excited by induced surface…
We study theoretically the cascaded four-wave mixing (FWM) in broadband tapered plasmonic nanoantennas and demonstrate a 300-fold increase in nonlinear frequency conversion detected in the main lobe of the nanoantenna far-field pattern.…
We study light scattering by spherical nanoshells consistent of metal/dielectric composites. We consider two geometries of metallic nanoshell with dielectric core, and dielectric coated metallic nanoparticle. We demonstrate that for both…
Photoluminescence from a gold nanotip, which is induced by surface plasmons propagating over a curved tapered nanotip surface is considered in a co-moving accelerated reference frame. Similar to the surface-enhanced Raman scattering (SERS)…
Strong light-matter interactions enabled by surface plasmons have given rise to a wide range of photonic, optoelectronic and chemical functionalities. In recent years, the interest in this research area has focused on the quantum regime,…
Nonlinear optical processes rely on the intrinsically weak interactions between photons enabled by their coupling with matter. Unfortunately, many applications in nonlinear optics are severely hindered by the small response of conventional…
Localized surface plasmon resonances have recently attracted considerable attention due to their ability to dramatically enhance near-field optical intensities and boost nanoscale light-matter interactions. Here we demonstrate unambiguously…
Efficiency is a critical factor limiting the applications of nonlinear plasmonic devices. We show by theory and experiments that high efficiency four-wave mixing (FWM) is achieved in nanometer size plasmonic hotspots, which open up…
Molecular vibrations couple to visible light only weakly, have small mutual interactions, and hence are often ignored for non-linear optics. Here we show the extreme confinement provided by plasmonic nano- and pico-cavities can sufficiently…
We demonstrate that both linear and nonlinear Fano resonances can be realized on two dimensional magnetic metamaterials. The Fano resonance comes from the interference between localized magnetic plasmon resonance and propagating surface…
The plasmonic amplification of non-linear vibrational sum frequency spectroscopy (SFG) at the surfaces of gold nanoparticles is systematically investigated by tuning the incident visible wavelength. The SFG spectra of dodecanethiol-coated…
We demonstrate fluorescence generation through a sequential multiphoton process with real intermediary states. Our findings suggest new directions for optical control of previously unexplored molecular excitation pathways.
This study found that plasmonic hotspots (HSs) between silver nanoparticles (NPs) and silver nanowires (NWs) generated two-photon excited emissions, including hyper-Rayleigh, hyper-Raman, and two-photon fluorescence of dye molecules with…
Efficient conversion of photons to electrical energy has a wide variety of applications including imaging, energy harvesting, and infrared detection. The coupling of electromagnetic radiation to free electron oscillations at a metal…
We present an electrically driven plasmonic device consisting of a gold nanoparticle trapped in a gap between two electrodes. The tunneling current in the device generates plasmons, which decay radiatively. The emitted spectrum extends up…