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Nonlinear nanophotonics leverages engineered nanostructures to funnel light into small volumes and intensify nonlinear optical processes with spectral and spatial control. Due to its intrinsically large and electrically tunable nonlinear…
Field localization boosts nonlinear optical processes at the hot spots of metal nanostructures. Fano resonances can further enhance these "local" processes taking place at the hot spots. However, in conventional nonlinear materials, the…
The fluorescence of organic fluorophore molecules is enhanced when they are placed in contact with certain metals (Al, Ag, Cu, Au, etc.) whose surface plasmon waves couple into the radiative modes of the molecules and increase the radiative…
Notwithstanding its long history, the study of nonlinear optics from metal surfaces is still an active field of research. For instance, in view of the presence of absorption questions remain concerning the possibility of significantly…
Nonlinear optical phenomena such as parametric amplification and frequency conversion are typically driven by external optical fields. Free electrons can also act as electromagnetic sources, offering unmatched spatial precision. Combining…
We report modifications to the optical properties of fluorophores in the vicinity of noble metal nanotips. The fluorescence from small clusters of quantum dots has been imaged using an apertureless scanning near-field optical microscope.…
We demonstrate that the decay rates of a fluorescent molecule can be controlled by electrically shifting a transparency introduced by a Fano resonance. An auxiliary quantum object (QO), located at the hotspot of a plasmonic nanoparticle,…
The resonance effects on the optical second harmonic generation from 140 nm silver nanoparticles is studied experimentally by hyper-Rayleigh scattering and numerically by finite element method calculations. We find that the interferences…
We introduce a modular approach for efficiently interfacing photonic integrated circuits with deep-sub-wavelength hybrid plasmonic functionality. We demonstrate that an off-the-shelf silicon-on-insulator waveguide can be post-processed into…
We investigate light scattering by coated spheres composed of a dispersive plasmonic core and a dielectric shell. By writing the absorption cross-section in terms of the internal electromagnetic fields, we demonstrate it is an observable…
A distant-neighbor quantum-mechanical method is used to study the nonlinear optical wave mixing in graphene nanoflakes (GNFs), including sum- and difference-frequency generation, as well as four-wave mixing. Our analysis shows that…
Plasmonic nanocavities have proven to be a powerful optical platform for confining light at a length scale much smaller than the diffraction limit. Enhanced electromagnetic fields within the cavity mode volume enable multiple significant…
Localized plasmons in metallic nanostructures have been widely used to enhance nonlinear optical effects due to their ability to concentrate and enhance light down to extreme-subwavelength scales. As alternatives to noble metal…
Plasmonics aims to interface photonics and electronics. Finding optical, near-field analogues of much used electro-technical components is crucial to the success of such a platform. Here we present the plasmonic analogue of a non-reciprocal…
We aim to clarify the role that absorption plays in nonlinear optical processes in a variety of metallic nanostructures and show how it relates to emission and conversion efficiency. We define a figure of merit that establishes the…
Nonlinear optical processes in low dimensional materials are often weak or symmetry forbidden, limiting their use in nanoscale light sources and on chip frequency conversion. Here, we show that combining two weakly nonlinear systems,…
Achieving efficient nonlinear optical frequency conversion in small volumes is key for future on-chip photonic devices that would provide a higher-speed alternative to modern electronics. However, the already intrinsically low conversion…
Plasmonic molecular nanojunctions exhibit opto-mechanical coupling at the nanoscale, enabling intertwined optical, vibrational and electronic phenomena. Here, we demonstrate plasmon-mediated phonon pumping, driven by inelastic electron…
Modern nanotechnology opens the possibility of combining nanocrystals of various materials with very different characteristics in one superstructure. The resultant superstructure may provide new physical properties not encountered in…
Graphene is known to possess strong optical nonlinearity. Its nonlinear response can be further enhanced by graphene plasmons. Here, we report a novel nonlinear electro-absorption effect observed in nanostructured graphene due to excitation…