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A general variational approach for computing the rovibrational dynamics of polyatomic molecules in the presence of external electric fields is presented. Highly accurate, full-dimensional variational calculations provide a basis of…

Chemical Physics · Physics 2018-04-18 Alec Owens , Andrey Yachmenev

We analyze atomic photoexcitation into the discrete states by twisted photons, or photons carrying extra orbital angular momentum along their direction of propagation. From the angular momentum and parity considerations, we are able to…

Atomic Physics · Physics 2018-03-07 Andrei Afanasev , Carl E. Carlson , Maria Solyanik

Photonic molecules - particular systems composed of coupled optical resonators - emulate the behavior of complex physical systems exhibiting discrete energy levels. In this work, we present a novel photonic molecule composed of two strongly…

Optics · Physics 2023-12-06 Sara Kacmoli , Deborah L. Sivco , Claire F. Gmachl

Compton scattering of low-frequency radiation by an isotropic distribution of (i) mildly and (ii) ultra relativistic electrons is considered. It is shown that the ensemble-averaged differential cross-section in this case is noticeably…

Astrophysics · Physics 2011-05-23 Sergei Y. Sazonov , Rashid A. Sunyaev

The Complex Kohn variational method for electron-polyatomic molecule scattering is formulated using an overset grid representation of the scattering wave function. The overset grid consists of a central grid and multiple dense,…

Chemical Physics · Physics 2017-12-06 Loren Greenman , Robert R. Lucchese , C. William McCurdy

We establish a link between quantum mechanical molecular simulations and the transfer matrix of a molecule. The transfer matrix (T-matrix) of an object provides a complete description of its electromagnetic response. Once the T-matrices of…

Chemical Physics · Physics 2020-04-21 Ivan Fernandez-Corbaton , Carsten Rockstuhl , Wim Klopper

We investigate attosecond time delays in the emission of photoelectrons using a hierarchy of models of the $CO_2$ molecule including the strong field approximation, Coulomb-scattering, short-range parts of the molecular potential, Hartree…

Atomic Physics · Physics 2021-03-30 Hakon Volkmann , Vinay P. Majety , Armin Scrinzi

We employ the exact factorization of a multi-component wavefunction to analyze the dynamics of interacting photons, electrons and nuclei. We consider physical situations emerging in the regime of strong coupling between light excitations…

Chemical Physics · Physics 2026-04-24 Claudia Magi , Peter Schuerger , David Lauvergnat , Federica Agostini

Electron scattering and dielectronic recombination with an ion in the presence of a neighboring atom is studied. The incident electron is assumed to be captured by the ion, leading to resonant excitation of the atom which afterwards may…

Atomic Physics · Physics 2018-08-01 A. Eckey , A. Jacob , A. B. Voitkiv , C. Müller

In these notes we present a detailed and complete scheme for the calculation of polarization phenomena in elastic electron-nucleon scattering. The longitudinal and transversal components of the polarization for the scattered nucleon,…

Nuclear Theory · Physics 2007-05-23 Michail P. Rekalo , Egle Tomasi-Gustafsson

Chiral molecules ionized by circularly polarized fields produce a photoelectron current orthogonal to the polarization plane. This current has opposite directions for opposite enantiomers and provides an extremely sensitive probe of…

Atomic Physics · Physics 2022-06-28 Andres F. Ordonez , Olga Smirnova

For a molecule, the two-center interference and the molecular scattering phase of the electron are important for almost all the processes that may occur in a laser field. In this study, we investigate their effects in the transfer of linear…

Atomic Physics · Physics 2018-12-19 Hao Liang , Mu-Xue Wang , Xiang-Ru Xiao , Qihuang Gong , Liang-You Peng

The regions of pair particle energies and emergence angles in the process of photoproduction of electron-positron pairs in the coulomb field by polarized photons are found in which a value of cross section asymmetry is essentially large.…

High Energy Physics - Experiment · Physics 2007-05-23 R. O. Avakian , K. R. Dallakyan , S. M. Darbinyan

We employ ptychography, a phase-retrieval imaging technique, to show experimentally for the first time that a partially coherent high-energy matter (electron) wave emanating from an extended source can be decomposed into a set of mutually…

Mesoscale and Nanoscale Physics · Physics 2017-01-04 S. Cao , P. Kok , P. Li , A. M. Maiden , J. M. Rodenburg

In this work we discuss the rotational structure of Rydberg molecules. We calculate the complete wave function in a laboratory fixed frame and derive the transition matrix elements for the pho- toassociation of free ground state atoms. We…

Atomic Physics · Physics 2018-08-01 O. Thomas , C. Lippe , T. Eichert , H. Ott

The interaction of a fast electron with a photonic crystal is studied by solving the Maxwell equations exactly for the external field provided by the electron in the presence of the crystal. The polarization currents and charges produced by…

Condensed Matter · Physics 2009-11-07 L. A. Blanco , F. J. Garcia de Abajo

We analyze the real-time electron-photon dynamics in long-range polariton-mediated energy transfer using a real-time quantum electrodynamics coupled cluster (RT-QED-CC) model, which allows for spatial and temporal visualization of transport…

Chemical Physics · Physics 2024-04-16 Matteo Castagnola , Marcus T. Lexander , Enrico Ronca , Henrik Koch

We study ionization of aligned H$_2^+$ in strong elliptically-polarized laser fields numerically and analytically. The calculated offset angle in photoelectron momentum distribution is several degrees larger for the molecule than a model…

Atomic Physics · Physics 2023-01-03 J. Y. Che , Y. G. Peng , F. B. Zhang , X. J. Xie , G. G. Xin , Y. J. Chen

We present a theoretical study on polarization-averaged molecular-frame photoelectron angular distributions (PA-MFPADs) emitted from $1s$ orbital of oxygen atom of dissociating dicationic carbon monoxide CO$^{2+}$. Due to the…

Chemical Physics · Physics 2020-11-17 Fukiko Ota , Kaoru Yamazaki , Didier Sébilleau , Kiyoshi Ueda , Keisuke Hatada

The backscattering of laser radiation by a relativistic electron beam is a widely used method for measuring the spin polarization of electrons. We consider again the properties of the scattering process paying special attention to recoil…

Accelerator Physics · Physics 2022-10-19 N. Yu. Muchnoi