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We present a novel approach to calculating strong field ionization dynamics of multielectron molecular targets. Adopting a multielectron wavefunction ansatz based on field-free ab initio neutral and ionic multielectron states, a set of…

Atomic Physics · Physics 2015-05-14 Michael Spanner , Serguei Patchkovskii

Effects of the interchannel coupling on the spin polarization of energetic photoelectrons emitted from atomic Ne valence subshells are examined. Like previously obtained results for cross sections and angular distributions, the…

Atomic Physics · Physics 2021-06-08 Himadri S. Chakraborty , Pranawa C. Deshmukh , Steven T. Manson

We investigate the effect of high order radiative corrections in unpolarized electron proton elastic scattering and compare with the calculations at lowest order, which are usually applied to experimental data. Particular attention is…

High Energy Physics - Phenomenology · Physics 2015-06-17 E. A. Kuraev , A. I. Ahmadov , Yu. M. Bystritskiy , E. Tomasi-Gustafsson

Photoelectron circular dichroism results from one-photon ionization of chiral molecules by circularly polarized light and manifests itself in forward-backward asymmetry of electron emission in the direction orthogonal to the light…

Atomic Physics · Physics 2019-04-24 Andres F. Ordonez , Olga Smirnova

Photoelectron spectroscopy is a powerful method that provides insight into the quantum mechanical properties of a wide range of systems. The ionized electron wavefunction carries information on the structure of the bound orbital, the ionic…

A new version of the R-matrix Floquet theory for laser-assisted electron-atom scattering is presented. The theory is non-perturbative and applicable to a non-relativistic many-electron atom or ion in a homogeneous linearly polarized field.…

Atomic Physics · Physics 2009-11-07 Mariko Terao-Dunseath , Kevin Dunseath

We describe upgrades to a numerical code which computes synchrotron and inverse-Compton emission from relativistic plasma including full polarization. The introduced upgrades concern scattering kernel which is now capable of scattering the…

High Energy Astrophysical Phenomena · Physics 2022-11-16 M. Moscibrodzka

The relative roles of multiple electron scattering and in-molecule free-space propagation in transmission electron microscopy of small molecules are discussed. It is argued that while multiple scattering tends to have only a moderate effect…

Image and Video Processing · Electrical Eng. & Systems 2019-12-02 T. E. Gureyev , H. M. Quiney , A. Kozlov , L. J. Allen

Photoelectron Angular Distributions (PADs) resulting from 800 nm and 1300 nm strong field ionization of impulsively aligned CF$_3$I molecules were analyzed using time-dependent density functional theory (TDDFT). The normalized difference…

In this paper we consider the possibility and conditions for pair photoemission whereby two incident photons emit pairs of electrons from a candidate material as a novel method to measure and visualize electronic correlations. As opposed to…

The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

Chemical Physics · Physics 2017-05-18 David Ayuso

We give examples showing that two well-known versions of the S-matrix theory, which describes a nonresonant multiphoton ionization of atoms and ions in intense laser fields, lead to qualitatively different results. The latter refer not only…

Atomic Physics · Physics 2015-05-28 J. H. Bauer

If matter absorbs a photon of sufficient energy it emits an electron. The question of the duration of the emission process has intrigued scientists for decades. With the advent of attosecond metrology, experiments addressing such ultrashort…

Monte Carlo evaluation is used to calculate heavy-ion elastic scattering including the center-of-mass correction and the Coulomb interaction.Angular distributions are presented for a number of nuclear pairs over a wide energy range using…

Nuclear Theory · Physics 2015-06-04 W. R. Gibbs , Jean-Pierre Dedonder

Within thunderstorms electrons can gain energies of up to hundred(s) of MeV. These electrons can create X-rays and gamma-rays as Bremsstrahlung when they collide with air molecules. Here we calculate the distribution of angles between…

Atmospheric and Oceanic Physics · Physics 2016-12-02 Christoph Köhn , Ute Ebert

We review the study of dissociative recombination and ro-vibrational excitation of diatomic and small polyatomic molecular ions initiating complex organic molecules formation. In particular, we show how Multichannel Quantum Defect Theory…

We describe an ab initio and non-perturbative $R$-matrix with time-dependence theory for ultrafast atomic processes in light fields of arbitrary polarization. The theory is applicable to complex, multielectron atoms and atomic ions subject…

Atomic Physics · Physics 2018-12-04 D. D. A. Clarke , G. S. J. Armstrong , A. C. Brown , H. W. van der Hart

Photoionization cross sections calculations on the halogen-like ions; Kr$^+$ and Xe$^+$ have been performed for a photon energy range from each ion threshold to 15 eV, using large-scale close-coupling calculations within the Dirac-Coulomb…

Earth and Planetary Astrophysics · Physics 2012-04-02 B. M. McLaughlin , C. P. Ballance

High-resolution photoelectron momentum distributions of Xe atoms ionized by 800-nm linearly polarized laser fields have been traced at intensities from 1.1*1013 to 3.5*1013W/cm2 using velocity-map imaging techniques. At certain laser…

Atomic Physics · Physics 2015-12-09 Min Li , Peng Zhang , Siqiang Luo , Yueming Zhou , Qingbin Zhang , Pengfei Lan , Peixiang Lu

Optical control of polyatomic molecules promises new opportunities in precision metrology, fundamental chemistry, quantum information, and many-body science. Contemporary experimental and theoretical efforts have mostly focused on cycling…

Atomic Physics · Physics 2022-12-26 Phelan Yu , Adrian Lopez , William A. Goddard , Nicholas R. Hutzler