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Photoelectron angular distributions (PADs) of oriented polar molecules in response to different polarized lasers are systematically investigated. It is found that the PADs of polar CO molecules show three distinct styles excited by…

Chemical Physics · Physics 2013-03-05 Xiaosong Zhu , Qingbin Zhang , Weiyi Hong , Peixiang Lu , Zhizhan Xu

Intense light with frequencies above typical atomic or molecular ionization potentials as provided by free-electron lasers couples many photons into extended targets such as clusters and biomolecules. This implies, in contrast to…

Atomic and Molecular Clusters · Physics 2011-05-25 Christian Gnodtke , Ulf Saalmann , Jan-Michael Rost

The process of the elastic scattering of photons on atoms, known as the Rayleigh scattering, is investigated. Expressing the scattering observables in terms of the electric and magnetic complex scattering amplitudes, we work over the…

Atomic Physics · Physics 2020-10-20 A. V. Volotka , A. Surzhykov , S. Fritzsche

The multiple scattering of ultra relativistic electrons in an amorphous matter leads to the suppression of the soft part of radiation spectrum (the Landau-Pomeranchuk-Migdal effect), and also can change essentially the angular distribution…

Accelerator Physics · Physics 2017-05-10 Alex Fomin , Serguei Fomin , Nikolai Shul'ga

We report fully differential photoelectron spectra from an {\it ab-inito} coupled channels treatment of CO$_2$. Photoionization by laser pulses centered at 400 nm and 800 nm wavelength are considered, with arbitrary molecular alignment and…

Atomic Physics · Physics 2017-09-05 Vinay Pramod Majety , Armin Scrinzi

An alternative method to the density matrix formalism for the derivation of general expressions of the interaction of polarized atoms with polarized photons and electrons is presented. The expression for the cross-section describing the…

Quantum Physics · Physics 2015-06-26 A. Kupliauskiene

We present a time-dependent density-functional method able to describe the photoelectron spectrum of atoms and molecules when excited by laser pulses. This computationally feasible scheme is based on a geometrical partitioning that…

Atomic Physics · Physics 2012-06-28 U. De Giovannini , D. Varsano , M. A. L. Marques , H. Appel , E. K. U. Gross , A. Rubio

We present a theoretical approach to investigate the scattering of polarized electrons from light nuclei using the multipole expansion for the scattering cross section within the framework of the unified electroweak theory. Scattering…

Nuclear Theory · Physics 2026-05-01 Minh Truong Vo , Vu Dong Tran , Quang Hung Nguyen

We revisit strong-field ionization of aligned O$_2$, CO$_2$, and CS$_2$ molecules in light of recent advances in the field of strong-field physics, in particular the inclusion of multielectron polarization in the numerical solution of the…

Atomic Physics · Physics 2022-08-17 M. Abu-samha , Lars Bojer Madsen

Photoelectron spectroscopy in intense laser fields has proven to be a powerful tool for providing detailed insights into molecular structure. The ionizing molecular orbital, however, has not been reconstructed from the photoelectron…

Atomic Physics · Physics 2023-04-14 XuanYang Lai , RenPing Sun , ShaoGang Yu , YanLan Wang , Wei Quan , André Staudte , XiaoJun Liu

Most bright sources of the radiation in hard x-ray and gamma--ray regions are undulator sources and Compton based ones. These sources are ultimate for production of polarized positrons necessary for future linear colliders ILC, CLIC. We…

Accelerator Physics · Physics 2015-09-14 Eugene Bulyak , Nikolay Shul'ga

We study nondipole effects in multiphoton ionization of a two-dimensional hydrogen-like atom by a flat-top laser pulse of varied intensity. For this purpose, we solve numerically a two-dimensional Schr\"odinger equation treating a…

Atomic Physics · Physics 2024-12-25 J. Z. Kamiński , K. Krajewska

Various properties of the general two-center two-electron integral over the explicitly correlated exponential function are analyzed for the potential use in high precision calculations for diatomic molecules. A compact one dimensional…

Chemical Physics · Physics 2015-06-11 Krzysztof Pachucki

We study ionization dynamics of aligned diatomic molecules N$_2$ in strong elliptical laser fields experimentally and theoretically. The alignment dependence of photoelectron momentum distributions (PMDs) of N$_2$ measured in experiments is…

The feasibility of complete photoionization experiments, in which the full set of photoionization matrix elements are determined, using multiphoton ionization schemes with polarization-shaped pulses has recently been demonstrated [Hockett…

Atomic Physics · Physics 2015-07-22 P. Hockett , M. Wollenhaupt , C. Lux , T. Baumert

With angle resolved photoemission experiments and \emph{ab-initio} electronic structure calculations, the pentacene monolayers on Ag(110) and Cu(110) are compared and contrasted allowing the molecular orientation and an unambiguous…

We present and discuss a new computationally inexpensive method to study, within the single active electron approximation, the interaction of a complex system with an intense ultrashort laser pulse. As a first application, we consider the…

We use extreme-ultraviolet interferometry to measure the phase of high-order harmonic generation from transiently aligned CO2 molecules. We unambiguously observe a reversal in phase of the high order harmonic emission for higher harmonic…

Atomic Physics · Physics 2009-11-13 Xibin Zhou , Robynne Lock , Wen Li , Nick Wagner , Margaret. M. Murnane , Henry C. Kapteyn

Using the eigenchannel R-matrix method we calculate partial photoionization cross sections from the ground state of the helium atom for incident photon energies up to the N=9 manifold. The wide energy range covered by our calculations…

Atomic Physics · Physics 2009-11-07 Tobias Schneider , Chien-Nan Liu , Jan-Michael Rost

Theoretically self-consistent calculations for photoionization and (e + ion) recombination are described. An identical eigenfunction expansion for the ion is employed in coupled channel calculations for both processes, thus ensuring…

Astrophysics · Physics 2007-05-23 Sultana N. Nahar