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We propose a novel actuation mechanism for colloids, which is based on the Seebeck effect of the electrolyte solution: Laser heating of a nonionic particle accumulates in its vicinity a net charge Q, which is proportional to the excess…

Soft Condensed Matter · Physics 2014-01-30 Arghya Majee , Alois Würger

Aqueous electrolyte solutions under the influence of a temperature gradient can generate thermoelectric fields, which arise from different responses of the positive and negative charges. This is related to the thermo diffusion effect which…

Soft Condensed Matter · Physics 2022-06-23 André Luiz Sehnem , Antônio Martins Figueiredo Neto

The electric field in an extended phase of a liquid electrolyte exposed to a temperature gradient is attributed to different thermophoretic mobilities of the ion species. As shown herein, such Soret-type ion thermodiffusion is not required…

Fluid Dynamics · Physics 2020-12-24 Mathias Dietzel , Steffen Hardt

We theoretically study the electrolyte Seebeck effect in the vicinity of a heated metal nanostructure, such as the cap of an active Janus colloid in an electrolyte, or gold- coated interfaces in optofluidic devices. The thermocharge…

Soft Condensed Matter · Physics 2018-02-27 Aboubakry Ly , Arghya Majee , Alois Würger

We have developed a method to probe the temperature of surface state electrons (SSE) above a superfluid Helium-4 surface using the Seebeck effect. In contrast to previously used SSE thermometry, this technique does not require detailed…

Mesoscale and Nanoscale Physics · Physics 2018-12-12 Ethan I. Kleinbaum , Stephen A. Lyon

Single-ion Soret coefficients $\alpha_{i}$ characterize the tendency of ions in an electrolyte solution to move in a thermal gradient. When these coefficients differ between cations and anions, an electric field can be generated. For this…

Chemical Physics · Physics 2021-05-03 André Luiz Sehnem , Mathijs Janssen

We use the one-dimensional object-oriented particle-in-cell Monte Carlo collision code oopd1 to explore the charged particle densities, the electronegativity, the electron energy probability function (EEPF), and the electron heating…

Plasma Physics · Physics 2017-11-28 Jon Tomas Gudmundsson , David I. Snorrason

Recent calculations by Vorobev and Malyshenko (JETP Letters, 71, 39, 2000) show that molecular hydrogen may stay liquid and superfluid in strong electric fields of the order of $4\times 10^7 V/cm$. I demonstrate that strong local electric…

Strongly Correlated Electrons · Physics 2009-10-31 Igor I. Smolyaninov

A novel method to pump fluid in lab on chip devices with velocities up to tens of micrometer per second is introduced. A focused laser beam locally heats up an electrolyte. A net charge tends to accumulate in the heat-absorbing area, due to…

Soft Condensed Matter · Physics 2014-05-08 Reza Kiani Iranpour , Seyyed Nader Rasuli

We study the thermal diffusion coefficient DT of a charged colloid in a temperature gradient, and find that it is to a large extent determined by the thermoelectric response of the electrolyte solution. The thermally induced salinity…

Soft Condensed Matter · Physics 2014-01-30 Alois Würger

We investigate nonequilibrium effects in the transport of interacting electrons in quantum conductors, proposing the nonlocal thermoelectric response as a direct indicator of the presence of interactions, nonthermal states and the effect of…

Mesoscale and Nanoscale Physics · Physics 2024-05-10 Alessandro Braggio , Matteo Carrega , Björn Sothmann , Rafael Sánchez

The Seebeck and Soret coefficients of ionically stabilized suspension of maghemite nanoparticles in dimethyl sulfoxide are experimentally studied as a function of nanoparticle volume fraction. In the presence of a temperature gradient, the…

We present data exhibiting hot spots spontaneously emerging in forward biased thin film photovoltaics based on a-Si:H technology. These spots evolve over time shrinking in their diameter and increasing temperature up to approximately 300…

Disordered Systems and Neural Networks · Physics 2014-01-03 Anthony C. Vasko , Aarohi Vijh , Victor G. Karpov

We report on the direct observation of the thermoelectric transport in a nondegenerate correlated electron system formed on the surface of liquid helium. We find that the microwave-induced excitation of the vertical transitions of electrons…

Other Condensed Matter · Physics 2021-11-10 Ivan Kostylev , A. A. Zadorozhko , M. Hatifi , Denis Konstantinov

In this experiment liquid water is subject to an inhomogeneous electric field (${\nabla}^2 E_a {\approx} 10^{10} \frac{V}{m^2}$ ) using a high voltage (20 kV) point-plane electrode system. With interferometry it was found that the…

Mesoscale and Nanoscale Physics · Physics 2016-06-29 Adam D. Wexler , Sandra Drusová , Jakob Woisetschläger , Elmar C. Fuchs

When two electrolyte-immersed electrodes have different temperatures, a voltage $\Delta \psi$ can be measured between them. This electrolyte Seebeck effect is usually explained by cations and anions flowing differently in thermal gradients.…

Chemical Physics · Physics 2023-09-15 Ole Nickel , Ludwig J. V. Ahrens-Iwers , Robert H. Meißner , Mathijs Janssen

The Seebeck coefficient in liquids often reaches the mV/K range, yet its microscopic origin remains unclear due to the complexity of electrolyte systems. Here we propose a minimal electrostatic theory focusing on solvation entropy. Using…

Statistical Mechanics · Physics 2026-03-06 Wataru Kobayashi

A systematic theoretical study of thermoelectric effect and temperature-gradient-driven electrokinetic flow of electrolyte solutions in charged nanocapillaries is presented. The study is based on a semianalytical model developed by…

Fluid Dynamics · Physics 2023-09-14 Wenyao Zhang , Qiuwang Wang , Min Zeng , Cunlu Zhao

The atomic variations of electronic wavefunctions at the surface and electron scattering near a defect have been detected unprecedentedly by tracing thermoelectric voltages given a temperature bias [Cho et al., Nature Mater. 12, 913…

Mesoscale and Nanoscale Physics · Physics 2014-04-02 Eui-Sup Lee , Sanghee Cho , Ho-Ki Lyeo , Yong-Hyun Kim

We present a field theory approach to study changes in local temperature due to an applied electric field (the electrocaloric effect) in electrolyte solutions. Steric effects and a field-dependent dielectric function are found to be of…

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