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In this study we explore, both from theoretical and experimental side, the effect of Fe doping in ZrO2 (ZrO2:Fe). By means of first principles simulation we study the magnetization density and the magnetic interaction between Fe atoms. We…

We address one of the main challenges to TiO2-photocatalysis, namely band gap narrowing, by combining nanostructural changes with doping. With this aim we compare TiO2's electronic properties for small 0D clusters, 1D nanorods and…

Materials Science · Physics 2010-01-18 D. J. Mowbray , J. I. Martinez , J. M. García-Lastra , K. S. Thygesen , K. W. Jacobsen

Thermodynamic theory is developed for the ferroelectric phase transition of an ultrathin film in equilibrium with a chemical environment that supplies ionic species to compensate its surface. Equations of state and free energy expressions…

Materials Science · Physics 2015-05-20 G. Brian Stephenson , Matthew J. Highland

We report spin polarized density functional calculations of ferromagnetic properties of a series of ZnO clusters and solid containing one or two substitutional carbon impurities. We analyze the eigen value spectra, spin densities and…

Materials Science · Physics 2016-09-28 B. J. Nagare , Sajeev Chacko , D. G. Kanhere

The (111), (110), and (001) surfaces properties of PuO2 are studied by using density-functional theory+U method. The total-energy static calculations determine the relative order of stability for low-index PuO2 surfaces, namely,…

Materials Science · Physics 2012-08-21 Bo Sun , Haifeng Liu , Haifeng Song , Guang-Cai Zhang , Hui Zheng , Xian-Geng Zhao , Ping Zhang

We realize Mn $\delta$-doping into Si and Si/Ge interfaces using Mn atomic chains on Si(001). Highly sensitive X-ray absorption fine structure techniques reveal that encapsulation at room temperature prevents the formation of silicides /…

We report a novel effect that the visible photoluminescence (in the blue-green band) from ZnO anoparticles can be controlled by changing the ionic or polar nature of the medium in which the nanoparticles are dispersed. We find that the…

Materials Science · Physics 2009-11-13 Manoranjan Ghosh , A. K. Raychaudhuri

We report on the structural and magnetic characterization of Co0.1Zn0.9O and Mn0.1Zn0.9O nanopowders obtained by a soft chemistry route. We show that those samples fired at low temperatures display a ferromagnetic interaction that can not…

Materials Science · Physics 2009-11-11 D. Rubi , A. Calleja , J. Arbiol , X. G. Capdevila , M. Segarra , Ll. Aragones , J. Fontcuberta

Relaxations at nonpolar surfaces of III-V compounds result from a competition between dehybridization and charge transfer. First principles calculations for the (110) and (10$\bar{1}$0) faces of zincblende and wurtzite AlN, GaN and InN…

Materials Science · Physics 2009-10-31 Alessio Filippetti , Vincenzo Fiorentini , Giancarlo Cappellini , Andrea Bosin

Cubic gauche polynitrogen (cg-N) is an attractive high-energy density material. However, high-pressure synthesized cg-N will decompose at low-pressure and cannot exist at ambient conditions. Here, the stabilities of cg-N surfaces with and…

Materials Science · Physics 2024-12-02 Guo Chen , Caoping Niu , Wenming Xia , Jie Zhang , Zhi Zeng , Xianlong Wang

In this work, we study the emergence of polarization doping in AlxGa1-xN layers with graded composition from a theoretical viewpoint. We demonstrate that the charge conservation law applies for fixed and mobile charges separately, leading…

This study combines surface-sensitive photoemission experiments with density functional theory (DFT) to give a microscopic description of H adsorption-induced modifications of the ZnO(10${\overline{1}}$0) surface electronic structure. We…

Materials Science · Physics 2015-06-23 J. -C. Deinert , O. T. Hofmann , M. Meyer , P. Rinke , J. Stähler

Zn1-xRxO (R = Li, Mg, Cr, Mn, Fe and Cd) were obtained by using co-precipitation synthesis technique with constant weight percent of 3% from R ions. The phase composition, crystal structure, morphology, Density Functional Theory (DFT), and,…

Materials Science · Physics 2021-10-26 T. A. Abdel-Baset , M. Abdel-Hafiez

We show that the HF acid etch commonly used to prepare SrTiO3(001) for heteroepitaxial growth of complex oxides results in a non-negligible level of F doping within the terminal surface layer of TiO2. Using a combination of x-ray…

Materials Science · Physics 2015-05-30 Scott A. Chambers , Timothy C. Droubay , Cigdem Capan , Guangyuan Sun

The structural stabilities of the monoclinic and tetragonal phases of Si-doped HfO$_{2}$ at finite temperatures were analyzed using a computational scheme to assess the effects of impurity doping. The finite temperature effects considered…

The study particularly focuses on the effect of the Cr co-doping on the structural, optical and magnetic properties of Zn0.99Fe0.01O. Zn0.99-xFe0.01CrxO (x =0, 0.01, 0.03 and 0.05) nanoparticles. Powder x-ray diffraction (XRD) analysis…

Materials Science · Physics 2021-11-16 H. S. Lokesha , P. Mohanty , C. J. Sheppard , A. R. E. Prinsloo

Strain effects on the stabilization of Al ad-atom on graphene oxide(GO)nanosheet as well as its implications for NH3 storage have been investigated using first-principles calculations.The binding energy of Al ad-atom on GO is found to be a…

Materials Science · Physics 2015-06-05 Yunguo Li , Abir De Sarkar , Biswarup Pathak , Rajeev Ahuja

We report the structural and magnetic properties of ZnO single crystals implanted at 623 K with up to 10 at. % of Ni. As revealed by X-ray diffraction, crystalline fcc-Ni nanoparticles were formed inside ZnO. The magnetic behavior…

Materials Science · Physics 2007-05-23 Shengqiang Zhou , K. Potzger , Gufei Zhang , F. Eichhorn , W. Skorupa , M. Helm , J. Fassbender

The cubic perovsike strontium titanate SrTiO$_3$ (STO) is one of the most studied, polarizable transition metal oxides. When excess charge is introduced to this material, e.g., through doping or atomic defects, STO tends to host polarons:…

Materials Science · Physics 2022-09-13 Florian Ellinger , Muhammad Shafiq , Iftikhar Ahmad , Michele Reticcioli , Cesare Franchini

Ordinary ice has a proton-disordered phase which is kinetically metastable, unable to reach, spontaneously, the ferroelectric (FE) ground state at low temperature where a residual Pauling entropy persists. Upon light doping with KOH at low…

Materials Science · Physics 2021-01-01 Jorge Lasave , Sergio Koval , Alessandro Laio , Erio Tosatti