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Solids exposed to intense electric fields release electrons through tunnelling. This fundamental quantum process lies at the heart of various applications, ranging from high brightness electron sources in DC operation to petahertz vacuum…

Ultrashort electron pulses with a high average current provide a powerful means of enhancing time-resolved imaging and photon generation. In this study, we report the attosecond shaping of sub-relativistic electron beams using membranes in…

Recent experiments on measuring time-delays during tunnelling of cold atoms through an optically created potential barrier are reinvigorating the controversial debate regarding possible time-delays during light-induced tunnelling of an…

We demonstrate an accurate phase retrieval of XUV atomic ionization by streaking the photoelectron in a circularly polarized IR laser field. The streaking phase can then be converted to the atomic time delay containing the Wigner and…

In the semiclassical picture of photoionization process in intense laser fields, the ionization rate solely depends on the amplitude of the electric field and the final photoelectron momentum corresponds to the instant of ionization of the…

Atomic Physics · Physics 2019-05-09 Li Guo , Shilin Hu , Mingqing Liu , Zheng Shu , Xiwang Liu , Jie Li , Weifeng Yang , Ronghua Lu , Shensheng Han , Jing Chen

In a recent paper [Phys. Rev. Lett. 125, 043201 (2020)] (Ref.1) Liao et al. propose a theory of the interferometric photoemission delay based on the concepts of the photoelectron phase and photoelectron effective mass. The present comment…

Materials Science · Physics 2021-04-26 E. E. Krasovskii , R. O. Kuzian

We experimentally demonstrate spatiotemporal steering of photoelectron emission in multiphoton above-threshold single ionization of atoms exposed to a phase-controlled orthogonally polarized two-color (OTC) laser pulse. Spatial and energy…

The present review addresses the technical advances and the theoretical developments to realize and rationalize attosecond-science experiments that reveal a new dynamical time scale ($10^{-15}$-$10^{-18}$ s), with a particular emphasis on…

Chemical Physics · Physics 2020-02-07 Denitsa Baykusheva , Hans Jakob Wörner

Attosecond time-resolution experiments using noncollinear interferometers require precise and active control of the optical delay to prevent instabilities - including both slow drifts and rapid vibrations - that can obscure the time…

In nuclear collisions, nuclear bremsstrahlung can cause nuclear Coulomb excitation via photon exchange in the projectile as well as the target nuclei. Such a process originating in nuclear timescales (zeptoseconds) can also influence the…

Atomic Physics · Physics 2025-03-25 T. Nandi , Soumya Chatterjee , Adya P. Mishra , Y. Azuma , F. Koike , A. S. Kheifets

Recent angle-resolved RABBITT experiments have shown that the photoionization time delay depends on the emission angle of the photoelectron. In this work we demonstrate that for photoemission from helium accompanied by shake-up (correlation…

Atomic Physics · Physics 2020-09-30 Stefan Donsa , Manuel Ederer , Renate Pazourek , Joachim Burgdörfer , Iva Březinová

The energy-time uncertainty is an intrinsic limit for time-resolved experiments imposing a tradeoff between the duration of the light pulses used in experiments and their frequency content. In standard time-resolved photoemission, this…

Strongly Correlated Electrons · Physics 2017-03-22 Francesco Randi , Daniele Fausti , Martin Eckstein

Strong field ionization provides a unique mean to address complex dynamics of an electron in competing Coulomb and laser fields. Recent streak camera experiment (K\"ubel, et al., Phys. Rev. Lett. 119, 183201) analyzed asymmetries in the…

Using time dependent density functional theory (TDDFT) we examine the energy, angular and time-resolved photoelectron spectra (TRPES) of ethylene in a pump-probe setup. To simulate TRPES we expose ethylene to an ultraviolet (UV) femtosecond…

Atomic and Molecular Clusters · Physics 2014-08-28 Alison Crawford-Uranga , Umberto De Giovannini , Duncan John Mowbray , Stefan Kurth , Angel Rubio

In our model the electron dynamics are described by a two-state approximation. This might appear a rough approximation since it neglects coupling through excited electronic states and ionization channels. However at high intensity (laser…

Atomic Physics · Physics 2007-05-23 J F McCann , Liang-You Peng , I D Williams

The collective response of matter is ubiquitous and widely exploited, e.g. in plasmonic, optical and electronic devices. Here we trace on an attosecond time scale the birth of collective excitations in a finite system and find distinct new…

Atomic and Molecular Clusters · Physics 2017-02-15 A. S. Moskalenko , Y. Pavlyukh , J. Berakdar

Time- and angle-resolved photoemission spectroscopy is a powerful technique for investigating the dynamics of excited carriers in quantum materials. Typically, data analysis proceeds via the inspection of time distribution curves (TDCs),…

Attosecond science promises to reveal the most fundamental electronic dynamics occurring in matter and it can develop further by meeting two linked technological goals related to high-order harmonic sources: higher photon flux (permitting…

Measuring and controlling the ionization dynamics by intense laser fields has recently led to important breakthroughs, from the investigation of tunneling time delays to attosecond molecular imaging by electron holography. In these…

Over the last three decades numerous numerical methods for solving the time-dependent Schr\"{o}dinger equation within the single-active electron approximation have been developed for studying ionization of atomic targets exposed to an…

Atomic Physics · Physics 2020-08-12 B. Fetić , W. Becker , D. B. Milošević