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The present work explores quantitative limits to the Single-Active Electron (SAE) approximation, often used to deal with strong-field ionization and subsequent attosecond dynamics. Using a time-dependent multi\-configuration approach,…

Atomic Physics · Physics 2025-11-04 Jean-Nicolas Vigneau , Tung Nguyen-Dang , Eric Charron , Osman Atabek

A molecular rotation assisted non-sequential double ionization (MR-NSDI) mechanism is identified in the breakup of rotational H$_2$ molecules in a few-cycle intense laser pulse using a semi-classical trajectory Monte Carlo method. Applying…

Atomic Physics · Physics 2022-05-31 Ahai Chen

Fully accounting for non-dipole effects in the electron dynamics, double ionization is studied for He driven by a near-infrared laser field and for Xe driven by a mid-infrared laser field. Using a three-dimensional semiclassical model, the…

Atomic Physics · Physics 2017-03-15 A. Emmanouilidou , T. Meltzer

We investigate the possibility to deduce momentum space properties from time-dependent density functional calculations. Electron and ion momentum distributions after double ionization of a model Helium atom in a strong few-cycle laser pulse…

Atomic Physics · Physics 2009-11-13 F. Wilken , D. Bauer

Recent experimental developments of high-intensity, short-pulse XUV light sources are enhancing our ability to study electron-electron correlations. We perform time-dependent calculations to investigate the so-called "sequential" regime…

Atomic Physics · Physics 2010-01-19 J. Feist , S. Nagele , R. Pazourek , E. Persson , B. I. Schneider , L. A. Collins , J. Burgdörfer

We investigate laser induced nonsequential multiple ionization using a simple statistical model in which an electron recollides inelastically with its parent ion. In this collision, it thermalizes with the remaining $N-1$ bound electrons…

Atomic Physics · Physics 2007-05-23 C. Figueira de Morisson Faria , X. Liu

Double ionization of diatomic molecules by short linearly polarized laser pulses is analyzed. We consider the final stage of the ionization process, that is the decay of a highly excited two electron molecule, which is formed after…

Atomic Physics · Physics 2016-09-08 Jakub S. Prauzner-Bechcicki , Krzysztof Sacha , Bruno Eckhardt , Jakub Zakrzewski

We calculate various differential and double differential characteristics of ionization by a single photon for H$^-$, He and for the two-electron ions with Z=3,4,5 in the region of the so-called quasi-free mechanism (QFM) domination. We…

Atomic Physics · Physics 2020-04-13 Miron Ya. Amusia , Evgeny G. Drukarev , Evgeny Z. Liverts

We present the momentum distributions of the nucleus and of the electrons from double ionization of the helium atom by Compton scattering of photons with $h\nu=40$ keV. We find that the doubly charged ion momentum distribution is very close…

We consider the process of double photoionization (DPI) in a rare gas atom as a two-step process, namely (i) photoionization in an inner shell followed by (ii) the emission of an Auger electron from an outer shell. An angular correlation…

Atomic Physics · Physics 2009-11-07 Dipankar Chattarji , Chiranjib Sur

Obtaining a detailed understanding of strong-field double ionisation of many-electron systems (heavy atoms and molecules) remains a challenging task. By comparing experimental and theoretical results in the mid-IR regime, we have…

A systematic QED treatment of electron correlation is presented for ions along the lithium isoelectronic sequence. We start with the zeroth-order approximation that accounts for a part of the electron-electron interaction by a local model…

Atomic Physics · Physics 2009-11-13 V. A. Yerokhin , A. N. Artemyev , V. M. Shabaev

We address the influence of the orbital symmetry and of the molecular alignment with respect to the laser-field polarization on laser-induced nonsequential double ionization of diatomic molecules, in the length and velocity gauges. We work…

Atomic Physics · Physics 2009-11-13 C. Figueira de Morisson Faria , T. Shaaran , X. Liu , W. Yang

The angular distribution of the emitted electrons, following the two-photon ionization of the hydrogen-like ions, is studied within the framework of second order perturbation theory and the Dirac equation. Using a density matrix approach,…

Atomic Physics · Physics 2007-05-23 Peter Koval , Stephan Fritzsche , Andrey Surzhykov

Double ionization of an atom by single-photon absorption in the presence of a neighbouring atom is studied. The latter is, first, resonantly photoexcited and, afterwards, transfers the excitation energy radiationlessly to the other atom,…

Atomic Physics · Physics 2020-02-19 A. Eckey , A. B. Voitkiv , C. Müller

We study double ionization (DI) dynamics of vibrating HeH$^+$ versus its isotopic variant HeT$^+$ in strong laser fields numerically. Our simulations show that for both cases, these two electrons in DI prefer to release together along the…

Atomic Physics · Physics 2020-03-18 S. Wang , R. H. Xu , W. Y. Li , X. Liu , W. Li , G. G. Xin , Y. J. Chen

We examine correlated electron and doubly charged ion momentum spectra from strong field double ionization of Neon employing intense elliptically polarized laser pulses. An ellipticity-dependent asymmetry of correlated electron and ion…

We perform a detailed analysis of the importance of causality within the strong-field approximation and the steepest descent framework for the recollision-excitation with subsequent tunneling ionization (RESI) pathway in laser-induced…

Atomic Physics · Physics 2012-02-29 T. Shaaran , C. Figueira de Morisson Faria , H. Schomerus

R-matrix with time-dependence theory is applied to electron-impact ionisation processes for He in the S-wave model. Cross sections for electron-impact excitation, ionisation and ionisation with excitation for impact energies between 25 and…

Atomic Physics · Physics 2016-09-21 Jack Wragg , Hugo W. van der Hart

At intensities below-the-recollision threshold, we show that re-collision-induced excitation with one electron escaping fast after re-collision and the other electron escaping with a time delay via a Coulomb slingshot motion is one of the…

Atomic Physics · Physics 2020-02-12 G. P. Katsoulis , A. Hadjipittas , B. Bergues , M. F. Kling , A. Emmanouilidou