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Coupling together distinct correlated and topologically non-trivial electronic phases of matter can potentially induce novel electronic orders and phase transitions among them. Transition metal dichalcogenide compounds serve as a bedrock…

Two-dimensional (2D) van der Waals (vdW) magnetic $3d$-transition metal trihalides are a new class of functional materials showing exotic physical properties useful for spintronic and memory storage applications. In this article, we report…

1T-TaS$_2$ undergoes successive phase transitions upon cooling and eventually enters an insulating state of mysterious origin. Some consider this state to be a band insulator with interlayer stacking order, yet others attribute it to Mott…

Strongly Correlated Electrons · Physics 2020-08-26 Y. D. Wang , W. L. Yao , Z. M. Xin , T. T. Han , Z. G. Wang , L. Chen , C. Cai , Yuan Li , Y. Zhang

Density functional theory calculations are used to systematically investigate the structural and electronic properties of MX$_2$ transition metal dichalcogenide monolayers with M = Cr, Mo, W and X = S, Se, Te that are doped with single (V,…

Materials Science · Physics 2024-01-03 Yuqiang Gao , Paul J. Kelly

The dimer Mott insulator $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ can be tuned into a metallic and superconducting state upon applying pressure of 1.5 kbar and more. We have performed dielectric spectroscopy measurements (7 kHz to 5 MHz) on…

Strongly Correlated Electrons · Physics 2021-03-17 R. Rösslhuber , A. Pustogow , E. Uykur , A. Böhme , A. Löhle , R. Hübner , J. Schlueter , Y. Tan , V. Dobrosavljević , M. Dressel

Strong electron-electron interaction can induce Mott insulating state, which is believed to host unusual correlated phenomena such as quantum spin liquid when quantum fluctuation dominates and unconventional superconductivity through…

Strongly Correlated Electrons · Physics 2025-04-24 Qiang Gao , Haiyang Chen , Wen-shin Lu , Yang-hao Chan , Zhenhua Chen , Yaobo Huang , Zhengtai Liu , Peng Chen

We present a combined density-functional theory and dynamical mean-field theory (DFT+DMFT) study of the full structural phase space of rutile-based vanadium dioxide (VO$_2$), including also the less studied M2 and T phases, using an…

Strongly Correlated Electrons · Physics 2026-03-30 Peter Mlkvik , Nicola A. Spaldin , Claude Ederer

Low-dimensional electron systems, as realized naturally in graphene or created artificially at the interfaces of heterostructures, exhibit a variety of fascinating quantum phenomena with great prospects for future applications. Once…

Strongly Correlated Electrons · Physics 2016-08-03 T. Ritschel , J. Trinckauf , K. Koepernik , B. Büchner , M. v. Zimmermann , H. Berger , Y. I. Joe , P. Abbamonte , J. Geck

We discuss the effect of the dielectric environment (insulators and metal gates) on electronic transport in two-dimensional (2D) transition metal dichalcogenides (TMD) monolayers. We employ well-known ab initio methods to calculate the…

Mesoscale and Nanoscale Physics · Physics 2022-08-24 Sanjay Gopalan , Maarten L. Van de Put , Gautam Gaddemane , Massimo V. Fischetti

Two recent electronic transport experiments from Columbia University and Harvard University have reported record high mobility and low channel densities in transition metal dichalcogenide (TMD) WSe$_2$ monolayers [J. Pack, et al.,…

Mesoscale and Nanoscale Physics · Physics 2024-06-28 Yi Huang , Sankar Das Sarma

Charge-density waves (CDWs) are correlated states of matter, where the electronic density is modulated periodically as a consequence of electronic and phononic interactions. Often, CDW phases coexist with other correlated states, such as…

Mesoscale and Nanoscale Physics · Physics 2025-01-24 Lisa M. Rütten , Eva Liebhaber , Kai Rossnagel , Katharina J. Franke

We study the structural, electronic and vibrational properties of single-layer 1TNbSe$_2$ from first principles. Within the generalized gradient approximation, the 1T polytype is highly unstable with respect to the 2H. The DFT+U method…

Materials Science · Physics 2018-07-18 Matteo Calandra

The applicability of DFT+$U$ to the star-of-David phase of $1T$-TaS$_2$ is examined. The viability of a Mott phase as a ground state for the bulk of this material is briefly discussed in light of the available experimental evidence.

Strongly Correlated Electrons · Physics 2023-08-14 Diego Pasquier

In this paper we critically discuss several examples of two-dimensional electronic systems displaying interaction-driven metal-insulator transitions of the Mott (or Wigner--Mott) type, including dilute two-dimension electron gases (2DEG) in…

Strongly Correlated Electrons · Physics 2022-07-04 Yuting Tan , Vladimir Dobrosavljevic , Louk Rademaker

Transition metal dichalcogenides (TMDs) host multiple competing structural and electronic phases, making them an ideal platform for constructing polytype heterostructures with emergent quantum properties. However, controlling phase…

Materials Science · Physics 2025-12-03 Yanyan Geng , Manyu Wang , Shumin Meng , Shuo Mi , Chang Li , Huiji Hu , Jianfeng Guo , Rui Xu , Fei Pang , Wei Ji , Weichang Zhou , Zhihai Cheng

Transition metal dichalcogenides (TMDs) exist in various crystal structures with semiconducting, semi-metallic, and metallic properties. The dynamic control of these phases is of immediate interest for next generation electronics such as…

Materials Science · Physics 2026-01-21 Dante Zakhidov , Daniel A. Rehn , Evan J. Reed , Alberto Salleo

We investigate the interplay of spin-orbit coupling, electronic correlations, and lattice distortions in the $5d^1$ double perovskite Ba$_2$MgReO$_6$. Combining density-functional theory (DFT) and dynamical mean-field theory (DMFT), we…

Strongly Correlated Electrons · Physics 2023-12-18 Maximilian E. Merkel , Aria Mansouri Tehrani , Claude Ederer

The low-temperature metallic phase of 1T-TaS2 may originate from current- and voltage-driven destabilization of the commensurate charge density wave (CDW) in a strongly correlated Mott insulator, alongside the robust yet rarely realized…

We study the conduction band spin splitting that arises in transition metal dichalcogenide (TMD) semiconductor monolayers such as MoS$_2$, MoSe$_2$, WS$_2$ and WSe$_2$ due to the combination of spin-orbit coupling and lack of inversion…

Materials Science · Physics 2014-01-01 K. Kośmider , J. W. González , J. Fernández-Rossier

Single layer (SL) two-dimensional transition metal dichalcogenides (TMDs), such as MoS2, ReS2, WSe2, and MoTe2 have now become the focus of intensive fundamental and applied researches due to their intriguing and tunable physical…

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