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The commensurate charge-density-wave phase of the prototypical transition metal dichalcogenide $1T$-TaS$_2$ is investigated by temperature- and polarization-dependent infrared spectroscopy, revealing distinct charge dynamics parallel and…

Strongly Correlated Electrons · Physics 2026-01-21 Achyut Tiwari , Maxim Wenzel , Renjith Mathew Roy , Christian Prange , Bruno Gompf , Martin Dressel

Compelling evidence suggests distinct correlated electron behavior may exist only in clean 2D materials such as 1T-TaS2. Unfortunately, experiment and theory suggest that extrinsic disorder in free standing 2D layers disrupts…

1$T$-TaSe$_2$ is widely believed to host a Mott metal-insulator transition in the charge density wave (CDW) phase according to the spectroscopic observation of a band gap that extends across all momentum space. Previous investigations…

Strongly Correlated Electrons · Physics 2023-04-17 C. J. Sayers , G. Cerullo , Y. Zhang , C. E. Sanders , R. T. Chapman , A. S. Wyatt , G. Chatterjee , E. Springate , D. Wolverson , E. Da Como , E. Carpene

Transitions between different charge density wave (CDW) states in quasi-two-dimensional materials may be accompanied also by changes in the inter-layer stacking of the CDW. Using MeV ultrafast electron diffraction, the out-of-plane stacking…

Materials Science · Physics 2017-11-09 L. Le Guyader , T. Chase , A. Reid , R. K. Li , D. Svetin , X. Shen , T. Vecchione , X. J. Wang , D. Mihailovic , H. A. Dürr

Thinning crystalline materials to two dimensions (2D) creates a rich playground for electronic phases, including charge, spin, superconducting, and topological order. Bulk materials hosting charge density waves (CDWs), when reduced to…

For layered materials, the interlayer stacking is a critical degree of freedom tuning electronic properties, while its microscopic characterization faces great challenges. The transition-metal dichalcogenide 1T-TaS$_2$ represents a novel…

Materials Science · Physics 2025-08-01 Li Cheng , Linpeng Nie , Xuanyu Long , Li Liang , Dan Zhao , Jian Li , Zheng Liu , Tao Wu , Xianhui Chen , Xiaolong Zou

The layered transition metal dichalcogenide, TaSe2, exhibits rich electronic phenomena across its polymorphs, 1T, 2H, and 3R, largely driven by differences in atomic coordination and c-axis stacking. In the 1T phase, octahedral coordination…

Superconductivity · Physics 2026-02-13 Kusal Dharmasiri , Maxim Avdeev , Despina Louca

Two-dimensional layered transition metal dichalcogenide (TMDC) materials often exhibit exotic quantum matter phases due to the delicate coupling and competitions between the charge, lattice, orbital, and spin degrees of freedom.…

Mesoscale and Nanoscale Physics · Physics 2018-02-07 Seho Yi , Zhenyu Zhang , Jun-Hyung Cho

Two-dimensional (2D) materials have become a fertile playground for the exploration and manipulation of novel collective electronic states. Recent experiments have unveiled a variety of robust 2D orders in highly-crystalline materials…

Quantum states of strongly correlated electrons are of prime importance to understand exotic properties of condensed matter systems and the controllability over those states promises unique electronic devices such as a Mott memory. As a…

Materials Science · Physics 2017-07-12 Doohee Cho , Sangmo Cheon , Ki-Seok Kim , Sung-Hoon Lee , Yong-Heum Cho , Sang-Wook Cheong , Han Woong Yeom

We investigate the charge density wave (CDW) instability in single and double layers, as well as in the bulk 2H-NbSe$_{2}$. We demonstrate that the density functional theory correctly describes the metallic CDW state in the bulk…

Materials Science · Physics 2015-05-14 Matteo Calandra , I. I. Mazin , Francesco Mauri

Two-dimensional layered transition-metal-dichalcogenide compound 1T-TaS2 shows the rare coexistence of charge density wave (CDW) and electron correlation driven Mott transition. In addition, atomic-cluster spins on the triangular lattice of…

Strongly Correlated Electrons · Physics 2022-07-28 Sudip Pal , Kranti Kumar , Rohit Sharma , A Banerjee , S B Roy , Je-Geun Park , A. K. Nigam , Sang-Wook Cheong

We present the discovery of a charge density wave (CDW) ground state in heavily electron-doped molybdenum disulfide (MoS$_2$). This is the first observation of a CDW in any $d^2$ (column 6) transition metal dichalcogenide (TMD). The band…

Two-dimensional (2D) 1T-VSe$_2$ has prompted significant interest due to the discrepancies regarding alleged ferromagnetism (FM) at room temperature, charge density wave (CDW) states and the interplay between the two. We employed a combined…

By quantitative low-energy electron diffraction (LEED) we investigate the extensively studied commensurate charge density wave (CDW) phase of trigonal tantalum disulphide (1T-TaS$_2$), which develops at low temperatures with a…

Layered van der Waals materials are exciting as they often host multiple, competing electronic phases. This article reports experimental observation of the co-existence of insulating and metallic phases deep within the commensurate charge…

Mesoscale and Nanoscale Physics · Physics 2021-12-23 Sruthi S , Hemanta Kumar Kundu , Prasad Vishnubhotla , Aveek Bid

The coexistence of charge density wave (CDW) and superconductivity in tantalum disulfide (2H-TaS$_2$) at ambient pressure, is boosted by applying hydrostatic pressures up to 30GPa, thereby inducing a typical dome-shaped superconducting…

We have investigated the influence of potassium intercalation on the formation of the charge-density wave (CDW) instability in 2H-tantalum diselenide by means of Electron Energy-Loss Spectroscopy and density functional theory. Our…

Strongly Correlated Electrons · Physics 2015-06-11 A. König , K. Koepernik , R. Schuster , R. Kraus , M. Knupfer , B. Büchner , H. Berger

Transition metal dichalcogenides (TMDs) are a class of widely studied 2D layered materials which exist in various polymorphs. The 1T' phase of MoTe2 is of prime importance as it has been reported to show quantum spin hall (QSH) behavior…

Strongly Correlated Electrons · Physics 2021-07-06 Suvodeep Paul , Saheb Karak , Manasi Mandal , Ankita Ram , Sourav Marik , R. P. Singh , Surajit Saha

Using classical density functional theory (DFT) in a modified mean-field approximation we investigate the fluid phase behavior of quasi-two dimensional dipolar fluids confined to a plane. The particles carry three-dimensional dipole moments…

Statistical Mechanics · Physics 2013-06-18 R. Geiger , S. H. Klapp