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We present an experimental study of the pyrochlore coumpound Nd2Zr2O7 by means of neutron scattering and magnetization measurements down to 90 mK. The Nd$^{3+}$ magnetic moments exhibit a strong local $\langle$111$\rangle$ Ising anisotropy…

Strongly Correlated Electrons · Physics 2016-01-05 E. Lhotel , S. Petit , S. Guitteny , O. Florea , M. Ciomaga Hatnean , C. Colin , E. Ressouche , M. R. Lees , G. Balakrishnan

The rare earth pyrochlore magnet Yb2Ti2O7 is among a handful of materials that apparently exhibit no long range order down to the lowest explored temperatures and well below the Curie-Weiss temperature. Paramagnetic neutron scattering on a…

Statistical Mechanics · Physics 2011-04-11 J. D. Thompson , P. A. McClarty , M. J. P. Gingras

Our single-crystal polarized neutron scattering at 65 mK and powder unpolarized neutron diffraction at 0.5 K show no evidence for a long-range magnetic order and even detect no sign of diffuse magnetic neutron scattering in single-crystal…

Strongly Correlated Electrons · Physics 2016-03-17 Haifeng Li , Binyang Hou , Andrew Wildes , Anatoliy Senyshyn , Karin Schmalzl , Wolfgang Schmidt , Cong Zhang , Thomas Brueckel , Georg Roth

Pyrochlores offer an ideal playground to investigate the magnetic ground state of frustrated magnetic systems. In this class of materials, competition between various magnetic interactions remains frustrated and prevents an ordered magnetic…

Strongly Correlated Electrons · Physics 2022-10-06 Karan Singh , Dheeraj Ranaut , G. Sharma , K. Mukherjee

Tb2Ti2O7 is a pyrochlore antiferromagnet that has dynamical spins and only short-range correlations even at 50 mK; the lowest temperature explored so far, which is much smaller than the scale set by the Curie-Weiss temperature T_{CW}~14 K.…

Statistical Mechanics · Physics 2009-12-16 Hamid R. Molavian , Paul A. McClarty , Michel J. P. Gingras

A single crystal of the Co2+ based pyrochlore NaCaCo2F7 was studied by inelastic neutron scattering. This frustrated magnet with quenched exchange disorder remains in a strongly correlated paramagnetic state down to one 60th of the…

Strongly Correlated Electrons · Physics 2016-02-03 Kate A. Ross , Jason W. Krizan , Jose A. Rodriguez-Rivera , Robert J. Cava , Collin L. Broholm

We report temperature dependence of low-energy phonons in magnetic nonsuperconducting TbNi2B2C single crystals measured by inelastic neutron scattering. We observed a low-temperature softening and broadening of two phonon branches,…

Superconductivity · Physics 2011-09-16 S. Anissimova , A. Kreyssig , O. Stockert , M. Loewenhaupt , D. Reznik

We report time-of-flight neutron scattering measurements of the magnetic spectrum of Tb3+ in Tb2Ti2O7. The data, which extend up to 120 meV and have calibrated intensity, enable us to consolidate and extend previous studies of the…

Strongly Correlated Electrons · Physics 2015-09-04 A. J. Princep , H. C. Walker , D. T. Adroja , D. Prabhakaran , A. T. Boothroyd

The superconducting and magnetic properties of HoNi2B2C single crystals are investigated through transport, magnetometry and small-angle neutron scattering measurements. In the magnetic phases that enter below the superconducting critical…

Superconductivity · Physics 2015-06-19 M. Ramazanoglu , M. Laver , A. Yagmurcu , E. -M. Choi , S. -I. Lee , A. Knigavko , B. D. Gaulin

We present a model of the lattice dynamics of the rare earth titanate pyrochlores R2Ti2O7 (R=Tb, Dy, Ho), which are important materials in the study of frustrated magnetism. The phonon modes are obtained by density functional calculations,…

Neutron scattering and magnetization measurements have been performed on the stuffed pyrochlore system Tb2+xTi2-2xNbxO7. We find that despite the introduction of chemical disorder and increasingly antiferromagnetic interactions, a spin…

Strongly Correlated Electrons · Physics 2010-02-25 B. G. Ueland , J. S. Gardner , A. J. Williams , M. L. Dahlberg , J. G. Kim , Y. Qiu , J. R. D. Copley , P. Schiffer , R. J. Cava

We investigate the temperature dependence of the spin dynamics in the pyrochlore magnet Nd$_2$Zr$_2$O$_7$ by neutron scattering experiments. At low temperature, this material undergoes a transition towards an "all in - all out"…

Strongly Correlated Electrons · Physics 2021-07-22 M. Léger , E. Lhotel , M. Ciomaga Hatnean , J. Ollivier , A. R. Wildes , S. Raymond , E. Ressouche , G. Balakrishnan , S. Petit

At low temperatures, Tb$_2$Ti$_2$O$_7$ enters a spin liquid state, despite expectations of magnetic order and/or a structural distortion. Using neutron scattering, we have discovered that in this spin liquid state an excited crystal field…

Strongly Correlated Electrons · Physics 2014-01-16 T. Fennell , M. Kenzelmann , B. Roessli , H. Mutka , J. Ollivier , M. Ruminy , U. Stuhr , O. Zaharko , L. Bovo , A. Cervellino , M. K. Haas , R. J. Cava

The ytterbium pyrochlore magnets, Yb2B2O7 (B = Sn, Ti, Ge) are well described by S_eff = 1/2 quantum spins decorating a network of corner-sharing tetrahedra and interacting via anisotropic exchange. Structurally, only the non-magnetic…

Strongly Correlated Electrons · Physics 2016-03-30 A. M. Hallas , J. Gaudet , N. P. Butch , M. Tachibana , R. S. Freitas , G. M. Luke , C. R. Wiebe , B. D. Gaulin

The spin glass behavior of Y2Mo2O7 has puzzled physicists for nearly three decades. Free of bulk disorder within the resolution of powder diffraction methods, it is thought that this material is a rare realization of a spin glass resulting…

The quasi-one-dimensional antiferromagnetic Ising-like compound BaCo2V2O8 has been shown to be describable by the Tomonaga-Luttinger liquid theory in its gapless phase induced by a magnetic field applied along the Ising axis. Above 3.9 T,…

Strongly Correlated Electrons · Physics 2015-08-11 B. Grenier , V. Simonet , B. Canals , P. Lejay , M. Klanjsek , M. Horvatic , C. Berthier

In a recent letter [Phys. Rev. Lett. {\bf 82}, 1012 (1999)] it was found that the Tb$^{3+}$ magnetic moments in the Tb$_2$Ti$_2$O$_7$ pyrochlore lattice of corner-sharing tetrahedra remain in a {\it collective paramagnetic} state down to…

Disordered Systems and Neural Networks · Physics 2009-10-31 M. J. P. Gingras , B. C. den Hertog , M. Faucher , J. S. Gardner , L. J. Chang , B. D. Gaulin , N. P. Raju , J. E. Greedan

High resolution time-of-flight neutron scattering measurements on Tb2Ti2O7 reveal a rich low temperature phase diagram in the presence of a magnetic field applied along [110]. In zero field at T=0.4 K, terbium titanate is a highly…

Detailed neutron diffraction measurements on a single crystalline ErB$_2$C$_2$ were performed. We observed magnetic diffuse scattering which consists of three components just above the transition temperatures, which is also observed in…

Strongly Correlated Electrons · Physics 2009-11-10 Kenji Ohoyama , Kentaro Indoh , Aya Tobo , Koji Kaneko , Aya Hino , Hideya Onodera

We have investigated the magnetic diffuse scattering of isostructural $S$ = 5/2 fcc antiferromagnets Ba$_2$MnTeO$_6$ and Ba$_2$MnWO$_6$ using polarized neutrons. Both materials display short-range correlated magnetism above their respective…