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Transient grating spectroscopy has become a mainstay among metal and semiconductor characterization techniques. Here we extend the technique towards the shortest achievable timescales by using tabletop high-harmonic generation of attosecond…

Attosecond pulses from free-electron lasers have opened the doors to atomic site-specific pumping and probing of quantum systems. Key to their success has been electron beam shaping techniques enabling the generation of sub-femtosecond…

A practical approach is proposed for efficiently generating ultrashort attosecond pulses (APs) from realistic solid-state materials, aiming to optimize pulse width effectively. By adjusting the photon energy while maintaining a constant…

Optics · Physics 2025-02-25 Xinyuan Zhang , Shiqi Hu , Mengxue Guan , Sheng Meng

We report on the first streaking measurement of water-window attosecond pulses generated via high harmonic generation, driven by sub-2-cycle, CEP-stable, 1850 nm laser pulses. Both the central photon energy and the energy bandwidth far…

High-repetition-rate attosecond pulse sources are indispensable tools of time-resolved studies of electron dynamics, such as coincidence spectroscopy and experiments with high demands on statistics or signal-to-noise ratio, especially in…

Attosecond x-ray pulses play a crucial role in the study of ultrafast phenomena occurring within inner and valence electrons. Especially isolated attosecond pulses with high photon energy and high peak power are of great significance in…

Accelerator Physics · Physics 2024-09-06 Hao Sun , Xiaofan Wang , Li Zeng , Weiqing Zhang

High-order harmonic generation by few-cycle 800 nm laser pulses in neon gas in the presence of a strong terahertz (THz) field is investigated numerically with propagation effects taken into account. Our calculations show that the…

The field of attosecond science was first enabled by nonlinear compression of intense laser pulses to a duration below two optical cycles. Twenty years later, creating such short pulses still requires state-of-the-art few-cycle laser…

The sub-atomic experimental exploration of physical processes on extremely short time scales has become possible by the generation of high quality electron bunches and x-ray pulses with sub-femtosecond durations. Temporal coherence is…

Plasma Physics · Physics 2019-01-16 Zsolt Lécz , Alexander Andreev

Many experiments in attosecond science will benefit from attosecond pulses at high repetition rates with sufficient photon flux for pump-probe experiments. We use 7fs, 800nm pulses from a non-collinear optical parametric chirped pulse…

In this work we demonstrate the generation of two intense, ultrafast laser pulses that allow a controlled interferometric measurement of higher harmonic generation pulses with 12.8 attoseconds in resolution (half the atomic unit of time)…

Atomic Physics · Physics 2019-09-04 Jan Troß , Georgios Kolliopoulos , Carlos A. Trallero-Herrero

Attosecond pulses provide unique opportunities for studies of time-resolved electron dynamics. However, focusing these pulses, typically ranging from the vacuum ultraviolet to the soft-X-ray region, remains challenging. Conventional…

Attosecond streaking, as a measurement technique, was originally conceived as a means to characterize attosecond light pulses, which is a good approximation if the relevant transition matrix elements are approximately constant within the…

Atomic Physics · Physics 2015-05-19 Vladislav S. Yakovlev , Justin Gagnon , Nicholas Karpowicz , Ferenc Krausz

Quantum-mechanical investigation is presented to study single attosecond pulse generation by gating high-order harmonic emission from H$_2^+$ molecule in intense laser pulses with time-dependent ellipticity. The high-order harmonic…

Atomic Physics · Physics 2018-01-17 Nehzat Safaei

Ultra-short laser pulses with femtosecond to attosecond pulse duration are the shortest systematic events humans can create. Characterization (amplitude and phase) of these pulses is a key ingredient in ultrafast science, e.g., exploring…

Optics · Physics 2018-03-19 Tom Zahavy , Alex Dikopoltsev , Oren Cohen , Shie Mannor , Mordechai Segev

We present the first direct experimental confirmation of attosecond pulse generation in the hard X-ray regime with a free-electron laser. Our experiment is based on measurements of a nonlinear optical phenomenon known as amplified…

We report the generation of intense deep ultraviolet pulses at 200 nm with a duration of 48 fs and pulse energy of 130 uJ, achieved via cascaded sum frequency generation using 800 nm femtosecond pulses in barium borate crystals. Efficient…

Optics · Physics 2025-07-04 X. Xie , S. Soultanis , G. Knopp , A. L. Cavalieri , S. L. Johnson

We report on the development of tunable few-cycle pulses with central wavelengths from 1.6 um to 2 um. Theses pulses were used as a proof of principle for high harmonic generation in atomic and molecular targets. In order to generate such…

We explore stimulated photo-association in the context of attosecond pump-probe schemes of atomic matter. An attosecond pulse -- the probe -- is used to induce photo-association of an electronic wave packet which had been created before,…

Atomic Physics · Physics 2009-11-13 Paula Rivière , Camilo Ruiz , Jan-Michael Rost