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We study the magnetic properties of small Mn ring shaped clusters on a Pt(111) surface in the framework of density functional theory. We find that the Mn atoms possess large magnetic moments, of the order of 4uB/atom, and have dominating…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 M. S. Ribeiro , G. B. Corrêa , A. Bergman , L. Nordström , O. Eriksson , A. B. Klautau

We report on the crystal structure of the quantum magnet (CuCl)LaNb2O7 that was controversially described with respect to its structural organization and magnetic behavior. Using high-resolution synchrotron powder x-ray diffraction,…

Materials Science · Physics 2015-03-17 Alexander A. Tsirlin , Artem M. Abakumov , Gustaaf Van Tendeloo , Helge Rosner

We report the electronic structure and magnetic ordering of the single molecule magnet [Mn$_{10}$O$_{4}$(2,2'-biphenoxide)$_{4}$Br$_{12}$]$^{4-}$ based on first-principles all-electron density-functional calculations. We find that two of…

Materials Science · Physics 2009-11-07 Jens Kortus , Tunna Baruah , N. Bernstein , Mark R. Pederson

The phase diagram of weakly coupled $XXZ$ chains in a transverse magnetic field is studied using the mean-field approximation for the interchain coupling and known exact results for an effective one-dimensional model. Results are applied to…

Strongly Correlated Electrons · Physics 2009-11-10 D. V. Dmitriev , V. Ya. Krivnov

Cu(pz)$_2$(ClO$_4$)$_2$ (with pz denoting pyrazine C$_4$H$_4$N$_2$) is a two-dimensional spin-1/2 square-lattice antiferromagnet with $T_{\mathrm{N}}$ = 4.24 K. Due to a persisting focus on the low-temperature magnetic properties, its…

Materials Science · Physics 2023-10-24 N. Barbero , M. Medarde , T. Shang , D. Sheptyakov , C. P. Landee , J. Mesot , H. -R. Ott , T. Shiroka

The T=0 dynamical properties of the one-dimensional (1D) $s=1/2$ Heisenberg antiferromagnet in a uniform magnetic field are studied via Bethe ansatz for cyclic chains of $N$ sites. The ground state at magnetization $0<M_z<N/2$, which can be…

Strongly Correlated Electrons · Physics 2009-11-07 Michael Karbach , Daniel Biegel , Gerhard Muller

We present the results of a muon-spin relaxation (muSR) investigation into magnetic ordering in several families of layered quasi-two-dimensional molecular antiferromagnets based on transition metal ions such as S=1/2 Cu2+ bridged with…

We study the effects of Cu substitution in Fe1.1Te, the non-superconducting parent compound of the iron-based superconductor, Fe1+yTe1-xSex, utilizing neutron scattering techniques. It is found that the structural and magnetic transitions,…

We determined the crystal structure of Cs$_2$LiRuCl$_6$, which was synthesized first in this work, and investigated its magnetic properties. Cs$_2$LiRuCl$_6$ has a hexagonal structure composed of linear chains of face-sharing RuCl$_6$ and…

We show that the magnetism of double perovskite AFe_{1/2}M_{1/2}O_3 systems may be described by the Heisenberg model on the simple cubic lattice, where only half of sites are occupied by localized magnetic moments. The nearest-neighbor…

Materials Science · Physics 2015-01-16 R. O. Kuzian , I. V. Kondakova , A. -M. Dare , V. V. Laguta

Alternating current susceptibility and direct current magnetization have been studied for polycrystalline Ca$_{1-x}$Mn$_x$O. On increasing the Mn content, magnetic ordering changes from spin-glass behavior for $0.25 \leqslant x \leqslant…

Materials Science · Physics 2007-05-23 S. Kolesnik , B. Dabrowski

In this review, we present a summary of experimental studies of magnetism in Fe-based superconductors. The doping dependent phase diagram shows strong similarities to the generic phase diagram of the cuprates. Parent compounds exhibit…

Superconductivity · Physics 2010-05-19 M. D. Lumsden , A. D. Christianson

We investigate magnetic properties of the $s$ = 1/2 compound K$_{2}$Cu$_{3}$(MoO$_{4}$)$_{4}$ by combining magnetic susceptibility, magnetization, specific heat, and electron spin resonance (ESR) with density functional calculations. Its…

Exploring the uncharacterized magnetic phases of Co$^{2+}$ chain compounds is critical for finding new low-dimensional magnets hosting quantized excitations. We map the unexplored magnetic phases of the Co$^{2+}$ chain compound…

Strongly Correlated Electrons · Physics 2023-10-18 Zachary W. Riedel , Zhihao Jiang , Maxim Avdeev , André Schleife , Daniel P. Shoemaker

We present a study of the magnetic susceptibility $\chi_{mol}$ under variable hydrostatic pressure on single crystals of Cs$_2$CuCl$_{4-x}$Br$_x$. This includes the border compounds \textit{x} = 0 and 4, known as good realizations of the…

Strongly Correlated Electrons · Physics 2019-10-23 S. K. Thallapaka , B. Wolf , E. Gati , L. Postulka , U. Tutsch , B. Schmidt , P. Thalmeier , F. Ritter , C. Krellner , Y. Li , V. Borisov , R. Valentí , M. Lang

Elastic and inelastic neutron scattering were used to study the ordered phase of the quasi-one-dimensional spin-1/2 antiferromagnet ${\rm BaCu_{2}Si_{2}O_{7}}$. The previously proposed model for the low-temperature magnetic structure was…

Strongly Correlated Electrons · Physics 2016-08-15 M. Kenzelmann , A. Zheludev , S. Raymond , E. Ressouche , T. Masuda , P. Böni , K. Kakurai , I. Tsukada , K. Uchinokura , R. Coldea

A detailed investigation of Ba$_2$MnGe$_2$O$_7$ was performed in its low-temperature magnetoelectric state combining neutron diffraction with magnetization measurements on single crystals. In the paramagnetic state at 10 K, polarized…

Strongly Correlated Electrons · Physics 2023-03-07 A. Sazonov , H. Thoma , R. Dutta , M. Meven , A. Gukasov , R. Fittipaldi , V. Granata , T. Masuda , B. Náfrádi , V. Hutanu

The magnetic properties and the spin dynamics of two molecular magnets have been investigated by magnetization and d.c. susceptibility measurements, Electron Paramagnetic Resonance (EPR) and proton Nuclear Magnetic Resonance (NMR) over a…

Materials Science · Physics 2017-12-06 P. Khuntia , M. Mariani , M. C. Mozzati , L. Sorace , F. Orsini , A. Lascialfari , F. Borsa , M. Andruh , C. Maxim

Magnetic properties of two and three-dimensional clusters of quantum dots are studied with exact diagonalization of a generalized Hubbard model. We study the weak coupling limit, where the electrons interact only within a quantum dot and…

Strongly Correlated Electrons · Physics 2009-11-13 J. -P. Nikkarila , M. Koskinen , M. Manninen

Through analysis of single crystal neutron diffraction data, we present the magnetic structures of magnetoelectric Co4Nb2O9 under various magnetic fields. In zero-field, neutron diffraction experiments below TN=27 K reveal that the Co2+…

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