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A permanently available molecular-beam injection setup for controlled molecules (COMO) was installed and commissioned at the small quantum systems (SQS) instrument at the European x-ray free-electron laser (EuXFEL). A $b$-type electrostatic…

Beams of atoms and molecules are stalwart tools for spectroscopy and studies of collisional processes. The supersonic expansion technique can create cold beams of many species of atoms and molecules. However, the resulting beam is typically…

Atomic Physics · Physics 2012-10-02 Nicholas R. Hutzler , Hsin-I Lu , John M. Doyle

Helium nanodroplets doped with polar molecules are studied by electrostatic deflection. This broadly applicable method allows even polyatomic molecules to attain sub-Kelvin temperatures and nearly full orientation in the field. The…

Atomic and Molecular Clusters · Physics 2019-07-26 John W. Niman , Benjamin S. Kamerin , Daniel J. Merthe , Lorenz Kranabetter , Vitaly V. Kresin

We present a new concept for a multi-stage Zeeman decelerator that is optimized particularly for applications in molecular beam scattering experiments. The decelerator consists of a series of alternating hexapoles and solenoids, that…

We report a compact single-cell source of a continuous cold-atom beam with three-dimensional (3D) cooling. By integrating an off-axis moving optical molasses (OM) with a two-dimensional magneto-optical trap (MOT), we achieve simultaneous 3D…

Atomic Physics · Physics 2026-04-17 Sheng-Zhe Wang , Qian-Lan Cai , Zhi-Xin Meng , Yi-Cheng Deng , Yan-Ying Feng

Typical sources of ultracold atoms operate with a considerable delay between the delivery of ensembles due to sequential trapping and cooling schemes. Therefore, alternative schemes for the continuous generation of ultracold atoms are…

Quantum Physics · Physics 2015-11-23 J. Mahnke , I. Kruse , A. Hüper , S. Jöllenbeck , W. Ertmer , J. Arlt , C. Klempt

We present an opto-electrical cooling scheme for polar molecules based on a Sisyphus-type cooling cycle in suitably tailored electric trapping fields. Dissipation is provided by spontaneous vibrational decay in a closed level scheme found…

Quantum Physics · Physics 2009-10-07 M. Zeppenfeld , M. Motsch , P. W. H. Pinkse , G. Rempe

A simple method to control molecular translation with a chemical reaction is demonstrated. Slow NO molecules have been produced by partially canceling the molecular beam velocity of NO$_2$ with the recoil velocity of the NO photofragment.…

Chemical Physics · Physics 2009-09-10 Bum Suk Zhao , So Eun Shin , Sung Tai Park , Xingnan Sun , Doo Soo Chung

A novel type of particle "cooling", called Ionization Cooling, is applicable to slow (v of the order of 0.1c) ions stored in a small ring. The many traversals through a thin foil enhance the nuclear reaction probability, in a steady…

High Energy Physics - Phenomenology · Physics 2011-05-18 C. Rubbia , A. Ferrari , Y. Kadi , V. Vlachoudis

Controlling the internal degrees of freedom is a key challenge for applications of cold and ultracold molecules. Here, we demonstrate rotational-state cooling of trapped methyl fluoride molecules (CH3F) by optically pumping the population…

We show, through modeling and simulation, that it is feasible to construct a storage ring that will store dense bunches of strong-field-seeking polar molecules at 30 m/s (kinetic energy of 2K) and hold them, for several minutes, against…

Accelerator Physics · Physics 2009-11-11 Hiroshi Nishimura , Glen Lambertson , Juris G. Kalnins , Harvey Gould

A continuous guided atomic beam of $^{88}\mathrm{Sr}$ with a phase-space density exceeding $10^{-4}$ in the moving frame and a flux of $3 \times 10^{7} \, \mathrm{at \, s^{-1}}$ is demonstrated. This phase-space density is around three…

Coherent optical bichromatic forces have been shown to be effective tools for rapidly slowing and cooling simple atomic systems. While previous estimates suggest that these forces may also be effective for rapidly decelerating molecules or…

Atomic Physics · Physics 2016-01-27 L. Aldridge , S. E. Galica , E. E. Eyler

Stark deceleration is a technique that uses time-varying inhomogeneous electric fields to decelerate polar molecules for various molecular beam and trapping experiments. New ring-geometry Stark decelerators with continuously varying…

Chemical Physics · Physics 2017-12-20 Yomay Shyur , Jason A. Bossert , H. J. Lewandowski

Electrostatic velocity filtering and guiding is an established technique to produce high fluxes of cold polar molecules. In this paper we clarify different aspects of this technique by comparing experiments to detailed calculations. In the…

Chemical Physics · Physics 2009-01-14 M. Motsch , L. D. van Buuren , C. Sommer , M. Zeppenfeld , G. Rempe , P. W. H. Pinkse

We report direct laser cooling of a symmetric top molecule, reducing the transverse temperature of a beam of calcium monomethoxide (CaOCH$_3$) to $1.8\pm0.7$ mK while addressing two distinct nuclear spin isomers. These results open a path…

We demonstrate a cryogenic buffer gas-cooled molecular beam source capable of producing bright, continuous beams of cold and slow free radicals via laser ablation over durations of up to 60~seconds. The source design uses a closed liquid…

Atomic Physics · Physics 2020-10-28 J. C. Shaw , D. J. McCarron

We have demonstrated a new, accessible and economical technique, dubbed photostop, for producing high densities of trappable molecules. Direct measurements are presented of NO molecules produced with a narrow velocity distribution centered…

Chemical Physics · Physics 2013-08-12 Alexandre Trottier , David Carty , Eckart Wrede

A new regime is described for Radiation Pressure Acceleration of a thin foil by an intense laser beam of above 10^20 W/cm^2. Highly monoenergetic proton beams extending to GeV energies can be produced with very high efficiency using…

Plasma Physics · Physics 2009-11-13 A. P. L. Robinson , M. Zepf , S. Kar , R. G. Evans , C. Bellei

We present a study of Sisyphus cooling of molecules: the scattering of a single-photon remove a substantial amount of the molecular kinetic energy and an optical pumping step allow to repeat the process. A review of the produced cold…

Chemical Physics · Physics 2014-04-11 Daniel Comparat
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