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We have focused and decelerated benzonitrile (C$_7$H$_5$N) molecules from a molecular beam, using an array of time-varying inhomogeneous electric fields in alternating gradient configuration. Benzonitrile is prototypical for large…

We describe the production of cold, slow-moving LiH molecules. The molecules are produced in the ground state using laser ablation and supersonic expansion, and 68% of the population is transferred to the rotationally excited state using…

Atomic Physics · Physics 2015-05-13 S. K. Tokunaga , J. M. Dyne , E. A. Hinds , M. R. Tarbutt

We present a cold atomic beam source based on a two-dimensional (2D)+ magneto-optical trap (MOT), capable of generating a continuous cold beam of 87Rb atoms with a flux up to 4.3*10^9 atoms/s, a mean velocity of 10.96(2.20) m/s, and a…

Atomic Physics · Physics 2023-12-20 Shengzhe Wang , Zhixin Meng , and Peiqiang Yan , Yuanxing Liu , Yanying Feng

In this paper we describe the high-voltage generation system we have developed for a traveling-wave Stark decelerator (TWSD). The TWSD can reduce the forward velocity of a molecular beam of heavy neutral polar molecules such as strontium…

Atomic Physics · Physics 2026-02-12 Lucas van Sloten , Leo Huisman , Steven Hoekstra

A special class of molecules that are important to many subfields in molecular dynamics and chemical physics, namely free radical molecules, now enjoy a significant degree of center-of-mass motion control in the laboratory frame. The…

Atomic Physics · Physics 2009-11-10 J. R. Bochinski , Eric R. Hudson , H. J. Lewandowski , Jun Ye

We introduce a scheme for deep laser cooling of molecules based on robust dark states at zero velocity. By simulating this scheme, we show it to be a widely applicable method that can reach the recoil limit or below. We demonstrate and…

Atomic Physics · Physics 2019-07-24 L. Caldwell , J. A. Devlin , H. J. Williams , N. J. Fitch , E. A. Hinds , B. E. Sauer , M. R. Tarbutt

We here report on the implementation of a microwave lens for neutral polar molecules suitable to focus molecules both in low-field-seeking and in high-field-seeking states. By using the TE_11m modes of a 12 cm long cylindrically symmetric…

Chemical Physics · Physics 2010-06-30 Hitoshi Odashima , Simon Merz , Katsunari Enomoto , Melanie Schnell , Gerard Meijer

We demonstrate and characterize a high-flux beam source for cold, slow atoms or molecules. The desired species is vaporized using laser ablation, then cooled by thermalization in a cryogenic cell of buffer gas. The beam is formed by…

We demonstrate slowing and longitudinal cooling of a supersonic beam of CaF molecules using counter-propagating laser light resonant with a closed rotational and almost closed vibrational transition. A group of molecules are decelerated by…

We have produced a cryogenic buffer-gas cooled beam of the diatomic molecular radical CH (methylidyne). This molecule is of interest for studying cold chemical reactions and fundamental physics measurements. Its light mass and ground-state…

We realize a novel high flux source of cold atoms and molecules employing hydrodynamic enhancement of an effusive aperture at cryogenic temperatures. Molecular oxygen from the source is coupled to a magnetic guide, delivering a cold,…

Chemical Physics · Physics 2007-05-23 David Patterson , John M. Doyle

Strong optical forces with minimal spontaneous emission are desired for molecular deceleration and atom interferometry applications. We report experimental benchmarking of such a stimulated optical force driven by ultrafast laser pulses. We…

Atomic Physics · Physics 2019-07-23 Xueping Long , Scarlett S. Yu , Andrew M. Jayich , Wesley C. Campbell

We demonstrate an intense, continuous cold atom beam generated via post nozzle seeding of a supersonic helium jet with $^7$Li atoms. The nozzle is cooled to about 4.4 K to reduce the forward velocity of the atoms. The atomic beam is brought…

Atomic Physics · Physics 2023-01-18 William Huntington , Jeremy Glick , Michael Borysow , Daniel J. Heinzen

Multistage Zeeman deceleration is a technique used to reduce the velocity of neutral molecules with a magnetic dipole moment. Here we present a Zeeman decelerator that consists of 100 solenoids and 100 magnetic hexapoles, that is based on a…

We examine two approaches for significantly extending the velocity range of the optical bichromatic force (BCF), to make it useful for laser deceleration of atomic and molecular beams. First, we present experimental results and calculations…

Atomic Physics · Physics 2012-12-04 M. A. Chieda , E. E. Eyler

We demonstrate launching of laser-cooled Yb atoms in a continuous atomic beam. The continuous cold beam has significant advantages over the more-common pulsed fountain, which was also demonstrated by us recently. The cold beam is formed in…

Atomic Physics · Physics 2013-06-19 K. D. Rathod , Alok K. Singh , Vasant Natarajan

A continuously operated electrostatic trap for polar molecules is demonstrated. The trap has a volume of ~0.6 cm^3 and holds molecules with a positive Stark shift. With deuterated ammonia from a quadrupole velocity filter, a trap density of…

Chemical Physics · Physics 2007-05-23 T. Rieger , T. Junglen , S. A. Rangwala , P. W. H. Pinkse , G. Rempe

We study the properties of a cryogenic buffer gas source that uses a low temperature two-stage buffer gas cell to produce very slow beams of ytterbium monofluoride molecules. The molecules are produced by laser ablation inside the cell and…

Atomic Physics · Physics 2024-11-19 A. D. White , S. Popa , J. Mellado-Munoz , N. J. Fitch , B. E. Sauer , J. Lim , M. R. Tarbutt

We use two-dimensional transverse laser cooling to produce an ultracold beam of YbF molecules. Through experiments and numerical simulations, we study how the cooling is influenced by the polarization configuration, laser intensity, laser…

We report on the production, deceleration and detection of a SrF molecular beam. The molecules are captured from a supersonic expansion and are decelerated in the X$^2\Sigma^+ (v=0, N=1)$ state. We demonstrate the removal of up to 40% of…