Related papers: Broadband high-resolution two-photon spectroscopy …
Biphoton frequency combs are promising resources for quantum networking due in large part to their compatibility with the telecommunication infrastructure. In this work, we propose a method to periodically compress broadband…
The detection of light of thermal origin is the principal means by which humanity has learned about our world and the cosmos. In optical astronomy, in particular, direct detection of thermal photons and the resolution of their spectra have…
The spectral resolution of broadband Fourier-transform coherent anti-Stokes Raman spectroscopy is limited by the maximum optical path length difference that can be scanned within a short time in an interferometer. However, alternatives to…
Femtosecond interferometry combined with acousto-optical phase modulation is an effective approach to implement various types of coherent nonlinear and multidimensional spectroscopy schemes. The high sensitivity of this method has recently…
The concept of mode locking in laser is applied to a two-photon state with frequency entanglement. Cavity enhanced parametric down-conversion is found to produce exactly such a state. The mode-locked two-photon state exhibits a comb-like…
Focusing on the transient regime, we explore atomic two-photon spectroscopy with self-aligned homodyne interferometry in a $\Lambda$-system with large optical depth. The two light sources at the origin of the interference are the…
The interferometric signals produced in conventional dual-comb laser ranging require femtosecond lasers with long-term f_CEO stability, and are limited to an upper sampling rate by radio-frequency aliasing considerations. By using…
Dual-comb spectroscopy enables broadband, high-resolution measurements with microsecond temporal resolution, but extending this capability to the 10~12.5 $\mu$m molecular fingerprint region remains technically challenging, particularly for…
We present gapless, high-resolution absorption and dispersion spectra obtained with quantum cascade laser frequency combs covering 55 cm$^{-1}$. Using phase-sensitive dual comb design, the comb lines are gradually swept over 10 GHz,…
Dual-comb spectroscopy is a rapidly developing technique enabling ultraprecise broadband optical diagnostics of atoms and molecules. This powerful tool typically requires two phase-locked femtosecond lasers, yet it has been shown that it…
A theoretical analysis is carried out for the recently developed three-pulse photon echo spectroscopy employing dual frequency combs (DFC) as the light sources. In this method, the molecular sample interacts with three pulse trains derived…
We propose and demonstrate a method for measuring the joint spectrum of photon pairs via Fourier spectroscopy. The biphoton spectral intensity is computed from a two-dimensional interferogram of coincidence counts. The method has been…
Coherent Raman microscopy provide label-free imaging by interrogating the intrinsic vibration of biomolecules. Nevertheless, trade-off between high chemical-specificity and high imaging-speed currently exists in transition from spectroscopy…
We experimentally demonstrate a versatile technique for performing dual-comb interferometry using a single frequency comb. By rapid switching of the repetition rate, the output pulse train can be delayed and heterodyned with itself to…
Providing an accurate, representative sample of mass flux across large open areas for atmospheric studies or the extreme conditions of a hypersonic engine is challenging for traditional intrusive or point-based sensors. Here, we demonstrate…
We demonstrate simple optical frequency combs based on semiconductor quantum well laser diodes. The frequency comb spectrum can be tailored by choice of material properties and quantum-well widths, providing spectral flexibility. Finally,…
In virtual-state spectroscopy, information about the energy-level structure of an arbitrary sample is retrieved by Fourier transforming sets of measured two-photon absorption probabilities of entangled photon pairs where the degree of…
We report a demonstration of laser Doppler holography at a sustained acquisition rate of 250 Hz on a 1 Megapixel complementary metal-oxide-semiconductor (CMOS) sensor array and image display at 10 Hz frame rate. The holograms are optically…
To meet the challenges of high-resolution molecular spectroscopy, increasingly sophisticated spectroscopic techniques were developed. For a long time FTIR and laser-based spectroscopies were used for these studies. The recent development of…
Recent advances in techniques for generating quantum light have stimulated research on novel spectroscopic measurements using quantum entangled photons. One such spectroscopy technique utilizes non-classical correlations among entangled…