Related papers: Broadband high-resolution two-photon spectroscopy …
We report a broadband long-wave infrared Fourier transform spectrometer with sensitivity exceeding that of previously reported direct-detection implementations. The system combines dual-comb spectroscopy with electro-optic sampling,…
Two-photon resonance transition technology has been proven to have a wide range of applications,it's limited by the available wavelength of commercial lasers.The application of optical comb technology with direct two-photon transition…
Dual-comb spectroscopy has emerged as an indispensable analytical technique in applications that require high resolution and broadband coverage within short acquisition times. Its experimental realization, however, remains hampered by…
High resolution and fast detection of molecular vibrational absorption is important for organic synthesis, pharmaceutical process and environmental monitoring, and is enabled by mid-infrared (mid-IR) laser frequency combs via dual-comb…
We present two-color modulation transfer spectroscopy as a tool for precision studies of atomic properties of excited states. The bi-colored technique addresses a narrow set of velocity groups of a thermal atomic vapour using a two-step…
We have used two-photon Fourier transform spectroscopy to investigate the first singlet excited state (S1) of a prototypical polyene molecule 1,5 -- Diphenyl-1,3,5-hexatriene. As the S1 state in the polyenes is a one-photon forbidden…
Frequency comb spectroscopy provides broadband access to molecular fingerprints with mode-defined spectral resolution. However, its deployment in non-cooperative gas sensing remains challenging because conventional implementations require…
Two-photon absorption is theoretically analyzed within the semiclassical formalism of radiation-matter interaction. We consider an ensemble of inhomogeneously broadened three-level atoms subjected to the action of two counterpropagating…
Optical frequency combs have had a remarkable impact on precision spectroscopy. Enabling this technology in the x-ray domain is expected to result in wide-ranging applications, such as stringent tests of astrophysical models and quantum…
We describe a proof-of-principal experiment demonstrating a Fourier technique for measuring the shape of biphoton wavepackets. The technique is based on the use of synchronously driven fast modulators and slow (integrating) detectors.
A modified Hong--Ou--Mandel (HOM) interference reveals that the two-photon interference phenomenon can be explained only by the concept of a two-photon wave packet rather than a single-photon one. However, the temporal interferogram in the…
Femtosecond dual-comb lasers have revolutionized linear Fourier-domain spectroscopy by offering a rapid motion-free, precise and accurate measurement mode with easy registration of the combs beat note in the RF domain. Extensions of this…
The major development recently undergone by quantum cascade lasers has effectively extended frequency comb emission to longer-wavelength spectral regions, i.e. the mid and far infrared. Unlike classical pulsed frequency combs, their…
In this paper, we introduce an all-fibered dual-comb spectrometer based on a new design of highly nonlinear fiber to efficiently convert frequency combs from 1.55 micron to 2 micron We show that our spectrometer can be used to measure…
Photodetector nonlinearity, the main limiting factor in terms of optical power in the detection chain, is corrected to improve the signal-to-noise ratio of a short-time measurement in dual-comb spectroscopy. An iterative correction…
We apply our recently developed theory of frequency-filtered and time-resolved N-photon correlations to study the two-photon spectra of a variety of systems of increasing complexity: single mode emitters with two limiting statistics (one…
We report experimental results of parallel measurement of spectral components of the light. The temporal fluctuations of an optical field mixed with a separate reference are recorded with a high throughput complementary metal oxide…
Dual Comb Spectroscopy proved its versatile capabilities in molecular fingerprinting in different spectral regions, but not yet in the ultraviolet (UV). Unlocking this spectral window would expand fingerprinting to the electronic energy…
This is the first in a series of two papers investigating the effect of electron-phonon coupling in two-dimensional Fourier transformed electronic spectroscopy. We present a series of one- and two-dimensional nonlinear spectroscopic…
We describe methods using frequency combs and optical resonators for recording two-dimensional (2D) ultrafast spectroscopy signals with high sensitivity. By coupling multiple frequency combs to higher-order modes of one or more optical…