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We describe an approach to optically trapping small, chemically stable molecules at cryogenic temperatures by buffer-gas loading a deep optical dipole trap. The ~10 K trap depth will be produced by a tightly-focused, 1064-nm cavity capable…

The interaction of CO with the Fe3O4(001)-(rt2xrt2)R45{\deg} surface was studied using temperature programmed desorption (TPD), scanning tunneling microscopy (STM) and x-ray photoelectron spectroscopy (XPS), the latter both under ultrahigh…

Nitrogen-doped carbon nanotubes can provide reactive sites on the porphyrin-like defects. It's well known that many porphyrins have transition metal atoms, and we have explored transition metal atoms bonded to those porphyrin-like defects…

Materials Science · Physics 2015-05-27 J. M. de Almeida , A. R. Rocha , A. J. R. da Silva , A. Fazzio

We report on results of a theoretical study of the adsorption process of a single carbon oxide molecule on a Platinum (111) surface. A four-component relativistic density functional method was applied to account for a proper description of…

Atomic and Molecular Clusters · Physics 2009-11-07 D. Geschke , T. Bastug , T. Jacob , S. Fritzsche , W. -D. Sepp , B. Fricke

Direct laser cooling of molecules has reached a phase space density exceeding 10$^{-6}$ in optical traps, but with rather small molecular numbers. To progress towards quantum degeneracy, a mechanism is needed that combines sub-Doppler…

Atomic Physics · Physics 2023-05-24 Justin J. Burau , Parul Aggarwal , Kameron Mehling , Jun Ye

Burning fossil fuels emits a significant amount of CO2, causing climate change concerns. CO2 Capture and Storage (CCS) aims to reduce emissions, with fullerenes showing promise as CO2 adsorbents. Recent research focuses on modifying…

We demonstrate significantly improved magneto-optical trapping of molecules using a very slow cryogenic beam source and RF modulated and DC magnetic fields. The RF MOT confines $1.1(3) \times 10^5$ CaF molecules at a density of $4(1) \times…

Single-photon cooling is a recently introduced method to cool atoms and molecules for which standard methods might not be applicable. We numerically examine this method in a two-dimensional wedge trap as well as in a two-dimensional…

Quantum Physics · Physics 2014-03-25 V. P. Singh , A. Ruschhaupt

We have investigated the impact of toxic N2O gas upon structural and electronic properties of 2D MoSe2 monolayer using DFT approach. In this work, as a result of N2O gas absorption, charge transfer, band gap and density of states (DOS) are…

Materials Science · Physics 2020-08-18 N. Mishra , Bramha P. Pandey

Diffusion Monte Carlo calculations on the adsorption of $^4$He in open-ended single walled (10,10) nanotubes are presented. We have found a first order phase transition separating a low density liquid phase in which all $^4$He atoms are…

Materials Science · Physics 2009-11-13 M. C. Gordillo , J. Boronat , J. Casulleras

In this work, we investigate the physical and electronic properties of $\beta_{12}$-borophene FET-based gas sensor using a theoretical quantum capacitance model based on tight-binding approach. We study the impact of adsorbed NH$_3$, NO,…

Superconductivity · Physics 2023-04-03 Nimisha Dutta , Reeta Devi , Arindam Boruah , Saumen Acharjee

Absorption of ultraviolet radiation by water ice coating interstellar grains can lead to dissociation and desorption of the ice molecules. These processes are thought to be important in the gas-grain chemistry in molecular clouds and…

Astrophysics · Physics 2009-11-13 S. Andersson , E. F. van Dishoeck

The first electrical conductivity measurements of monoatomic carbon chains are reported in this study. The chains were obtained by unraveling carbon atoms from graphene ribbons while an electrical current flowed through the ribbon and,…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 O. Cretu , A. R. Botello-Mendez , I. Janowska , C. Pham-Huu , J. -C. Charlier , F. Banhart

Centaurus A, the nearest AGN shows molecular absorption in the millimeter and radio regime. By observing the absorption with VLBI, we try to constrain the distribution of the gas, in particular whether it resides in the circumnuclear…

Astrophysics · Physics 2009-11-10 H. J. van Langevelde , Y. Pihlstroem , A. Beasley

Understanding how the local environment of a single-atom catalyst affects stability and reactivity remains a significant challenge. We present an in-depth study of Cu1, Ag1, Au1, Ni1, Pd1, Pt1, Rh1, and Ir1 species on Fe3O4(001); a model…

Cyclocarbon molecules are critical in understanding the carbon structure formation and the nature of the interaction between carbon atoms. In cyclocarbons, light elements such as H, O and N may interplay with rings to form doped cyclocarbon…

Mesoscale and Nanoscale Physics · Physics 2023-10-31 Liujia Min , Aigen Li , Xianghong Chen , Yonghui Li

It is demonstrated that the use of a Micrometric Thin $^{39}$K vapor Cell (MTC) and Saturated Absorption spectroscopy (SA) allows to form narrow atomic lines in transmission spectrum without unwanted Cross-Over (CO) resonances. Another…

Atomic Physics · Physics 2022-09-28 Armen Sargsyan , Rodolphe Momier , Claude Leroy , David Sarkisyan

The study of electron transport through single molecules is essential to the development of molecular electronics. Indeed, trends in electronic conductance through organic nanowires have emerged with the increasing reliability of electron…

Mesoscale and Nanoscale Physics · Physics 2007-05-24 Jordan R. Quinn , Frank W. Foss , Latha Venkataraman , Mark S. Hybertsen , Ronald Breslow

Laser cooling and trapping are central to modern atomic physics. The workhorse technique in cold-atom physics is the magneto-optical trap (MOT), which combines laser cooling with a restoring force from radiation pressure. For a variety of…

Atomic Physics · Physics 2014-10-20 J. F. Barry , D. J. McCarron , E. B. Norrgard , M. H. Steinecker , D. DeMille

Both the translational diffusion coefficient $D$ and the electrophoretic mobility $\mu$ of a short rod-like molecule (such as dsDNA) that is being pulled towards a nanopore by an electric field should depend on its orientation. Since a…

Biological Physics · Physics 2020-06-25 Le Qiao , Gary W. Slater