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One of the main characteristics of the new family of two-dimensional crystals of semiconducting transition metal dichalcogenides (TMD) is the strong spin-orbit interaction, which makes them very promising for future applications in…

Mesoscale and Nanoscale Physics · Physics 2015-11-11 R. Roldán , M. P. López-Sancho , E. Cappelluti , J. A. Silva-Guillén , P. Ordejón , F. Guinea

The spin-valley or Kramers qubit promises significantly enhanced spin-valley lifetimes due to strong coupling of the electrons' spin to their momentum (valley) degrees of freedom. In transition metal dichalcogenides (TMDCs) such spin-valley…

Mesoscale and Nanoscale Physics · Physics 2024-10-30 Aakash Shandilya , Sundeep Kapila , Radha Krishnan , Bent Weber , Bhaskaran Muralidharan

Spin-orbit coupling (SOC) is a relativistic effect, where an electron moving in an electric field experiences an effective magnetic field in its rest frame. In crystals without inversion symmetry, it lifts the spin degeneracy and leads to…

Effective spin-orbit (SO) Hamiltonians for conduction electrons in wurtzite heterostructures are lacking in the literature, in contrast to zincblende structures. Here we address this issue by deriving such an effective Hamiltonian valid for…

Mesoscale and Nanoscale Physics · Physics 2020-04-22 J. Y. Fu , P. H. Penteado , D. R. Candido , G. J. Ferreira , D. P. Pires , E. Bernardes , J. C. Egues

Strong spin-orbit coupling in transition metal dichalcogenide (TMDC) monolayers results in spin resolvable band structures about the $K$ and $K'$ valleys such that the eigenbasis of a 2D quantum dot (QD) in a TMDC monolayer in zero field is…

Mesoscale and Nanoscale Physics · Physics 2018-04-25 Matthew Brooks , Guido Burkard

Semiconducting transition metal dichalcogenides (TMDCs) are very promising materials for quantum dots and spin-qubit implementation. Reliable operation of spin qubits requires the knowledge of Land\'e g-factor, which can be measured by…

Mesoscale and Nanoscale Physics · Physics 2023-03-28 P. Kumar , H. Kim , S. Tripathy , K. Watanabe , T. Taniguchi , K. S. Novoselov , D. Kotekar-Patil

Spin qubits composed of either one or three electrons are realized in a quantum dot formed at a Si/SiO_2-interface in isotopically enriched silicon. Using pulsed electron spin resonance, we perform coherent control of both types of qubits,…

Mesoscale and Nanoscale Physics · Physics 2015-11-11 M. Veldhorst , R. Ruskov , C. H. Yang , J. C. C. Hwang , F. E. Hudson , M. E. Flatté , C. Tahan , K. M. Itoh , A. Morello , A. S. Dzurak

The negligible intrinsic spin-orbit coupling (SOC) in graphene can be enhanced by proximity effects in stacked heterostructures of graphene and transition metal dichalcogenides (TMDCs). The composition of the TMDC layer plays a key role in…

Mesoscale and Nanoscale Physics · Physics 2022-09-20 Zahra Khatibi , Stephen R. Power

Transition metal dichalcogenide (TMDC) monolayers are newly discovered semiconductors for a wide range of applications in electronics and optoelectronics. Most studies have focused on binary monolayers that share common properties: direct…

We study the conduction band spin splitting that arises in transition metal dichalcogenide (TMD) semiconductor monolayers such as MoS$_2$, MoSe$_2$, WS$_2$ and WSe$_2$ due to the combination of spin-orbit coupling and lack of inversion…

Materials Science · Physics 2014-01-01 K. Kośmider , J. W. González , J. Fernández-Rossier

Spins confined to atomically-thin semiconductors are being actively explored as quantum information carriers. In transition metal dichalcogenides (TMDCs), the hexagonal crystal lattice gives rise to an additional valley degree of freedom…

Mesoscale and Nanoscale Physics · Physics 2023-06-29 Radha Krishnan , Sangram Biswas , Yu-Ling Hsueh , Hongyang Ma , Rajib Rahman , Bent Weber

The metallic transition-metal dichalcogenides (TMDCs) are benchmark systems for studying and controlling intertwined electronic orders in solids, with superconductivity developing upon cooling from a charge density wave state. The interplay…

Silicon quantum dots are considered an excellent platform for spin qubits, partly due to their weak spin-orbit interaction. However, the sharp interfaces in the heterostructures induce a small but significant spin-orbit interaction which…

In monolayer Transition Metal Dichalcogenides (TMDs) the valence and conduction bands are spin split because of the strong spin-orbit interaction. In tungsten-based TMDs the spin-ordering of the conduction band is such that the so-called…

Strong electron correlation and spin-orbit coupling (SOC) provide two non-trivial threads to condensed matter physics. When these two strands of physics come together, a plethora of quantum phenomena with novel topological order have been…

Mesoscale and Nanoscale Physics · Physics 2024-02-26 Jiang-Xiazi Lin , Ya-Hui Zhang , Erin Morissette , Zhi Wang , Song Liu , Daniel Rhodes , K. Watanabe , T. Taniguchi , James Hone , J. I. A. Li

We develop a microscopic and atomistic theory of electron spin-based qubits in gated quantum dots in a single layer of transition metal dichalcogenides. The qubits are identified with two degenerate locked spin and valley states in a gated…

Mesoscale and Nanoscale Physics · Physics 2021-11-24 Abdulmenaf Altıntaş , Maciej Bieniek , Amintor Dusko , Marek Korkusiński , Jarosław Pawłowski , Paweł Hawrylak

While bulk silicon has long been understood to exhibit relatively weak spin-orbit coupling (SOC), confinement of electrons to quantum dots (QDs) at a silicon heterointerface results in significantly larger SOC. This is a concern for…

Tunable synthetic spin-orbit coupling (s-SOC) is one of the key challenges in various quantum systems, such as ultracold atomic gases, topological superconductors, and semiconductor quantum dots. Here we experimentally demonstrate…

Spin-orbit coupling (SOC) lifts molecular orbital degeneracy, enabling bi-level electronic platforms suitable for next-generation digital devices. However, common light-atom molecular feedstocks exhibit weak SOC due to the absence of heavy…

Materials Science · Physics 2025-05-07 Zihao Wang , Wan-Lu Li , Shaowei Li

In monolayer group-VI transition metal dichalcogenides (TMDC), charge carriers have spin and valley degrees of freedom, both associated with magnetic moments. On the other hand, the layer degree of freedom in multilayers is associated with…

Mesoscale and Nanoscale Physics · Physics 2013-07-19 Zhirui Gong , Gui-Bin Liu , Hongyi Yu , Di Xiao , Xiaodong Cui , Xiaodong Xu , Wang Yao
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