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We calculate the rate of two-photon absorption for frequency entangled photons in a tapered optical fiber whose diameter is comparable to the wavelength of the light. The confinement of the electric field in the transverse direction…

Quantum Physics · Physics 2010-04-12 Hao You , S. M. Hendrickson , J. D. Franson

Entangled two-photon absorption can enable a linear scaling of fluorescence emission with the excitation power. In comparison to classical two-photon absorption with a quadratic scaling, this can allow fluorescence imaging or…

The study of entangled states has greatly improved the basic understanding about two-photon interferometry. Two-photon interference is not the interference of two photons but the result of superposition among indistinguishable two-photon…

Quantum Physics · Physics 2009-11-10 Giuliano Scarcelli , Alejandra Valencia , Yanhua Shih

We closely replicated and extended a recent experiment ("Spatial properties of entangled two-photon absorption," Phys. Rev. Lett. 129, 183601, 2022) that reportedly observed enhancement of two-photon absorption rates in molecular samples by…

Quantum Physics · Physics 2024-04-26 Tiemo Landes , Brian J. Smith , Michael G. Raymer

We numerically analyze the use of intense entangled twin beams for ultra-sensitive spectroscopic measurements in chemical and biological systems. The examined scheme makes use of intense frequency-modulated (chirped) entangled beams to…

Quantum Physics · Physics 2018-05-16 Jiří Svozilík , Jan Peřina , Roberto de J. León-Montiel

Two-photon absorption (TPA) and other nonlinear interactions of molecules with time-frequency-entangled photon pairs (EPP) has been predicted to display a variety of fascinating effects. Therefore, their potential use in practical…

Quantum Physics · Physics 2021-09-15 Michael G. Raymer , Tiemo Landes , Andrew H. Marcus

While two-photon absorption (TPA) and other forms of nonlinear interactions of molecules with isolated time-frequency-entangled photon pairs (EPP) have been predicted to display a variety of fascinating effects, their potential use in…

We propose a novel scheme to achieve two-photon super bunching of thermal light through multiple two-photon-path interference, in which two mutually first-order incoherent optical channels are introduced by inserting a modified Michelson…

Quantum Physics · Physics 2013-05-30 Peilong Hong , Jianbin Liu , Guoquan Zhang

Over the last 50 years entangled photon pairs have received attention for use in lowering the flux in two-photon absorption imaging and spectroscopy. Despite this, evidence for entangled two-photon absorption (ETPA) effects remain highly…

Two-photon interference and "ghost" imaging with entangled light have attracted much attention since the last century because of the novel features such as non-locality and sub-wavelength effect. Recently, it has been found that…

Quantum Physics · Physics 2009-11-11 Yan-Hua Zhai , Xi-Hao Chen , Da Zhang , Ling-An Wu

The phenomena of subthreshold photoemission and absorption under coherent and entangled-photon-pair illumination are reviewed, and the generation and properties of entangled-photon pairs are surveyed. Three prominent forms of subthreshold…

Quantum Physics · Physics 2026-05-05 Malvin Carl Teich , Mark C. Booth , Francesco Lissandrin , Bahaa E. A. Saleh

Entangled two-photon absorption spectroscopy (TPA) has been widely recognized as a powerful tool for revealing relevant information about the structure of complex molecular systems. However, to date, the experimental implementation of this…

Quantum Physics · Physics 2019-07-10 Roberto de J. León-Montiel , Jiří Svozilík , Juan P. Torres , Alfred B. U'Ren

When a low flux of time-frequency-entangled photon pairs (EPP) illuminates a two-photon transition, the rate of two-photon absorption (TPA) can be enhanced considerably by the quantum nature of photon number correlations and frequency…

We report how the unique temporal and spectral features of pulsed entangled photons from a parametric downconversion source can be utilized for manipulating electronic excitations through the optimization of their spectral phase. A new…

Chemical Physics · Physics 2024-09-18 Sajal Kumar Giri , George C. Schatz

Excitation with entangled photon pairs may lead to an increase in the efficiency of two-photon absorption at low photon flux. The corresponding process, entangled two-photon absorption (E2PA), has been investigated in numerous theoretical…

We report the first experimental demonstration of two-photon imaging with a pseudo-thermal source. Similarly to the case of entangled states, a two-photon Gaussian thin lens equation is observed, indicating EPR type correlation in position.…

Quantum Physics · Physics 2009-11-10 Alejandra Valencia , Giuliano Scarcelli , Milena D'Angelo , Y. Shih

Two-photon absorption (TPA) fluorescence of biomarkers has been decisive in advancing the fields of biosensing and deep-tissue in vivo imaging of live specimens. However, due to the extremely small TPA cross section and the quadratic…

Optics · Physics 2020-06-25 Tian Li , Fu Li , Charles Altuzarra , Anton Classen , Girish S. Agarwal

We analyze the rate of two-photon absorption in tapered optical fibers with diameters less than the wavelength of the incident light. The rate of two-photon absorption is shown to be enhanced due to the small mode volume of the tapered…

Quantum Physics · Physics 2009-11-13 Hao You , S. M. Hendrickson , J. D. Franson

We present a theoretical analysis of two-photon absorption of classical and squeezed light valid when one-photon absorption to an intermediate state is either resonant or far-detuned from resonance, and in both the low and high intensity…

Quantum Physics · Physics 2022-09-14 Christian Drago , John Sipe

It has been proposed that entangled two-photon absorption (E2PA) can be observed with up to 10 orders of magnitude lower photon flux than its classical counterpart. However, there is a significant controversy regarding the magnitude of this…

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