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We experimentally study entangled two-photon absorption in Rhodamine 6G as a function of the spatial properties of a high flux of broadband entangled photon pairs. We first demonstrate a key signature dependence of the entangled two-photon…

Quantum Physics · Physics 2022-06-10 D. Tabakaev , A. Djorovic , L. La Volpe , G. Gaulier , S. Ghosh , L. Bonacina , J. -P. Wolf , H. Zbinden , R. T. Thew

In virtual-state spectroscopy, information about the energy-level structure of an arbitrary sample is retrieved by Fourier transforming sets of measured two-photon absorption probabilities of entangled photon pairs where the degree of…

Quantum Physics · Physics 2021-08-04 Lutz Mertenskötter , Kurt Busch , Roberto de J. León-Montiel

The aim of this review paper is to enlighten some recent progresses in quantum optical metrology in the part of quantum efficiency measurements of photo-detectors performed with bi-photon states. The intrinsic correlated nature of entangled…

Quantum Physics · Physics 2015-06-26 G. Brida , M. Genovese , M. Gramegna

Nonlinear spectroscopic techniques using entangled photon pairs can provide an opportunity to exploit non-classical correlations encoded in two-photon wavefunctions to manipulate two-exciton wavefunctions. We propose an entangled photon…

Quantum Physics · Physics 2026-04-10 Arunangshu Debnath , Shaul Mukamel

Entangling independent photons is not only of fundamental interest but also of crucial importance for quantum information science. Two-photon interference is a major method to entangle independent identical photons. If two photons are…

Quantum Physics · Physics 2015-01-27 Tian-Ming Zhao , Han Zhang , Jian Yang , Zi-Ru Sang , Xiao Jiang , Xiao-Hui Bao , Jian-Wei Pan

Fluorescence excitation by absorption of entangled photon pairs offers benefits compared to classical imaging techniques, such as the attainment of higher signal levels at low excitation power while simultaneously mitigating photo-toxicity.…

Quantum Physics · Physics 2023-11-02 Tobias Bernd Gäbler , Patrick Hendra , Nitish Jain , Markus Gräfe

Ultrafast optical spectroscopy is a powerful technique for studying the dynamic processes of molecular systems in condensed phases. However, in molecular systems containing many dye molecules, the spectra can become crowded and difficult to…

Chemical Physics · Physics 2025-02-05 Yuta Fujihashi , Akihito Ishizaki , Ryosuke Shimizu

Most experimental demonstrations of entanglement require nonclassical states and correlated measurements of single-photon detection events. It is shown here that entanglement can produce a large decrease in the rate of two-photon absorption…

Quantum Physics · Physics 2009-11-11 J. D. Franson

Two-photon superbunching of pseudothermal light is observed with single-mode continuous-wave laser light in a linear optical system. By adding more two-photon paths via three rotating ground glasses,g(2)(0) = 7.10 is experimentally…

Optics · Physics 2017-10-11 Bin Bai , Jianbin Liu , Yu Zhou , Huaibin Zheng , Hui Chen , Songlin Zhang , Yuchen He , Fuli Li , Zhuo Xu

For dissipation-free photon-photon interaction at the single photon level, we analyze one-photon transition and two-photon transition induced by photon pairs in three-level atoms using two-photon wavefunctions. We show that the two-photon…

Quantum Physics · Physics 2011-06-16 Toshihiro Nakanishi , Hirokazu Kobayashi , Kazuhiko Sugiyama , Masao Kitano

We examine the possibility of storing and retrieving a single photon using electromagnetically induced transparency (EIT). We consider the theory of a proof of principle two-photon interference experiment, in which an atomic vapor cell is…

Quantum Physics · Physics 2007-05-23 Jianming Wen , Morton H. Rubin

We report on the dynamics of photodegradation and subsequent recovery of two-photon fluorescence in a dye-doped polymer. The energy dependence suggests that photo-degradation is a linear process while recovery is entropic. Such recovery…

Optics · Physics 2009-11-13 Ye Zhu , Juefei Zhou , Mark G. Kuzyk

We experimentally demonstrate shaping of the two-photon wavefunction of entangled photon-pairs, utilizing coherent pulse-shaping techniques. By performing spectral-phase manipulations we tailor the two-photon wavefunction exactly like a…

Quantum Physics · Physics 2011-12-06 Avi pe'er , Barak Dayan , Asher A. Friesem , Yaron Silberberg

Tho-photon absorption holds potential for many practical applications. We theoretically investigate the onset of this phenomenon in a semiconductor quantum dot -- metallic nanoshell composite subjected to a resonant CW excitation.…

Mesoscale and Nanoscale Physics · Physics 2021-01-08 Bintoro S. Nugroho , Alexander A. Iskandar , Victor A. Malyshev , Jasper Knoester

Two-photon absorption is theoretically analyzed within the semiclassical formalism of radiation-matter interaction. We consider an ensemble of inhomogeneously broadened three-level atoms subjected to the action of two counterpropagating…

Quantum Physics · Physics 2007-05-23 I. Perez-Arjona , G. J. de Valcarcel , Eugenio Roldan

The phenomenon of Entangled Two-Photon Absorption (ETPA) presents a persistent controversy in the literature, evidenced by a wide disparity in the reported values for the $\sigma_E$ cross-sections. Much of this discrepancy is attributed to…

Quantum Physics · Physics 2025-12-02 Pablo Yepiz-Graciano , Gabriel Ramos-Ortiz , Roberto Ramírez-Alarcón

Two-photon (2P) microscopy is a powerful technique for deep-tissue fluorescence imaging; however, tissue scattering limits its effectiveness for depth imaging using conventional approaches. Despite typical strategies having been put forward…

Optics · Physics 2025-05-21 Lei Zhu , Bernhard Rauer , Hilton B. De Aguiar , Sylvain Gigan

We introduce a method for determining the sensitivity of any given Entangled Two-Photon Absorption (ETPA) measurement. By modeling all signal and noise contributions to the measurement, we derive a single numerical value that describes the…

Quantum Physics · Physics 2025-12-23 René Pollmann , Franz Roeder , Christine Silberhorn , Benjamin Brecht

Entangled two-photon absorption (eTPA) has been recognized as a potentially powerful tool for the implementation of ultra-sensitive spectroscopy. Unfortunately, there exists a general agreement in the quantum optics community that…

Quantum Physics · Physics 2025-01-31 Áulide Martínez-Tapia , Roberto de J. León-Montiel

We experimentally demonstrate amplitude and phase modulation of a time-energy entangled two-photon wave function. The entangled photons are produced by spontaneous parametric down-conversion, spectrally dispersed in an prism compressor,…

Quantum Physics · Physics 2009-01-23 F. Zäh , M. Halder , T. Feurer