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We analyze, through resonant photoluminescence, the spin dynamics of an individual magnetic atom (Mn) coupled to a hole in a semiconductor quantum dot. The hybrid Mn-hole spin and the positively charged exciton in a CdTe/ZnTe quantum dot…

Mesoscale and Nanoscale Physics · Physics 2017-06-21 A. Lafuente-Sampietro , H. Boukari , L. Besombes

Mn2+-doped semiconductor nanocrystals with tuned location and concentration of Mn2+ ions can yield diverse coupling regimes, which can highly influence their optical properties such as emission wavelength and photoluminescence (PL)…

Asymmetrical horizontal interdot coupling was demonstrated to exist in a system of a single plane of self-assembled CdTe/ZnTe quantum dots. Photoluminescence excitation (PLE), second order photon correlation and optical orientation were…

Other Condensed Matter · Physics 2009-06-12 T. Kazimierczuk , J. Suffczynski , P. Wojnar , A. Golnik , J. A. Gaj , P. Kossacki

Systematic measurements of auto- and cross-correlations of photons emitted from individual CdTe/ZnTe quantum dots under pulsed excitation were used to elucidate non-resonant excitation mechanisms in this self-assembled system. Memory…

Incorporation of manganese impurities into II-VI semiconductors results in a dramatic change in their properties due to strong exchange interactions between the Mn ion and the semiconductor host. In colloidal quantum dots (QDs), these…

Materials Science · Physics 2024-12-24 Jungchul Noh , Clément Livache , Donghyo Hahm , Valerio Pinchetti , Ho Jin , Changjo Kim , Victor I. Klimov

We report on the micro-photoluminescence spectroscopy of InAs/GaAs quantum dots (QD) doped by a single Mn atom in a magnetic field either longitudinal or perpendicular to the optical axis. In both cases the spectral features of positive…

Materials Science · Physics 2015-05-14 Olivier Krebs , Emile Benjamin , Aristide Lemaître

We show that two major carrier excitation mechanisms are present in II-VI self-assembled quantum dots. The first one is related to direct excited state - ground state transition. It manifests itself by the presence of sharp and intense…

Doping a self-assembled InGaAs/GaAs quantum dot (QD) with a single Mn atom, a magnetic acceptor impurity, provides a quantum system with discrete energy levels and original spin-dependent optical selection rules, which thus has large…

Mesoscale and Nanoscale Physics · Physics 2024-10-28 Jovana Filipovic , Ankit Kundu , Neelesh Kumar Vij , Simon Fécherolle , Aristide Lemaître , Shilpi Gupta , Olivier Krebs

Mechanisms of nonradiative recombination of electron-hole complexes in Cd(Mn)Se/Zn(Mn)Se quantum dots accompanied by interconfigurational excitations of Mn$^{2+}$ ions are analyzed within the framework of single electron model of deep {\it…

Mesoscale and Nanoscale Physics · Physics 2010-08-25 A. V. Chernenko , A. S. Brichkin , N. A. Sobolev , M. C. Carmo

We have observed strong photoluminescence from a single CdSe quantum dot embedded in a ZnSe nanowire. Exciton, biexciton and charged exciton lines have been identified unambiguously using photon correlation spectroscopy. This technique has…

We present photoluminescence studies of CdTe and CdMnTe quantum dots grown in two adjacent layers. We show that when the dots are 8 nm apart, their magnetooptical properties - Zeeman shifts and transition linewidths - are analogous to those…

Mesoscale and Nanoscale Physics · Physics 2015-08-12 Ł. Kłopotowski , P. Wojnar , Ł. Cywiński , T. Jakubczyk , M. Goryca , K. Fronc , T. Wojtowicz , G. Karczewski

We demonstrate that resonant excitation of CdMnTe self-assembled quantum dots creates an ensemble of spin-polarized magnetic polarons at B=0 T. The strong spatial confinement characteristic of quantum dots significantly increases the…

Soft Condensed Matter · Physics 2009-11-10 S. Mackowski , T. Gurung , T. A. Nguyen , H. E. Jackson , L. M. Smith , G. Karczewski , J. Kossut

We study the formation dynamics of a spontaneous ferromagnetic order in single self-assembled CdMnTe quantum dots. By measuring time-resolved photoluminescence, we determine the formation times for QDs with Mn ion contents x varying from…

We report on photon coincidence measurement in a single GaAs self-assembled quantum dot (QD) using a pulsed excitation light source. At low excitation, when a neutral exciton line was present in the photoluminescence (PL) spectrum, we…

We investigated optical spin orientation and dynamic nuclear polarization (DNP) in individual self-assembled InGaAs/GaAs quantum dots (QDs) doped by a single Mn atom, a magnetic impurity providing a neutral acceptor A$^0$ with an effective…

Mesoscale and Nanoscale Physics · Physics 2016-11-15 O. Krebs , E. Baudin , A. Lemaître

A photo-excited II-VI semiconductor nanocrystal doped with a few Mn spins is considered. The effects of spin-exciton interactions and the resulting multi-spin correlations on the photoluminescence are calculated by numerical diagonalization…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 J. Fernández-Rossier

A quantum dot strongly coupled to a photonic crystal has been recently proposed as a source of entangled photon pairs [R. Johne et al., Phys. Rev. Lett. 100, 240404 (2008)]. The biexction decay via intermediate polariton states can be used…

Quantum Physics · Physics 2015-05-13 Robert Johne , Nikolay A. Gippius , Guillaume Malpuech

We present a comprehensive experimental and theoretical studies of photoluminescence of single CdMnTe quantum dots with Mn content x ranging from 0.01 to 0.2. We distinguish three stages of the equilibration of the exciton-Mn ion spin…

Mesoscale and Nanoscale Physics · Physics 2013-07-23 Ł. Kłopotowski , Ł. Cywiński , M. Szymura , V. Voliotis , R. Grousson , P. Wojnar , K. Fronc , T. Kazimierczuk , A. Golnik , G. Karczewski , T. Wojtowicz

The spin dynamics of a single Mn atom in a laser driven CdTe quantum dot is addressed theoretically. Recent experimental results\cite{Le-Gall_PRL_2009,Goryca_PRL_2009,Le-Gall_PRB_2010}show that it is possible to induce Mn spin polarization…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 C. L. Cao , L. Besombes , J. Fernández-Rossier

Two electrons in a quantum dot (QD) can form triplet states. We analyze the exchange coupling of the triplet states of the negatively charged exciton in a QD (X$^-$, two electrons and one hole) with the spin of a magnetic atom (Mn). Two…

Mesoscale and Nanoscale Physics · Physics 2023-07-12 L. Besombes , S. Ando , S. Kuroda , H. Boukari