We study the formation dynamics of a spontaneous ferromagnetic order in single self-assembled CdMnTe quantum dots. By measuring time-resolved photoluminescence, we determine the formation times for QDs with Mn ion contents x varying from 0.01 to 0.2. At low x these times are orders of magnitude longer than exciton spin relaxation times evaluated from the decay of photoluminescence circular polarization. This allows us to conclude that the direction of the spontaneous magnetization is determined by a momentary Mn spin fluctuation rather than resulting from an optical orientation. At higher x, the formation times are of the same order of magnitude as found in previous studies on higher dimensional systems. We also find that the exciton spin relaxation accelerates with increasing Mn concentration.
@article{arxiv.1012.1179,
title = {Magnetic polaron formation and exciton spin relaxation in single CdMnTe quantum dots},
author = {Łukasz Kłopotowski and Łukasz Cywiński and Piotr Wojnar and Valia Voliotis and Krzysztof Fronc and Tomasz Kazimierczuk and Andrzej Golnik and Marco Ravarro and Roger Grousson and Grzegorz Karczewski and Tomasz Wojtowicz},
journal= {arXiv preprint arXiv:1012.1179},
year = {2011}
}