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The very low temperature properties of two pyrochlore compounds, Yb2Ti2O7 and Gd2Sn2O7, were investigated using an ensemble of microscopic and bulk techniques. In both compounds, a first order transition is evidenced, as well as spin…

Inelastic neutron scattering experiments were performed on single crystals of the heavy-fermion compound CeIn$_{3}$ for temperatures below and above the N\'eel temperature, $T_N$. In the antiferromagnetically ordered phase, well-defined…

Strongly Correlated Electrons · Physics 2009-11-10 W. Knafo , S. Raymond , B. Fak , G. Lapertot , P. C. Canfield , J. Flouquet

We report on neutron diffraction, thermal expansion, magnetostriction, dielectric, and specific heat measurements on polycrystalline FeCr2S4 in external magnetic fields. The ferrimagnetic ordering temperatures $T_{\mathrm{C}}\approx 170$ K…

The crystallographic and physical properties of polycrystalline and single crystal samples of BaCo2As2 and K-doped Ba{1-x}K{x}Co2As2 (x = 0.06, 0.22) are investigated by x-ray and neutron powder diffraction, magnetic susceptibility chi,…

We study the ground state properties, the electronic excitations and lattice dynamics in spin-liquid candidate TbInO$_3$. By employing polarization resolved Raman spectroscopy we define the inter- and intra-multiplet excitations, and…

Strongly Correlated Electrons · Physics 2021-08-11 Mai Ye , Xianghan Xu , Xiangyue Wang , Jaewook Kim , Sang-Wook Cheong , Girsh Blumberg

We combine two aspects of magnetic frustration, multiferroicity and emergent quasi-particles in spin liquids, by studying magneto-electric monopoles. Spin ice offers to couple these emergent topological defects to external fields, and to…

Strongly Correlated Electrons · Physics 2015-06-24 Ludovic D. C. Jaubert , R. Moessner

We report on the magnetic structures of Tb3RuO7 and Nd3RuO7 determined from powder neutron-diffraction experiments. In Tb3RuO7, alternating-bond spin-3/2 Ru1-Ru2 chains are formed. The Ru1 and Ru2 moments are ordered and disordered…

Strongly Correlated Electrons · Physics 2021-09-30 Masashi Hase , Andreas Dönni , Vladimir Yu. Pomjakushin

Spin correlations of the frustrated pyrochlore oxide Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been investigated by using inelastic neutron scattering on single crystalline samples ($x=-0.007, 0.000,$ and $0.003$), which have the putative…

Strongly Correlated Electrons · Physics 2019-01-08 Hiroaki Kadowaki , Mika Wakita , Björn Fåk , Jacques Ollivier , Seiko Ohira-Kawamura , Kenji Nakajima , Jeffrey W. Lynn

The superconductor Nb$_3$Sn has a high critical temperature and high critical field, widely used for high-field superconducting magnets. In this work we investigate its microscopic electronic structure with $^{93}$Nb nuclear magnetic…

We report inelastic neutron scattering measurements of crystal field transitions in PrFeAsO, PrFeAsO0.87F0.13, and NdFeAsO0.85F0.15. Doping with fluorine produces additional crystal field excitations, providing evidence that there are two…

LuCuGaO4 has magnetic Cu2+ and diamagnetic Ga3+ ions distributed on a triangular bilayer and is suggested to undergo a spin-glass transition with T_g approximately 0.4 K. Using muSR and neutron scattering measurements, we show that at low…

Materials Science · Physics 2013-05-29 S Calder , SR Giblin , DR Parker , PP Deen , C Ritter , JR Stewart , S Rols , T Fennell

We report a positive muon spin relaxation and rotation (\muSR) study of the quantum spin ice materials Yb2Ti2O7 and Yb2Sn2O7 focusing on the low field response. In agreement with earlier reports, data recorded in small longitudinal fields…

Strongly Correlated Electrons · Physics 2015-09-24 A. Maisuradze , P. Dalmas de Reotier , A. Yaouanc , A. Forget , C. Baines , P. J. C. King

The Raman, IR and force field have been investigated for A2Mn2O7 (A= Tl, In) by means of a short-range force constant model which includes four stretching and four bending force constants. Unusual spectral and force field changes are…

Condensed Matter · Physics 2009-11-10 Sonal Brown , H. C. Gupta , J. A. Alonso , M. J. Martinez-Lope

The Gd2Sn2O7 pyrochlore Heisenberg antiferromagnet displays a phase transition to a four sublattice Neel ordered state at a temperature near 1 K. Despite the seemingly conventional nature of the ordered state, the specific heat has been…

Materials Science · Physics 2007-08-16 Adrian Del Maestro , Michel J. P. Gingras

We present neutron inelastic scattering measurements of the low-energy phonons in single crystal BiFeO3. The dispersions of the three acoustic phonon modes (LA along [100], TA1 along [010] and TA2 along [110]) and two low energy optic…

We have measured magnetic torque on a $T_N=7$ K single crystal of $\alpha$-RuCl$_3$, as a function of the field angle in the $ab$-plane, focusing on temperatures between 2 and 20 K and fields from 0 to 9 T. We find a number of features,…

Strongly Correlated Electrons · Physics 2025-01-20 Shaun Froude-Powers , Subin Kim , Jacob Gordon , Hae-Young Kee , Young-June Kim , Stephen R. Julian

We report on the crystal field level splitting and magnetic ground state of the Jeff = 1/2 square lattice antiferromagnets YbBi2ClO4 and YbBi2IO4 using powder inelastic neutron scattering (INS) and neutron diffraction measurements. Both…

Strongly Correlated Electrons · Physics 2025-03-25 Pyeongjae Park , Qianli Ma , G. Sala , S. Calder , Douglas L. Abernathy , Matthew B. Stone , Andrew F. May , Andrew D. Christianson

We have studied the Tb$_2$Sn$_2$O$_7$ frustrated magnet by neutron diffraction under isotropic pressure of 4.6 GPa, combined with uniaxial pressure of 0.3 GPa, in the temperature range 0.06 K$<$T$<$100 K. Magnetic order persists under…

Strongly Correlated Electrons · Physics 2015-05-13 I. Mirebeau , I. Goncharenko , H. Cao , A. Forget

The rare-earth perovskite TbScO$_3$ has been widely used as a substrate for the growth of epitaxial ferroelectric and multiferroic thin films, while its detailed low-temperature magnetic properties were rarely reported. In this paper, we…

We have carried out temperature and pressure-dependent Raman and x-ray measurements on single crystals of Tb$_2$Ti$_2$O$_7$. We attribute the observed anomalous temperature dependence of phonons to phonon-phonon anharmonic interactions. The…

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