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We investigated the magnetic transitions in BiFeO$_3$ at low temperature (5-300 K) and observed nearly 90$^o$ rotation of magnetic domains (imaged by vertical magnetic force microscopy) across 150 K in an epitaxial thin film of thickness…

We employ polarization-resolved Raman spectroscopy to study the lattice dynamics of the polar charge density wave phase of the superconductor Mo$_3$Al$_2$C with structural chirality. We show the phononic signatures of the charge density…

Superconductivity · Physics 2025-06-12 Shangfei Wu , Xianghan Xu , Fei-Ting Huang , Turan Birol , Sang-Wook Cheong , Girsh Blumberg

In this work, we present an analysis of magnetic properties of weak ferrimagnets of the YFe$_{1-x}$Cr$_x$O$_3$ type. Taking into account the main spin interactions - isotropic Heisenberg superexchange, antisymmetric Dzyaloshinskii-Moriya…

Strongly Correlated Electrons · Physics 2024-12-24 E. V. Vasinovich , A. S. Moskvin

Magnetic and crystallographic transitions in the Cairo pentagonal magnet Bi2Fe4O9 are investigated by means of infrared synchrotron-based spectroscopy as a function of temperature (20 - 300 K) and pressure (0 - 15.5 GPa). One of the phonon…

Other Condensed Matter · Physics 2021-05-05 M. Verseils , A. P. Litvinchuk , J-B Brubach , P. Roy , K. Beauvois , E. Ressouche , V. Skumryev , M. Gospodinov , V. Simonet , S. deBrion

The sequence of phase transitions in PbHf0.83Sn0.17O3 has been studied by THz, far infrared and Raman spectroscopies, revealing the complementary behaviour of both, polar and non-polar phonons and their impact on the transition lattice…

Our measured dielectric constant and mechanical response of multiferroic BiFeO3 indicate four phase transitions below room temperature. Features correlate with those reported at 50K (from a peak in the zero-field-cooled magnetic…

Materials Science · Physics 2008-06-23 S. A. T. Redfern , C. Wang , J. W. Hong , G. Catalan , J. F. Scott

We present the electrodynamic response of TiOBr, which undergoes a transition to a spin-singlet ground state for temperatures below T$_{C1}=28$ K. The temperature evolution of the phonon anomalies indicates, like in \cl, an extended…

Materials Science · Physics 2009-11-10 G. Caimi , L. Degiorgi , P. Lemmens , F. C. Chou

We report the evolution of the Raman active A_g phonon modes in the charge-ordered manganite Pr_{0.63}Ca_{0.37}MnO_{3} as a function of temperature from 300K to 25K. Our studies reveal that the linewidths of A_g(2) and A_g(4) phonons…

Strongly Correlated Electrons · Physics 2009-11-07 Rajeev Gupta , G. Venketeswara Pai , A. K. Sood , T. V. Ramakrishnan , C. N. R. Rao

We measured the temperature dependent infrared reflectivity spectra of MnF2 between 4 K and room temperature. We show that the phonon spectrum undergoes a strong renormalization at TN. The ab-initio calculation we performed on this compound…

Materials Science · Physics 2010-10-20 R. Schleck , Y. Nahas , R. P. S. M. Lobo , J. Varignon , M. B. Lepetit , C. S. Nelson , R. L. Moreira

We report studies of polycrystalline samples of the metallic ferromagnet Pr0.5Sr0.5CoO3 through measurements of the magnetization, a.c. magnetic susceptibility, resistivity, and specific heat. We find an unusual anomaly around TA = 120 K,…

Materials Science · Physics 2009-11-10 R. Mahendiran , P. Schiffer

Multiferroics possess two or more switchable states such as polarization, magnetization, etc. Phonon excitations in multiferroic phase are strongly modified by magnetoelectric coupling, spin-phonon coupling, and anharmonic phonon-phonon…

Materials Science · Physics 2021-10-26 Bommareddy Poojitha , Ankit Kumar , Anjali Rathore , Surajit Saha

Raman scattering spectra of zigzag spin chain TaFe$_{1.25}$Te$_3$ single crystal are presented in a temperature range from 80 to 300 K. Nine Raman active modes of $A_g$ and $B_g$ symmetry are clearly observed and assigned by probing…

Type-II multiferroics, where spin interactions induce a ferroelectric polarization, are interesting for new device functionalities due to large magnetoelectric coupling. We report on a new type of multiferroicity in the quadruple-perovskite…

We report inelastic light scattering experiments on superconductor Ce0.6Y0.4FeAsO0.8F0.2 from 4K to 300K covering the superconducting transition temperature Tc ~ 48.6K. A strong evidence of the superconductivity induced phonon…

Materials Science · Physics 2015-06-17 Pradeep Kumar , D. V. S. Muthu , J. Prakash , A. K. Ganguli , A. K. Sood

We measured the temperature dependent infrared reflectivity spectra of TbMnO3 with the electric field of light polarized along each of the three crystallographic axes. We analyzed the effect, on the phonon spectra, of the different phase…

Materials Science · Physics 2011-06-23 R. Schleck , R. L. Moreira , H. Sakata , R. P. S. M. Lobo

The effect of pressure and temperature on the Raman-active phonon mode of osmium metal has been investigated for pressures up to 20 GPa and temperatures in the range 10--300 K. Under hydrostatic conditions (He pressure medium) the phonon…

Other Condensed Matter · Physics 2009-11-11 Yu. S. Ponosov , I. Loa , V. E. Mogilenskikh , K. Syassen

We investigate the magnetization dynamics of $TmFeO_3$ single crystals across the spin-reorientation phase transition using broadband microwave absorption spectroscopy up to 87.5 GHz. Temperature- and magnetic-field-dependent…

Conventional Paramagnetism - a state with finite magnetic moment per ion sans long range magnetic ordering, but with lowering temperature the moment on each ion picks up a particular direction, breaking rotational symmetry, and results into…

Strongly Correlated Electrons · Physics 2019-09-10 Birender Singh , Deepu Kumar , Kaustuv Manna , A. K. Bera , G. Aslan Cansever , A. Maljuk , S. Wurmehl , B. Büchner , Pradeep Kumar

Infrared reflection and transmission as a function of temperature have been measured on single crystals of Cu$_{3}$Bi(SeO$_{3}$)$_{2}$O$_{2}$Cl. The complex dielectric function and optical properties along all three principal axes of the…

Materials Science · Physics 2015-06-05 K. H. Miller , P. W. Stephens , C. Martin , E. Constable , R. A. Lewis , H. Berger , G. L. Carr , D. B. Tanner

A prominent band centered at around 1000-1300 cm-1 and associated with resonant enhancement of two-phonon Raman scattering is reported in multiferroic BiFeO3 thin films and single crystals. A strong anomaly in this band occurs at the…