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The coupling between localized spins and phonons can lead to shifts in the dielectric constant of insulating materials at magnetic ordering transitions. Studies on isostructural SeCuO3 (ferromagnetic) and TeCuO3 (antiferromagnetic)…

Materials Science · Physics 2009-04-14 G. Lawes , T. Kimura , C. M. Varma , M. A. Subramanian , R. J. Cava , A. P. Ramirez

We present a comprehensive study of polar and magnetic excitations in BiFeO3 ceramics and a thin film epitaxially grown on an orthorhombic (110) TbScO3 substrate. Infrared reflectivity spectroscopy was performed at temperatures from 5 to…

Materials Science · Physics 2015-05-22 S. Skiadopoulou , V. Goian , C. Kadlec , F. Kadlec , X. F. Bai , I. C. Infante , B. Dkhil , C. Adamo , D. G. Schlom , S. Kamba

In the iron pnictides, the strong sensitivity of the iron magnetic moment to the arsenic position suggests a significant relationship between phonons and magnetism. We measured the phonon dispersion of several branches in the high…

By means of neutron inelastic scattering, magnetic excitations and phonons were measured for a single crystal of slightly overdoped superconductor Ca10Pt4As8(Fe1-xPtxAs)10 (x ~ 0.2) with the transition temperature Tc of ~33 K. Below Tc,…

Strongly interacting phonons and orbital excitations are observed in the same energy range for CuSb$_2$O$_6$, unlocking a so-far unexplored type of electron-phonon interaction. An orbital wave at $\sim 550$ cm$^{-1}$ softens on warming and…

Strongly Correlated Electrons · Physics 2018-05-17 D. T. Maimone , A. B. Christian , J. J. Neumeier , E. Granado

We calculate the temperature dependence of NMR relaxation rate and electrical resistivity for coupling to a local, strongly anharmonic phonon mode. We argue that the two-phonon Raman process is dominating NMR relaxation. Due to the strong…

Superconductivity · Physics 2007-10-30 Thomas Dahm , Kazuo Ueda

We have observed a softening of phonons and a structural phase transition in a superconducting Ba0.59K0.41BiO3 (Tc = 31 K) single crystal using elastic and inelastic neutron scattering measurements. The soft phonon occurs for the [111]…

Superconductivity · Physics 2011-07-27 H. J. Kang , Y. S. Lee , J. W. Lynn , S. V. Shiryaev , S. N. Barilo

The dielectric constant of the incipient ferroelectric EuTiO$_3$ exhibits a sharp decrease at about 5.5K, at which temperature antiferromagnetic ordering of the Eu spins simultaneously appears, indicating coupling between the magnetism and…

Materials Science · Physics 2009-11-07 Qing Jiang , Hua Wu

We investigate the electronic and magnetic properties as well as lattice dynamics and spin-phonon coupling of $\beta$-Na$_{0.33}$V$_2$O$_5$ using temperature-dependent Raman scattering, dc-magnetization and dc-resistivity, x-ray…

Materials Science · Physics 2022-11-23 Rishabh Shukla , Clemens Ulrich , R. S. Dhaka

We report inelastic neutron scattering measurements of the phonon spectra in a pure powder sample of the multiferroic material BiFeO3. A high-temperature range was covered to unravel the changes in the phonon dynamics across the Neel (T_N ~…

Materials Science · Physics 2015-03-19 M. Zbiri , H. Schober , N. Choudhury , R. Mittal , S. L. Chaplot , S. J. Patwe , S. N. Achary , A. K. Tyagi

Recently colossal positive volume thermal expansion has been found in the framework compounds Ag3Co(CN)6 and Ag3Fe(CN)6. Phonon spectra have been measured using the inelastic neutron scattering technique as a function of temperature and…

Materials Science · Physics 2015-06-05 R Mittal , M. Zbiri , H. Schober , S. N. Achary , A. K. Tyagi , S. L. Chaplot

Phase transitions with lowering temperature is a manifestation of decreased entropy and within the Landau theoretical framework these are accompanied by the symmetry breaking. Whenever a symmetry is broken weakly or strongly, it leaves its…

Strongly Correlated Electrons · Physics 2023-12-12 Atul G. Chakkar , Deepu Kumar , Pradeep Kumar

We study the low-temperature heat transport, as well as the magnetization and the specific heat, of TmMnO_3 single crystals to probe the transitions of magnetic structure induced by magnetic field. It is found that the low-T thermal…

Strongly Correlated Electrons · Physics 2012-11-19 X. M. Wang , Z. Y. Zhao , C. Fan , X. G. Liu , Q. J. Li , F. B. Zhang , L. M. Chen , X. Zhao , X. F. Sun

Raman scattering in the three-dimensional Dirac semimetal Cd3As2 shows an intricate interplay of electronic and phonon degrees of freedom. We observe resonant phonon scattering due to interband transitions, an anomalous anharmonicity of…

Materials Science · Physics 2017-07-05 A. Sharafeev , V. Gnezdilov , R. Sankar , F. C. Chou , P. Lemmens

Magnetization measurements and time-of-flight neutron powder-diffraction studies on the high-temperature (300--980 K) magnetism and crystal structure (321--1200 K) of a pulverized YCrO$_3$ single crystal have been performed.…

Strongly Correlated Electrons · Physics 2021-11-04 Yinghao Zhu , Si Wu , Bao Tu , Shangjian Jin , Ashfia Huq , Joerg Persson , Haoshi Gao , Defang Ouyang , Zhubing He , Dao-Xin Yao , Zikang Tang , Hai-Feng Li

We report on the high-temperature evolution of far- and mid- infrared reflectivity and emissivity spectra of ambient orthorhombic ErMnO3 from 12 K to sample decomposition above 1800 K. At low temperatures the number of phonons agrees with…

Strongly Correlated Electrons · Physics 2018-11-13 Néstor E. Massa , Leire del Campo , Karsten Holldack , Vinh Ta Phuoc , Patrick Echegut , Paula Kayser , José Antonio Alonso

The temperature and magnetic field dependence of lattice and carrier excitations in MnSi is studied in detail using inelastic light scattering. The pure symmetry components of the electronic response are derived from the polarization…

Strongly Correlated Electrons · Physics 2014-07-23 H. -M. Eiter , P. Jaschke , R. Hackl , A. Bauer , M. Gangl , C. Pfleiderer

We report temperature-dependent Raman spectra of CeFeAsO0.9F0.1 from 4 K to 300 K in spectral range of 60 to 1800 cm-1 and interpret them using estimates of phonon frequencies obtained from first-principles density functional calculations.…

The Mn spin correlations were studied near the O'-O phase transition at T{JT} = 750 K, up to 950 K with 17O and 139La NMR in a stoichiometric LaMnO3 crystalline sample. The measured local hyperfine fields originate from the electron density…

Strongly Correlated Electrons · Physics 2015-06-15 A. Trokiner , S. Verkhovskii , A. Gerashenko , Z. Volkova , O. Anikeenok , K. Mikhalev , M. Eremin

The quasi-one-dimensional Ising spin chain system $\alpha$-CoV$_2$O$_6$ is considered to exhibit fascinating magnetic properties at lower temperatures. We comprehensively study magnetic properties and lattice dynamics using a combination of…

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