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Single-phase polycrystalline La2MnVO6 samples were synthesized by arc melting and characterized by X-ray diffraction, magnetization and resistivity measurements. We find that the compound has cubic (space group), partly ordered double…

Materials Science · Physics 2009-11-07 J. Androulakis , N. Katsarakis , J. Giapintzakis

In electronic solids with strong spin-orbit interactions (SOIs), the spin and orbital degrees of freedom of an electron are quantum mechanically entangled, which may result in an exotic multipolar order instead of a conventional dipolar…

Strongly Correlated Electrons · Physics 2020-07-01 Daigorou Hirai , Hajime Sagayama , Shang Gao , Hiroyuki Ohsumi , Gang Chen , Taka-hisa Arima , Zenji Hiroi

The band structure, optical and defects properties of Ba_{2}TeO are systematically investigated using density functional theory with a view to understanding its potential as an optoelectronic or trans- parent conducting material. Ba_{2}TeO…

Materials Science · Physics 2015-06-11 Jifeng Sun , Hongliang Shi , Mao-Hua Du , Theo Siegrist , David J. Singh

Organic-inorganic metal halide perovskites (HaPs) are intensively studied for their light-harvesting properties. Owing to the interplay between strong electron-electron interaction and spin-orbit coupling (SOC), their quantitative…

Materials Science · Physics 2021-11-02 Cecilia Vona , Dmitrii Nabok , Claudia Draxl

Based on density functional theory calculations and group theoretical analysis, we have studied NaLaMnWO$_{6}$ compound which has been recently synthesized [Phys. Rev. B 79, 224428 (2009)] and belongs to the $AA'BB'{\rm O}_{6}$ family of…

Materials Science · Physics 2017-09-13 T. Fukushima , A. Stroppa , S. Picozzi , J. M. Perez-Mato

Using transmission electron microscopy (TEM) we studied CaCu3Ti4O12, an intriguing material that exhibits a huge dielectric response, up to kilohertz frequencies, over a wide range of temperature. Neither in single crystals, nor in…

Materials Science · Physics 2009-11-10 L. Wu , Y. Zhu , S. Park , S. Shapiro , G. Shirane , J. Tafto

In this paper, we employ CASTEP based on DFT (density functional theory) calculations to investigate various physical properties of BaVO3, SrVO3, CaVO3 and PbVO3. The elastic constants, bulk modulus, Shear modulus, Young's modulus, Pugh's…

Double-perovskite oxides that contain both 3d and 5d transition metal elements have attracted growing interest as they provide a model system to study the interplay of strong electron interaction and large spin-orbit coupling (SOC). Here,…

Strongly Correlated Electrons · Physics 2016-09-01 W. K. Zhu , J. -C. Tung , W. Tong , L. Ling , M. Starr , J. M. Wang , W. C. Yang , Y. Losovyj , H. D. Zhou , Y. Q. Wang , P. -H. Lee , Y. -K. Wang , Chi-Ken Lu , S. X. Zhang

We report on the synthesis of complex lead-free perovskite-type (1-x)(Ba$_{0.8}$Ca$_{0.2}$)TiO$_3$-xBi(Mg$_{0.75}$W$_{0.25}$)O$_3$ (BCT-xBMW) and (1-x)(Ba$_{0.8}$Ca$_{0.2}$)TiO$_3$-xBi(Mg$_{0.75}$Mo$_{0.25}$)O$_3$ (BCT-xBMM) solid solutions…

Materials Science · Physics 2021-11-02 Thomas Schulz , Vignaswaran K. Veerapandiyan , Theresa Gindel , Marco Deluca , Jörg Töpfer

In this review, I present the electronic properties of the beta-pyrochlore oxide CsW2O6 and other related materials. At 215 K, CsW2O6 exhibits an electronic phase transition to a nonmagnetic insulating state, which exhibits a complex…

Materials Science · Physics 2024-09-06 Yoshihiko Okamoto

We describe a first open-access database of experimentally investigated hybrid organic-inorganic materials with two-dimensional (2D) perovskite-like crystal structure. The database includes 515 compounds, containing 180 different organic…

Ab initio calculations using the APW+lo method as implemented in the WIEN2k code have been used to describe the electronic structure of the quasi-one-dimensional system BaCoO3. Both, GGA and LDA+U approximations were employed to study…

Strongly Correlated Electrons · Physics 2009-11-10 V. Pardo , P. Blaha , M. Iglesias , K. Schwarz , D. Baldomir , J. E. Arias

Bismuthate superconductor Ba(1-x)K(x)BiO3 (x=0.27-0.49, Tc=25-32K) grown by an electrolysis technique was studied by electron diffraction and high-resolution electron microscopy. The crystalline structure thereof has been found to be…

Superconductivity · Physics 2009-11-10 L. A. Klinkova , M. Uchida , Y. Matsui , V. I. Nikolaichik , N. V. Barkovskii

In this study, we report a tetragonal perovskite structure of SrIrO$_3$ (P4/mmm, a = 3.9362(9) \r{A}, c = 7.880(3) \r{A}) synthesized at 6 GPa and 1400 $\deg$C, employing the ambient pressure monoclinic SrIrO$_3$ with distorted 6H structure…

The geometrically frustrated double perovskite Ba2YRuO6 has magnetic 4d3 Ru5+ ions decorating an undistorted face-centered cubic (FCC) lattice. This material has been previously reported to exhibit commensurate long-range antiferromagnetic…

Strongly Correlated Electrons · Physics 2013-07-23 J. P. Carlo , J. P. Clancy , K. Fritsch , C. A. Marjerrison , G. E. Granroth , J. E. Greedan , H. A. Dabkowska , B. D. Gaulin

Double perovskites Cs$_2$Au$_2$X$_6$ (X=Cl, Br, I) are prototypical materials that exhibit charge disproportionation of gold into 1+ and 3+ states. It is known that the disproportionation is resolved under high pressures, and this has…

Materials Science · Physics 2024-05-16 Kazuki Morita , Andrew M. Rappe

Tuning the work functions of materials is of practical interest for maximizing the performance of microelectronic and (photo)electrochemical devices, as the efficiency of these systems depends on the ability to control electronic levels at…

Materials Science · Physics 2021-04-07 Yihuang Xiong , Weinan Chen , Wenbo Guo , Hua Wei , Ismaila Dabo

We present the self-interaction corrected local spin density (SIC-LSD) electronic structure and total energy calculations, leading also to valencies of the ground state configurations, for the half-metallic double perovskites such as…

Strongly Correlated Electrons · Physics 2009-11-10 Z. Szotek , W. M. Temmerman , A. Svane , L. Petit , H. Winter

Various physical properties (electronic, optical and thermoelectric) of cubic perovskite oxides $SrXO_3\; (X=Sc,\; Ge,\; Si)$ are investigated by using the density functional theory (DFT) within Wien2k code. This code is based on different…

Materials Science · Physics 2022-11-15 A Waqdim , M Agouri , A Abbassi , B. Elhadadi , Z. Zidane , S Taj , B Manaut , M Driouich , M El Idrissi

We predict through our first-principles calculations that four double perovskite oxides of Bi2ABO6 (AB = FeMo, MnMo, MnOs, CrOs) are half-metallic ferrimagnets. Our calculated results shows that the four optimized structures have negative…

Materials Science · Physics 2013-01-31 Si-Da Li , Peng Chen , Bang-Gui Liu