Related papers: Efficient spectral hole-burning and atomic frequen…
While Rydberg atoms have shown tremendous potential to serve as accurate and sensitive detectors of microwaves and millimeter waves, their response is generally limited to a single narrow frequency band around a chosen microwave transition.…
Noise-immune cavity-enhanced optical frequency comb spectroscopy (NICE-OFCS) is a recently developed technique that utilizes phase modulation to obtain immunity to frequency-to-amplitude noise conversion by the cavity modes and yields high…
Material absorption is a key limitation in nanophotonic systems; however, its characterization is often obscured by scattering and diffraction loss. Here we show that nanomechanical frequency spectroscopy can be used to characterize the…
Non-thermal molecular plasmas play a crucial role in numerous industrial processes and hold significant potential for driving essential chemical transformations. Accurate information about the molecular composition of the plasmas and the…
Density functional theory $(DFT)$ studies show that doping of $3d TM$ atoms into $Mg_4^{0,+} (TMMg_3^{0,+})$ can alter the endothermic nature of molecular hydrogen adsorption on bare $Mg_4^{0,+}$. $H_2$ adsorption on $TMMg_3^{0,+}$ clusters…
Dual-comb spectroscopy has been proven a powerful tool in molecular characterization, which remains challenging to implement in the mid-infrared region due to difficulties in the realization of two mutually locked comb sources and efficient…
Optical frequency conversion has applications ranging from tunable light sources to telecommunications-band interfaces for quantum information science. Here, we demonstrate efficient, low-noise frequency conversion on a nanophotonic chip…
Streamlined prediction of the electronic properties of photoactive materials warrants a Density Functional Theory (DFT) based approach that (i) yields reliable bandgaps, (ii) is free of empirically tuned parameters, and (iii) exhibits low…
Here we propose a solid-state quantum memory that does not require spectral holeburning, instead using strong rephasing pulses like traditional photon echo techniques. The memory uses external broadening fields to reduce the optical depth…
Optical frequency combs are utilized in a wide range of optical applications, including atomic clocks, interferometers, and various sensing technologies. They are often generated via four-wave mixing in chip-integrated microring resonators,…
Rare-earth (RE) ion doped nano-materials are promising candidates for a range of quantum technology applications. Among RE ions, the so-called Kramers' ions possess spin transitions in the GHz range at low magnetic fields, which allows for…
The quest for extrasolar planets and their characterisation as well as studies of fundamental physics on cosmological scales rely on capabilities of high-resolution astronomical spectroscopy. A central requirement is a precise wavelength…
We characterize a new mid-infrared frequency comb generator based on difference frequency generation around 3.2 microns. High power per comb mode (>10-7 W/mode) is obtained over a broad spectral span (>700 nm). The source is used for direct…
We have measured the frequency of the $6s^2S_{1/2} - 5d^2D_{3/2}$ electric-quadrupole transition of $^{171}$Yb$^+$ with a relative uncertainty of $1\times 10^{-14}$, $\nu_{Yb}$ = 688 358 979 309 312 Hz $\pm$ 6 Hz. A femtosecond frequency…
We present an experiment demonstrating high-resolution coherent control of a four-level atomic system in a closed (diamond) type configuration. A femtosecond frequency comb is used to establish phase coherence between a pair of two-photon…
We consider transitions of electron holes (vacancies in otherwise filled shells of atomic systems) in multiply-charged ions that, due to level-crossing of the holes, have frequencies within the range of optical atomic clocks. Strong E1…
We use spectral hole burning to investigate spin dynamics within the electronic Zeeman sublevels of the ground state of the erbium ions in erbium-doped fibers (EDF). Conducted at ultra-low temperatures and under varying magnetic fields, our…
Light guided by an optical nanofibre can have a very steep evanescent field gradient extending from the fibre surface. This can be exploited to drive electric quadrupole transitions in nearby quantum emitters. In this paper, we report on…
In this work we report about the fundamental correspondence between the high efficiency of the broadband quantum memory on multifrequency absorbers in the single-mode cavity and the topology of the observed frequency lines. We have found…
Frequency-modulated (FM) laser combs, which offer a periodic quasi-continuous-wave output and a flat-topped optical spectrum, are emerging as a promising solution for wavelength-division multiplexing applications, precision metrology, and…