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In this work, the $4D_{3/2}|3,\pm2\rangle \rightarrow 4D_{5/2}|3,\pm2\rangle$ transition in the Nb$^{4+}$ ion is identified as a promising candidate for a terahertz (THz) atomic clock, with the transition frequency occurring at 56.0224 THz.…

Atomic Physics · Physics 2025-04-23 Jyoti , A. Chakraborty , Zhiyang Wang , Jia Zhang , Jingbiao Chen , Bindiya Arora , B. K. Sahoo

Frequency comb spectroscopy has significantly advanced molecular spectroscopy across scientific research and diverse applications. Among its key performance metrics especially for time-resolved studies, sensitivity and measurement speed are…

We report rest frequencies for rotational transitions of the deuterated ammonium isotopologues NH3D+, NH2D2+ and NHD3+, measured in a cryogenic ion trap machine. For the symmetric tops NH3D+ and NHD3+ one and three transitions are detected,…

Astrophysics of Galaxies · Physics 2018-10-31 José-Luis Doménech , Stephan Schlemmer , Oskar asvany

We demonstrate a 0.95 GHz repetition rate fully stabilized Yb:fiber frequency comb without optical amplification. Benefitted from the high mode power and high coherence, this comb achieved 35 dB to 42 dB signal to noise ratio on the direct…

Optics · Physics 2019-10-02 Yuxuan Ma , Fei Meng , Yan Wang , Aimin Wang , Zhigang Zhang

Neutral atom arrays have emerged as a powerful platform for quantum computation, simulation, and metrology. Among them, alkaline-earth-like atoms exhibit distinct advantages, including long coherence time and high-fidelity Rydberg gates.…

We report molecular detection using dual frequency-comb spectroscopy with highly coherent broadband (6.6-11.4 {\m}m) long-wavelength infrared (LWIR) combs. The combs were produced via intra-pulse difference frequency generation (IDFG) in…

We present high S/N echelle spectra of the recently discovered ultraluminous QSO APM 08279+5255 and use these data to re-examine the abundance of Carbon in Ly alpha forest clouds. In agreement with previous work, we find that approximately…

We demonstrate high-resolution photonic RF filters using an RF bandwidth scaling approach based on integrated Kerr optical micro-combs. By employing both an active nonlinear micro-ring resonator (MRR) as a high-quality micro-comb source and…

Atom-based radio frequency electromagnetic field sensing using atomic Rydberg states is a promising technique that has recently attracted significant interest. Its unique advantages, such as extraordinary bandwidth, self-calibration and…

Atomic Physics · Physics 2022-09-07 Katelyn Dixon , Kent Nickerson , Donald W. Booth , James P. Shaffer

We report precision spectroscopy of ionic-core transitions in alkaline-earth Rydberg atoms. We demonstrate high-resolution measurements of isotope shifts and hyperfine splitting of dipole transitions in ionic cores which have not been…

Atomic Physics · Physics 2026-05-20 Mitsuki Odahara , Shinsuke Haze

Accurate Fourier-transform spectroscopic absorption measurements of vacuum ultraviolet transitions in atomic nitrogen and carbon were performed at the Soleil synchrotron. For $^{14}$N transitions from the $2s^22p^3\,^4$S$_{3/2}$ ground…

Atomic Physics · Physics 2020-09-04 K. -F. Lai , W. Ubachs , N. de Oliveira , E. J. Salumbides

We demonstrate fiber mode-locked dual frequency comb spectroscopy for broadband, high resolution measurements in a rapid compression machine (RCM). We apply an apodization technique to improve the short-term signal-to-noise-ratio (SNR),…

A phase-stabilized femtosecond laser comb is directly used for high-resolution spectroscopy and absolute optical frequency measurements of one- and two-photon transitions in laser-cooled \rb atoms. Absolute atomic transition frequencies,…

Atomic Physics · Physics 2009-11-11 Adela Marian , Matthew C. Stowe , Daniel Felinto , Jun Ye

We report the development of a new instrument for cavity-enhanced absorption spectroscopy of the fundamental rovibrational transitions of molecules in the long-wave mid-infrared (LWIR) region from 6500 to 10000 nm. Our setup combines a LWIR…

We demonstrate dual-comb spectroscopy based on difference frequency generation of frequency-agile near-infrared frequency combs, produced with the help of electro-optic modulators. The combs have a remarkably flat intensity distribution and…

$^{133}\text{Ba}^+$ has been identified as an attractive ion for quantum information processing due to the unique combination of its spin-1/2 nucleus and visible wavelength electronic transitions. Using a microgram source of radioactive…

Quantum Physics · Physics 2017-09-13 David Hucul , Justin E. Christensen , Eric R. Hudson , Wesley C. Campbell

Sustained mutual coherence between two combs over extended periods is a prerequisite for dual-comb spectroscopy (DCS), particularly in achieving high-resolution molecular spectroscopy and precise spectral measurements. However, achieving…

We use a Fourier transform spectrometer based on a compact mid-infrared difference frequency generation comb source to perform broadband high-resolution measurements of nitrous oxide, $^{14}$N$_2$$^{16}$O, and retrieve line center…

We observe an inverted crossover resonance in $\pi$-driven four-level systems, where $F'-F=0,+1$. The signal is observed through saturated absorption spectroscopy of the $(6s^{2})$ $^{1}S_{0}$ $-$ $(6s6p)$ $^{3}P_{1}$ transition in…

Atomic Physics · Physics 2016-05-31 J. J. McFerran

A compact and robust coherent laser light source that provides spectral coverage from the ultraviolet to infrared is desirable for numerous applications, including heterodyne super resolution imaging[1], broadband infrared microscopy[2],…