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We demonstrate the use of a femtosecond frequency comb to coherently drive stimulated Raman transitions between terahertz-spaced atomic energy levels. More specifically, we address the $3d~^2D_{3/2}$ and $3d~^2D_{5/2}$ fine structure levels…

Quantum Physics · Physics 2018-06-21 Cyrille Solaro , Steffen Meyer , Karin Fisher , Michael V. DePalatis , Michael Drewsen

We suggest an all-optical scheme for the storage, retrieval and processing of a single-photon wave packet through its off-resonant Raman interaction with a series of coherent control beams. These control beams, each with distinct carrier…

Quantum Physics · Physics 2016-12-09 Xiwen Zhang , Alexey Kalachev , Philip Hemmer , Olga Kocharovskaya

We present a demonstration of simultaneous high-efficiency, high-speed, and low-noise operation of a photonic quantum memory. By leveraging controllable collisional dephasing in a neutral barium atomic vapor, we demonstrate a significant…

Various near-term quantum networking applications will benefit from low-loss, fiber-coupled photonic quantum memory devices with high efficiencies. We demonstrate a fiber-coupled loop-and-switch quantum memory platform with a pass-through…

Quantum Physics · Physics 2025-10-23 Sandra Cheng , Carson Evans , Todd Pittman

We present and analyze four frequency measurements designed to characterize the performance of an optical frequency reference based on spectral hole burning in \EuYSO. The first frequency comparison, between a single unperturbed spectral…

The ground-state 4f fine-structure levels in the intrinsic optical transition gaps between the 2p and 5d orbitals of lanthanide sesquioxides (Ln2O3, Ln=La...Lu) were calculated by a two-way crossover search for the U parameters for DFT+U…

Strongly Correlated Electrons · Physics 2015-11-17 Bolong Huang

Frequency-modulated lasers (FMLs) are widely used in spectroscopy, biology, and LiDAR. The performance of these applications highly depends on the fast and precise tracking of the FMLs' absolute frequency, which remains a challenge. Here we…

Optics · Physics 2025-08-25 Weiwei Yang , Xingyu Jia , Jingyi Wang , Xinlun Cai , Yang Li , Guanhao Wu

We demonstrate coherent dual frequency-comb spectroscopy for detecting variations in greenhouse gases. High signal-to-noise spectra are acquired spanning 5990 to 6260 cm^-1 (1600 to 1670 nm) covering ~700 absorption features from CO2, CH4,…

We argue that long optical storage times are required to establish entanglement at high rates over large distances using memory-based quantum repeaters. Triggered by this conclusion, we investigate the $^3$H$_6$ $\leftrightarrow$ $^3$H$_4$…

We demonstrate experimentally a quantum memory scheme for the storage of weak coherent light pulses in an inhomogeneously broadened optical transition in a Pr^{3+}: YSO crystal at 2.1 K. Precise optical pumping using a frequency stable…

Quantum Physics · Physics 2015-05-14 M. Sabooni , F. Beaudoin , A. Walther , N. Lin , A. Amari , M. Huang , S. Kröll

A $\gamma$-ray-nuclear quantum interface is suggested as a new platform for quantum information processing, motivated by remarkable progresses in $\gamma$-ray quantum optics. The main advantages of a $\gamma$ photon over an optical photon…

Direct frequency comb spectroscopy of trapped ions is demonstated for the first time. It is shown that the 4s^2S_(1/2)-4p^2P_(3/2) transition in calcium ions can be excited directly with a frequency comb laser that is upconverted to 393 nm.…

Atomic Physics · Physics 2009-06-08 A. L. Wolf , S. A. van den Berg , W. Ubachs , K. S. E. Eikema

A systematic computational study on the structural, electronic, bonding, and optical properties of orthorhombic ammonium azide (NH$_4$N$_3$) has been performed using planewave pseudopotential (PW-PP) method based on density functional…

Materials Science · Physics 2013-11-07 N. Yedukondalu , Vikas D. Ghule , G. Vaitheeswaran

The detection of ultrafast optical and radio-frequency (RF) signals is crucial for applications ranging from high-speed communications to advanced sensing. However, conventional detectors are fundamentally constrained by their intrinsic…

Long-duration and efficient quantum memories for photons are key components of quantum repeater and network applications. To achieve long duration storage in atomic systems, a short-lived optical coherence can be mapped into a long-lived…

Quantum Physics · Physics 2026-02-11 Jingjing Chen , Mikael Afzelius

Optical frequency combs are indispensable links between the optical and microwave domains, enabling a wide range of applications including precision spectroscopy, ultrastable frequency generation, and timekeeping. Chip-scale integration…

Optics · Physics 2024-02-20 Yunxiang Song , Yaowen Hu , Marko Lončar , Kiyoul Yang

Using an ultrastable continuous-wave laser at 580 nm we performed spectral hole burning of Eu$^{3+}$:Y$_{2}$SiO$_{5}$ at very high spectral resolution. Essential parameters determining the usefulness as a "macroscopic" frequency reference:…

Quantum networks will enable a variety of applications, from secure communication and precision measurements to distributed quantum computing. Storing photonic qubits and controlling their frequency, bandwidth and retrieval time are…

Quantum Physics · Physics 2020-08-26 Ioana Craiciu , Mi Lei , Jake Rochman , John G. Bartholomew , Andrei Faraon

Hybrid quantum networks rely on efficient interfacing of dissimilar quantum nodes, since elements based on parametric down-conversion sources, quantum dots, color centres or atoms are fundamentally different in their frequencies and…

The highly energetic photons of ultraviolet light drive electronic and rovibronic transitions in all molecular species. This radiation is thus a prime tool for strongly selective spectroscopic fingerprinting and real-time environmental…

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