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We have studied (Tb$_{1-x}$La$_x$)$_2$Mo$_2$O$_7$ pyrochlores by neutron diffraction and $\mu$SR at ambient and under applied pressure. Substitution of Tb for La expands the lattice and induces a change from a spin-glass like state…

Strongly Correlated Electrons · Physics 2007-05-23 A. Apetrei , I. Mirebeau , I. Goncharenko , D. Andreica , P. Bonville

Some frustrated pyrochlore antiferromagnets, such as Y2Mo2O7, show a spin-freezing transition and magnetic irreversibilities below a temperature Tf similar to what is observed nonlinear magnetization measurements on Y2Mo2O7 that provide…

Disordered Systems and Neural Networks · Physics 2009-10-28 M. J. P. Gingras , C. V. Stager , N. P. Raju , B. D. Gaulin , J. E. Greedan

We report neutron scattering studies of the spin correlations of the geometrically frustrated pyrochlore Tb2Mo2O7 using single crystal samples. This material undergoes a spin-freezing transition below Tg~24 K, similar to Y2Mo2O7, and has…

Strongly Correlated Electrons · Physics 2009-11-13 D. K. Singh , J. S. Helton , S. Chu , T. H. Han , C. J. Bonnoit , S. Chang , H. J. Kang , J. W. Lynn , Y. S. Lee

In frustrated magnetic systems, geometric constraints or the competition amongst interactions introduce extremely high degeneracy and prevent the system from readily selecting a low-temperature ground state. The most frustrated known spin…

Strongly Correlated Electrons · Physics 2016-11-23 Darren C. Peets , Hasung Sim , Maxim Avdeev , Je-Geun Park

We study the effect in geometrically frustrated antiferromagnets of weak, random variations in the strength of exchange interactions. Without disorder the simplest classical models for these systems have macroscopically degenerate ground…

Disordered Systems and Neural Networks · Physics 2010-05-05 A. Andreanov , J. T. Chalker , T. E. Saunders , D. Sherrington

Two geometrically frustrated pyrochlore stannates, undergoing long range magnetic order below 1K, were investigated at very low temperature. Anomalies in the behaviour of hyperfine quantities are found, by 155Gd Mossbauer spectroscopy in…

Strongly Correlated Electrons · Physics 2009-11-13 P. Bonville , I. Mirebeau , J. P. Sanchez

Motivated by puzzling characteristics of spin-glass transitions widely observed in pyrochlore-based frustrated materials, we investigate effects of coupling to local lattice distortions in a bond-disordered antiferromagnet on the pyrochlore…

Strongly Correlated Electrons · Physics 2011-07-22 Hiroshi Shinaoka , Yusuke Tomita , Yukitoshi Motome

R$_2$Mo$_2$O$_7$ compounds show a ferromagnetic metal-insulator spin glass transition tuned by the radius of the rare earth ion R$^{3+}$. We have studied Gd$_2$Mo$_2$O$_7$ located on the verge of the transition, by neutron diffraction on a…

Strongly Correlated Electrons · Physics 2007-05-23 I. Mirebeau , A. Apetrei , I. Goncharenko , D. Andreica , P. Bonville , J. P. Sanchez , A. Amato , E. Suard , W. A. Crichton

In this study, I have investigated the magnetic and critical properties of manganese pyrochlore fluoride NaSrMn$_{2}$F$_{7}$, which exhibits a glass transition at T$_\text{f}$$=$2.5 (K) due to charge disorder. A DFT+$U$+SOC framework is…

Strongly Correlated Electrons · Physics 2023-05-09 Mohammad Amirabbasi

The very low temperature properties of two pyrochlore compounds, Yb2Ti2O7 and Gd2Sn2O7, were investigated using an ensemble of microscopic and bulk techniques. In both compounds, a first order transition is evidenced, as well as spin…

A "supercooled" liquid develops when a fluid does not crystallize upon cooling below its ordering temperature. Instead, the microscopic relaxation times diverge so rapidly that, upon further cooling, equilibration eventually becomes…

We report a study of the low temperature bulk magnetic properties of the spin ice compound Dy2Ti2O7 with particular attention to the (T < 4 K) spin freezing transition. While this transition is superficially similar to that in a spin glass,…

Materials Science · Physics 2007-05-23 J. Snyder , B. G. Ueland , J. S. Slusky , H. Karunadasa , R. J. Cava , P. Schiffer

Muon spin rotation and relaxation experiments in the pyrochlore iridate Eu2Ir2O7 yield a well-defined muon spin precession frequency below the metal-insulator/antiferromagnetic transition temperature TM = 120 K, indicative of long-range…

Strongly Correlated Electrons · Physics 2015-03-19 Songrui Zhao. J. M. Mackie , D. E. MacLaughlin , O. O. Bernal , J. J. Ishikawa , Y. Ohta , S. Nakatsuji

It is unexpected that a spin-glass transition, which generally occurs only in the system with some form of disorder, was observed in the ThCr2Si2-type compound PrAu2Si2 at a temperature of ~3 K. This puzzling phenomenon was later explained…

Strongly Correlated Electrons · Physics 2021-09-17 D. X. Li , Y. Shimizu , A. Nakamura , Y. J. Sato , A. Maurya , Y. Homma , F. Honda , D. Aoki

In the series La_{2/3-x}Tb_{x}Ca_{1/3}MnO_{3}, it is known that the compositions are ferromagnetic for smaller values of x and show spin glass characteristics at larger values of x. Our studies on the magnetic properties of various…

Strongly Correlated Electrons · Physics 2009-11-13 C. Raj Sankar , S. Vijayanand , P. A. Joy

Geometrical frustration, as in pyrochlore lattices made of corner-sharing tetrahedra, precludes the onset of conventional magnetic ordering, enabling the stabilization of fluctuating spin states at low temperature. Disorder is a subtle…

Various physical properties of the pyrochlore oxide Y2-xBixIr2O7 have been studied. The magnetizations M measured under the conditions of the zero-field-cooling(ZFC) and the field-cooling(FC) have different values below the temperature…

Strongly Correlated Electrons · Physics 2009-11-10 Natsuki Aito , Minoru Soda , Yoshiaki Kobayashi , Masatoshi Sato

The glassy behavior observed in the pyrochlore magnet Y2Mo2O7, where the magnetic Mo^{4+} ions interact predominantly via isotropic nearest neighbor antiferromagnetic exchange, possibly with additional weak disorder, is a distinct class of…

Statistical Mechanics · Physics 2010-09-08 Ka-Ming Tam , Adam J. Hitchcock , Michel J. P. Gingras

The description of thermodynamic phase transitions in terms of percolation transitions of suitably defined clusters has a long tradition and boasts a number of important successes, the most prominent ones being in ferromagnetic lattice…

Disordered Systems and Neural Networks · Physics 2024-08-20 Lambert Münster , Martin Weigel

The magnetisation relaxations of three different types of geometrically frustrated magnetic systems have been studied with the same experimental procedures as previously used in spin glasses. The materials investigated are Y$_2$Mo$_2$O$_7$…

Disordered Systems and Neural Networks · Physics 2009-11-10 F. Ladieu , F. Bert , V. Dupuis , E. Vincent , J. Hammann
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