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Surface tension-driven flow techniques have recently emerged as an efficient means of shedding light into the rheology of thin polymer films. Motivated by experimental and theoretical approaches in films bearing a varying surface…

Soft Condensed Matter · Physics 2017-04-26 Ioannis Tanis , Hendrik Meyer , Thomas Salez , Elie Raphaël , Anthony C. Maggs , Jörg Baschnagel

The surface of a thin liquid film with nonconstant curvature is unstable, as the Laplace pressure drives a flow mediated by viscosity. We present the results of experiments on one of the simplest variable curvature surfaces: a stepped…

Soft Condensed Matter · Physics 2015-06-11 Joshua D. McGraw , Thomas Salez , Oliver Bäumchen , Elie Raphaël , Kari Dalnoki-Veress

A thin liquid film with non-zero curvature at its free surface spontaneously flows to reach a flat configuration, a process driven by Laplace pressure gradients and resisted by the liquid's viscosity. Inspired by recent progresses on the…

We present experiments to study the relaxation of a nano-scale cylindrical perturbation at one of the two interfaces of a thin viscous free-standing polymeric film. Driven by capillarity, the film flows and evolves towards equilibrium by…

Soft Condensed Matter · Physics 2020-05-13 Vincent Bertin , John Niven , Howard A. Stone , Thomas Salez , Elie Raphael , Kari Dalnoki-Veress

We study theoretically the profile evolution of a thin viscoelastic film supported onto a no-slip flat substrate. Due to the nonconstant initial curvature at the free surface, there is a flow driven by Laplace pressure and mediated by…

Soft Condensed Matter · Physics 2014-05-16 Michael Benzaquen , Thomas Salez , Elie Raphaël

The morphology of crystalline thin films evolving on flat rigid substrates by condensation of extra film atoms or by evaporation of their own atoms in the surrounding vapor is studied in the framework of the theory of Stress Driven…

Analysis of PDEs · Mathematics 2024-11-05 Paolo Piovano , Francesco Sapio

We report on the capillary-driven levelling of a topographical perturbation at the surface of a free-standing liquid nanofilm. The width of a stepped surface profile is found to evolve as the square root of time. The hydrodynamic model is…

We study the free-surface deformation dynamics of an immersed glassy thin polymer film supported on a substrate, induced by an air nanobubble at the free surface.We combine analytical and numerical treatments of the glassy thin film…

Materials Science · Physics 2021-04-08 Christian Pedersen , Shuai Ren , Yuliang Wang , Andreas Carlson , Thomas Salez

Liquid films coating vertical cylinders can form annular liquid collars which translate downwards under gravity. We investigate the dynamics of a thin viscoplastic liquid film coating the interior or exterior of a vertical cylindrical tube,…

We report on the numerical implementation of thin film equations that describe the capillary-driven evolution of viscous films, in two-dimensional configurations. After recalling the general forms and features of these equations, we focus…

We find solutions that describe the levelling of a thin fluid film, comprising a non-Newtonian power-law fluid, that coats a substrate and evolves under the influence of surface tension. We consider the evolution from both periodic and…

Fluid Dynamics · Physics 2024-04-12 Michael C Dallaston

The relaxation dynamics of the contact angle between a viscous liquid and a smooth substrate is studied at the nanoscale. Through atomic force microscopy measurements of polystyrene nanostripes we monitor simultaneously the temporal…

Soft Condensed Matter · Physics 2015-12-03 Marco Rivetti , Thomas Salez , Michael Benzaquen , Elie Raphaël , Oliver Bäumchen

Thin liquid films on surfaces are part of our everyday life, they serve e.g. as coatings or lubricants. The stability of a thin layer is governed by interfacial forces, described by the effective interface potential, and has been subject of…

Soft Condensed Matter · Physics 2015-06-04 Oliver Bäumchen , Renate Fetzer , Mischa Klos , Matthias Lessel , Ludovic Marquant , Hendrik Hähl , Karin Jacobs

The study of viscous thin film flow has led to the development of highly nonlinear partial differential equations that model how the evolution of the film height is affected by different forces. We investigate a model of interaction between…

Fluid Dynamics · Physics 2024-07-25 Steven A Kedda , Michael C Dallaston , Scott W McCue

Liquid nanofilms are ubiquitous in nature and technology, and their equilibrium and out-of-equilibrium dynamics are key to a multitude of phenomena and processes. We numerically study the evolution and rupture of viscous nanometric films,…

The duality between deformations of elastic bodies and non-inertial flows in viscous liquids has been a guiding principle in decades of research. However, this duality is broken when a spheroidal or other doubly-curved liquid film is…

Soft Condensed Matter · Physics 2023-07-20 Benny Davidovitch , Avraham Klein

Flow in thin films is highly dependent on the boundary conditions. Here, we study the capillary levelling of thin bilayer films composed of two immiscible liquids. Specifically, a stepped polymer layer is placed atop another, flat polymer…

Soft Condensed Matter · Physics 2021-01-27 Vincent Bertin , Carmen Lee , Thomas Salez , Elie Raphael , Kari Dalnoki-Veress

Thin viscous liquid films driven by capillarity are well described in the lubrication theory through the thin film equation. In this article, we present an analytical solution of this equation for a particular initial profile: a stepped…

Soft Condensed Matter · Physics 2015-06-11 Thomas Salez , Joshua D. McGraw , Oliver Bäumchen , Kari Dalnoki-Veress , Élie Raphaël

We showed that a wetting layer in epitaxially strained thin films which decreases with increasing lattice mismatch strain arises due to the variation of nonlinear elastic free energy with film thickness. We calculated how and at what…

Materials Science · Physics 2007-05-23 Helen R. Eisenberg Daniel Kandel

We compare the capillary levelling of a random surface perturbation on a thin polystyrene film with a theoretical study on the two-dimensional capillary-driven thin film equation. Using atomic force microscopy, we follow the time evolution…

Soft Condensed Matter · Physics 2014-10-16 Michael Benzaquen , Paul Fowler , Laetitia Jubin , Thomas Salez , Kari Dalnoki-Veress , Elie Raphaël
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