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Physical parameters characterising electrokinetic transport in a confined electrolyte solution are reconstructed from the generic transport coefficients obtained within the classical non-equilibrium statistical thermodynamic framework. The…

Soft Condensed Matter · Physics 2014-11-18 Hiroaki Yoshida , Hideyuki Mizuno , Tomoyuki Kinjo , Hitoshi Washizu , Jean-Louis Barrat

The electrostatic interaction between two non-identical, moderately charged colloids situated in close proximity of each other at a fluid interface is studied. By resorting to a well-justified model system, this problem is analytically…

Soft Condensed Matter · Physics 2018-04-30 Arghya Majee , Timo Schmetzer , Markus Bier

This theoretical study investigates the nonlinear ionic current-voltage characteristics of nano-channels that have weakly overlapping electrical double layers. Numerical simulations as well as a 1-D mathematical model are developed to…

Chemical Physics · Physics 2017-01-10 Yang Liu , Lingzi Guo , Xin Zhu , Qiushi Ran , Robert Dutton

A model is developed for describing the transport of charged colloidal particles in an evaporating sessile droplet on the electrified metal substrate in the presence of a solvent flow. The model takes into account the electric charge of…

Soft Condensed Matter · Physics 2022-03-16 Semen V. Zavarzin , Andrei L. Kolesnikov , Yury A. Budkov , Lev Yu. Barash

We study here the curious particle dynamics resulting from electro-osmotic flow around a microchannel junction corner whose dielectric walls are weakly polarizable. The hydrodynamic velocity field is obtained via superposition of a linear…

Fluid Dynamics · Physics 2015-06-19 Matan Zehavi , Gilad Yossifon

Selectivity towards positive and negative ions in nanopores is often associated with electroosmotic flow, the control of which is pivotal in several micro-nanofluidic technologies. Selectivity is traditionally understood to be a consequence…

Fluid Dynamics · Physics 2022-04-21 Giovanni Di Muccio , Blasco Morozzo della Rocca , Mauro Chinappi

Catalytic bimetallic Janus particles swim by a bipolar electrochemical propulsion mechanism that results from electroosmotic fluid slip around the particle surface. The flow is driven by electrical body forces which are generated from a…

Fluid Dynamics · Physics 2015-06-17 Jeffrey L. Moran , Jonathan D. Posner

We present a numerical study of polyelectrolytes electrophoresing in free solution while squeezed by an axisymmetric confinement force transverse to their net displacement. Hybrid multi-particle collision dynamics and molecular dynamics…

Soft Condensed Matter · Physics 2016-06-22 Tyler N. Shendruk , Martin Bertrand , Gary W. Slater

Theoretical modeling of electroosmosis through conducting (ideally polarizable) nanochannels is reported. Based on the theory of induced charge electrokinetics, a novel nanofluidic system which possesses both adjustable ion selective…

Fluid Dynamics · Physics 2015-07-23 Cunlu Zhao , Chun Yang

We explore the force generation and surface interactions arising when electric fields are applied across fluid films. Using a surface force balance (SFB) we measure directly the force between two electrodes in crossed-cylinder geometry…

Soft Condensed Matter · Physics 2019-04-09 Carla Perez-Martinez , Susan Perkin

Advancements in understanding the lateral migration of particles have helped in enhanced separation in microfluidic devices. In this work, we investigate the effects of electrokinetics on the particle migration in a viscoelastic flow, where…

Soft Condensed Matter · Physics 2020-08-11 Akash Choudhary , Di Li , T. Renganathan , Xiangchun Xuan , S. Pushpavanam

We utilize the self-consistent field theory to explore the mechanical and electrical properties of charged surfaces immersed in polyelectrolyte solutions that could be potentially useful for electrochemical applications. Our research…

Soft Condensed Matter · Physics 2023-08-25 Yu. A. Budkov , N. N. Kalikin

The forces between charged macromolecules, usually given in terms of osmotic pressure, are highly affected by the intervening ionic solution. While in most theoretical studies the solution is treated as a homogeneous structureless…

Soft Condensed Matter · Physics 2014-04-22 Dan Ben-Yaakov , David Andelman , Daniel Harries , Rudi Podgornik

The properties of semidilute polymer solutions are investigated at equilibrium and under shear flow by mesoscale simulations, which combine molecular dynamics simulations and the multiparticle collision dynamics approach. In semidilute…

Soft Condensed Matter · Physics 2015-03-19 Chien-Cheng Huang , Roland G. Winkler , Godehard Sutmann , Gerhard Gompper

The adsorption of highly \textit{oppositely} charged flexible polyelectrolytes onto a charged spherical surface is investigated by means of Monte Carlo simulations in a fashion which resembles the layer-by-layer deposition technique…

Soft Condensed Matter · Physics 2007-05-23 Rene Messina , Christian Holm , Kurt Kremer

We consider the behaviour of a dielectric fluid-fluid interface in the presence of a strong electric field from a point charge and line charge, respectively, both statically and, in the latter case, dynamically. The fluid surface is…

Soft Condensed Matter · Physics 2012-11-08 Simen Å. Ellingsen , Iver Brevik

A new scenario of thermalization process of the adsorbate attached at solid surfaces is proposed. The scenario is based on existence of electric dipole layer in which the electron wavefunctions extend over the positive ions. Thus the strong…

Chemical Physics · Physics 2017-04-26 Paweł Strak , Konrad Sakowski , Stanisław Krukowski

A theoretical model of electromigrative, diffusive and convectivetransport polymer-gel composites is presented. Bulk properties are derived from the standard electrokinetic model with an impenetrable charged sphere embedded in an…

Soft Condensed Matter · Physics 2007-05-23 Reghan J. Hill

We present the results of mesoscopic dissipative particle dynamics (DPD) simulations of coupled electrohydrodynamic phenomena on the micro- and nanoscale. The effects of electroosmotic flow and slippage combined with polyelectrolyte…

Soft Condensed Matter · Physics 2010-07-22 Jens Smiatek , Friederike Schmid

Zeta potentials of several polar protic (water, ethylene glycol, formamide) as well as polar aprotic (dimethyl sulfoxide) liquids were measured in contact with three non-polar surfaces using closed-cell electro-osmosis. The test surfaces…

Chemical Physics · Physics 2014-02-12 Chih-Hsiu Lin , Gregory S. Ferguson , Manoj K. Chaudhury