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In a low-temperature study with a scanning tunneling microscope (STM), the irreducible lateral motion of a CO molecule adsorbed on a Si(001) surface showed a hyperlinear dependence on the tunneling current. This dependence implies that the…

We consider a scanning tunneling microscope (STM) such that tunneling occurs through two atomically sharp protrusions on its tip. When the two protrusions are separated by at least several atomic spacings, the differential conductance of…

Condensed Matter · Physics 2009-10-28 Michael E. Flatte' , Jeff M. Byers

Any evolving system can change of state via thermal mechanisms (hopping a barrier) or via quantum tunneling. Most of the time, efficient classical mechanisms dominate at high temperatures. This is why an increase of the temperature can…

Materials Science · Physics 2014-02-14 M. Minissale , E. Congiu , S. Baouche , H. Chaabouni , A. Moudens , F. Dulieu , M. Accolla , S. Cazaux , G. Manico , V. Pirronello

Indium arsenide nanowires grown by selective-area vapor phase epitaxy are used as tips for scanning tunneling microscopy (STM). The STM tips are realized by positioning the wires manually on the corner of a double cleaved gallium arsenide…

We have used a low-temperature scanning tunneling microscope (STM) to study the surface of heavily doped semiconductor InAs crystals. The crystals are cleaved in situ along the (110) plane. Apart from atomically flat areas, we also observe…

Materials Science · Physics 2007-05-23 A. Depuydt , C. Van Haesendonck , N. S. Maslova , V. I. Panov , V. V. Rakov , S. V. Savinov

Molecular dynamics simulations were performed to study the dependence of migration behaviours of single helium atoms near tungsten surfaces on the surface orientation and temperature. For W{100} and W{110} surfaces, He atoms can quickly…

Materials Science · Physics 2015-12-09 Xiaoshuang Wang , Zhangwen Wu , Qing Hou

Achieving a high intensity in inelastic scanning tunneling spectroscopy (IETS) is important for precise measurements. The intensity of the IETS signal can vary up to a factor three for various tips without an apparent reason accessible by…

Mesoscale and Nanoscale Physics · Physics 2016-04-15 Norio Okabayashi , Alexander Gustafsson , Angelo Peronio , Magnus Paulsson , Toyoko Arai , Franz J. Giessibl

In this work, we studied the adsorption behavior of deposited Si atoms along with their diffusion and other dynamic processes on a Pb monolayer-covered Si(111) surface from 125-230 K using a variable-temperature scanning tunneling…

Mesoscale and Nanoscale Physics · Physics 2017-06-28 Rakesh Kumar , Chuang-Kai Fang , Chih-Hao Lee , Ing-Shouh Hwang

The role of the tip in inelastic electron tunneling spectroscopy (IETS) performed with scanning tunneling microscopes (STM) is theoretically addressed via first-principles simulations of vibrational spectra of single carbon monoxide (CO)…

Mesoscale and Nanoscale Physics · Physics 2011-04-12 Aran Garcia-Lekue , Daniel Sanchez-Portal , Andres Arnau , Thomas Frederiksen

We describe a first principles method to calculate scanning tunneling microscopy (STM) images, and compare the results to well-characterized experiments combining STM with atomic force microscopy (AFM). The theory is based on density…

Mesoscale and Nanoscale Physics · Physics 2018-09-14 Alexander Gustafsson , Norio Okabayashi , Angelo Peronio , Franz J. Giessibl , Magnus Paulsson

An understanding of hydrogen diffusion on metal surfaces is important, not just for its role in heterogeneous catalysis and hydrogen fuel cell technology, but also because it provides model systems where tunneling can be studied under…

Chemical Physics · Physics 2014-04-30 Eliza M. McIntosh , K. Thor Wikfeldt , John Ellis , Angelos Michaelides , William Allison

Single atom/molecule manipulation with a scanning-tunneling-microscope (STM) tip is an innovative experimental technique of nanoscience. Using STM-tip as an engineering or analytical tool, artificial atomic-scale structures can be…

Materials Science · Physics 2015-06-25 Saw-Wai Hla

The control of atomic motion through laser cooling has revolutionized quantum technologies, enabling applications ranging from quantum computing to precision metrology. However, the spatial spreading of subrecoil-laser-cooled atoms --…

Statistical Mechanics · Physics 2025-03-20 Soma Shiraki , Eli Barkai , Takuma Akimoto

The distinction between point and line resolution in transmission electron microscopy (TEM) arises because an ability to image sub-0.2 nm fringes is a necessary, but not a sufficient, condition for imaging individual atoms. In scanned tip…

Instrumentation and Detectors · Physics 2007-05-23 P. Fraundorf , J. Tentschert

We introduce an orbital dependent electron tunneling model and implement it within the atom superposition approach for simulating scanning tunneling microscopy (STM) and spectroscopy (STS). Applying our method, we analyze the convergence…

Materials Science · Physics 2012-12-20 Krisztián Palotás , Gábor Mándi , László Szunyogh

We report the prediction of temperature-dependent diffusion coefficients of interstitial hydrogen, deuterium, and tritium atoms in $\alpha$-Ti using transition state theory. The microscopic parameters in the pre-factor and activation energy…

Materials Science · Physics 2015-06-15 Yong Lu , Ping Zhang

Configuration transitions of individual molecules and atoms on surfaces are traditionally described with energy barriers and attempt rates using an Arrhenius law. This approach yields consistent energy barrier values, but also attempt rates…

Mesoscale and Nanoscale Physics · Physics 2017-03-03 Jeffrey C. Gehrig , Marcos Penedo , Manfred Parschau , Johannes Schwenk , Miguel A. Marioni , Eric W. Hudson , Hans J. Hug

A novel scanning tunneling microscope manipulation scheme for a controlled molecular transport of weakly adsorbed molecules is demonstrated. Single sexiphenyl molecules adsorbed on a Ag(111) surface at 6 K are shot towards single…

Materials Science · Physics 2009-11-10 Saw-Wai Hla , Kai-Felix Braun , Bernhard Wassermann , Karl-Heinz Rieder

We present a low-temperature scanning tunneling spectroscopy study of the Au(111) and of the Cu(111) surface states showing that their binding energy increases when the tip is approached towards the surface. This result, supported by a…

Other Condensed Matter · Physics 2009-11-10 J. Kroeger , L. Limot , H. Jensen , R. Berndt , P. Johansson

We report a novel atom extraction mechanism from the native substrate by means of a scanning tunneling microscope tip-crash on a Ag(111) surface at 5 K. Individual atoms are scattered on the surface when a silver coated tip is dipped into…

Materials Science · Physics 2015-06-24 Saw Wai Hla , Kai-Felix Braun , Violeta Iancu , Aparna Deshpande