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Toroidal vortex is a kind of novel and exotic structured light with potential applications in photonic topology and quantum information. Here, we present the study on high harmonic generation (HHG) from the interaction of the intense…

Optics · Physics 2024-10-10 Zijian Lyu , Yiqi Fang , Yunquan Liu

Real-space picture of electron recollision with the parent ion guides our understanding of the highly nonlinear response of atoms and molecules to intense low-frequency laser fields. It is also among several leading contestants for the…

Optics · Physics 2019-11-06 Mrudul M. S. , Adhip Pattanayak , Misha Ivanov , Gopal Dixit

In this paper we explore the capabilities of MoS2 and WS2 2D monolayers to produce radiation in the terahertz range by generation of high-order harmonics. This phenomenon, which is a result of the non-linear response of the electronic…

Applied Physics · Physics 2024-02-13 Jose Manuel Iglesias , Elena Pascual , Maria J. Martin , Raul Rengel

An important goal in molecular physics and chemistry today is to obtain structure-dependent information about molecular function to obtain a deeper understanding into chemical reactions. However, until now, asymmetric tops, which comprise…

We formulate the concept of dominant interaction Hamiltonians to obtain an integrable approximation to the dynamics of an electron exposed to a strong laser field and an atomic potential leading to high harmonic generation. The concept…

Atomic Physics · Physics 2012-01-20 Carlos Zagoya , Christoph-Marian Goletz , Frank Grossmann , Jan M. Rost

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

Atomic Physics · Physics 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

High-harmonic generation is typically thought of as a sub-laser-cycle process, with the electron's excursion in the continuum lasting a fraction of the optical cycle. However, it was recently suggested that long-lived Rydberg states can…

We report theoretical investigations of the tomographic procedure suggested by Itatani {\it et al.} [Nature, {\bf 432} 867 (2004)] for reconstructing highest occupied molecular orbitals (HOMO) using high-order harmonic generation (HHG).…

Atomic Physics · Physics 2009-10-30 Van-Hoang Le , Anh-Thu Le , Rui-Hua Xie , C. D. Lin

Attosecond dynamics in strong-field tunnel ionization are encoded in intricate holographic patterns in the photoelectron momentum distributions (PMDs). These patterns show the interference between two or more superposed quantum electron…

The interaction of a helium atom with intense short 800 nm laser pulse is studied theoretically beyond the single-active-electron approximation. For this purpose, the time-dependent Schr\"odinger equation for the two-electron wave packet…

Atomic and Molecular Clusters · Physics 2017-03-08 Anton N. Artemyev , Lorenz S. Cederbaum , Philipp V. Demekhin

Several correlation and interference effects in strong-field physics are investigated. We show that the interference of continuum wave packets can be the dominant mechanism of high-harmonic generation (HHG) in the over-the-barrier regime.…

A usual assumption in the so-called {\it de Broglie - Bohm} approach to quantum dynamics is that the quantum trajectories subject to typical `guiding' wavefunctions turn to be quite irregular, i.e. {\it chaotic} (in the dynamical systems'…

Quantum Physics · Physics 2015-06-04 G. Contopoulos , N. Delis , C. Efthymiopoulos

High harmonic emissions from crystalline solids contain rich information on the dynamics of electrons driven by intense infrared laser fields and have been intensively studied owing to their potential use as a probe of microscopic…

Materials Science · Physics 2023-05-01 K. Uchida , K. Tanaka

The electrical conductance of molecular junctions may strongly depend on the temperature, and weakly on molecular length, under two distinct mechanisms: phase-coherent resonant conduction, with charges proceeding via delocalized molecular…

Mesoscale and Nanoscale Physics · Physics 2017-12-25 Hyehwang Kim , Dvira Segal

We develop a computational method for evaluating the damping of vibrational modes in mono-atomic metallic chains suspended between bulk crystals under external strain. The damping is due to the coupling between the chain and contact modes…

Mesoscale and Nanoscale Physics · Physics 2009-07-31 Mads Engelund , Mads Brandbyge , Antti-Pekka Jauho

We present a theoretical investigation into the two-center interference in aligned H$_2^+$. The influence of the laser field on the recombination step is investigated by comparing laser-induced harmonic generation with harmonic generation…

Atomic Physics · Physics 2015-05-19 Elmar V. van der Zwan , Manfred Lein

Nonadiabatic dynamics around an avoid crossing or a conical intersection play a crucial role in the photoinduced processes of most polyatomic molecules. The present work shows that the topological phase in conical intersection makes the…

Optics · Physics 2022-11-01 Guanglu Yuan , Ruifeng Lu , Shicheng Jiang , Konstantin Dorfman

The composite character of two-fermion bosons manifests itself in the interference of many composites as a deviation from the ideal bosonic behavior. A state of many composite bosons can be represented as a superposition of different…

Quantum Physics · Physics 2013-01-03 Malte C. Tichy , Peter Alexander Bouvrie , Klaus Mølmer

We illustrate that a Hermitian nonlinear optical system consisting of hybridized parametric amplification and second harmonic generation mimics non-Hermitian evolution dynamics. Oscillation damping, evolution to a static steady state, and…

Optics · Physics 2021-01-05 Noah Flemens , Nicolas Swenson , Jeffrey Moses

We investigate the possibility of characterizing the different thermalization pathways through a large-deviation approach. Specifically, we consider clean, disordered and quasi-periodic harmonic chains under energy and momentum-conserving…

Statistical Mechanics · Physics 2024-08-21 Stefano Lepri