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The emission of above-ionization-threshold harmonics results from the recombination of two electron wavepackets moving along a "short" and a "long" trajectory in the atomic continuum. Attosecond pulse train generation has so far been…

Optics · Physics 2015-05-19 J. E. Kruse , P. Tzallas , E. Skantzakis , D. Charalambidis

The increasing penetration of renewable energy sources, characterised by low inertia and intermittent disturbances, presents substantial challenges to power system stability. As critical indicators of system stability, frequency dynamics…

Systems and Control · Electrical Eng. & Systems 2025-02-19 Xiao Li , Xinyi Wen , Benjamin Schäfer

A model Hamiltonian for the reaction CH$_4^+ \rightarrow$ CH$_3^+$ + H, parametrized to exhibit either early or late inner transition states, is employed to investigate the dynamical characteristics of the roaming mechanism. Tight/loose…

Chemical Physics · Physics 2015-06-18 F. A. L. Mauguière , P. Collins , G. S. Ezra , S. C. Farantos , S. Wiggins

In present paper we develop an analytic theory for the harmonic generation of symmetric diatomic molecular ions beyond two-level model, emphasizing the influence of charge-resonance (CR) states those are strongly coupled to electromagnetic…

Atomic Physics · Physics 2009-11-13 Yanjun Chen , Jing Chen , Jie Liu

High-order harmonic generation (HHG) is combined with resonant x-ray excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process. To describe this setting, I develop a…

Atomic Physics · Physics 2015-10-15 Christian Buth

A theoretical optimization method of high-harmonic-generation (HHG) is developed in the framework of optimal-control-theory (OCT). The target of optimization is the emission radiation of a particular frequency. The OCT formulation includes…

Quantum Physics · Physics 2020-02-19 Ido Schaefer , Ronnie Kosloff

The higher order harmonic generation process in the nonperturbative regime at the interaction of coherent electromagnetic radiation with the AB-stacked bilayer graphene at high Fermi energies is considered. The applied coherent…

Mesoscale and Nanoscale Physics · Physics 2020-07-20 A. G. Ghazaryan , H. H. Matevosyan , Kh. V. Sedrakian

Path integral derivations are presented for two recently developed complex trajectory techniques for the propagation of wave packets, Complex WKB and BOMCA. Complex WKB is derived using a standard saddle point approximation of the path…

Quantum Physics · Physics 2013-05-29 Jeremy Schiff , Yair Goldfarb , David J. Tannor

Fragmentation of highly charged molecular ions or clusters consisting of more than two atoms can proceed in an onestep synchronous manner where all bonds break simultaneously or sequentially by emitting one ion after the other. We separated…

We consider optical high harmonic generation in a hydrogen atom confined in a breathing spherical box by considering atomic nucleus as fixed at the center of sphere. In such spherically symmetric, dynamical trap, the high harmonic…

Quantum Physics · Physics 2019-02-19 S. Rakhmanov , D. Matrasulov , B. Eshchanov , V. I. Matveev

The PhD thesis is devoted to the study of second harmonic generation of narrow beams in photonic crystals. The basic idea is that if both frequencies, the fundamental and second harmonics are in the region of self-collimation, then the…

Optics · Physics 2013-11-06 Cristian Nistor

Quantum interference (QI) in molecular transport junctions can lead to dramatic reductions of the electron transmission at certain energies. In a recent work [Markussen et al., Nano Lett. 2010, 10, 4260] we showed how the presence of such…

Mesoscale and Nanoscale Physics · Physics 2017-09-13 Troels Markussen , Robert Stadler , Kristian S. Thygesen

We theoretically investigate the interference effect of high-order harmonics generated from molecules at different alignment angles. It is shown that the interference of the harmonic emissions from molecules aligned at different angles can…

Optics · Physics 2015-02-27 Meiyan Qin , Xiaosong Zhu , Yang Li , Qingbin Zhang , Pengfei Lan , Peixiang Lu

We present a complete theory of bicircular high-order-harmonic emission from N-fold rotationally symmetric molecules. Using a rotating frame of reference we predict the complete structure of the high-order-harmonic spectra for arbitrary…

Atomic Physics · Physics 2016-09-26 Daniel M. Reich , Lars Bojer Madsen

We demonstrate and explore an all-optical technique for direct monitoring the orientation dynamics of gas phase molecular ensembles. The technique termed 'MOISH' utilizes the transiently lifted inversion symmetry of polar gas media and…

Chemical Physics · Physics 2022-10-12 Amit Beer , Ran Damari , Yun Chen , Sharly Fleischer

For the high-order harmonic generation in solids, we find a distinct and clean interference pattern in the high-energy end of the spectrum which can be interpreted as a Michelson interferometer of the Bloch electron. Our results are…

Hong-Ou-Mandel (HOM) interference unveils a distinct behavior of identical particles which cannot be distinguished from each other. Especially for bosons, two separated identical particles passing through a beamsplitter always go together…

Here is presented an original program based on molecular Schrodinger equations. It is dedicated to target specific states of infrared vibrational spectrum in a very precise way with a minimal usage of memory. An eigensolver combined with a…

Computational Physics · Physics 2018-07-26 Romain Garnier

A quantum optical model for the high-order harmonic generation is presented, in which both the exciting field and the high harmonic modes are quantized, while the target material appears via parameters only. As a consequence, the model is…

Based upon our previous works (Eur.Phys.J.D 6, 319(1999); Chin.Phys.Lett. 18, 236(2001)), we develop a classical approach to calculate the high-order harmonic generation of the laser driven atoms and molecules. The Coulomb singularities in…

Atomic Physics · Physics 2007-05-23 Chaohong Lee , Yiwu Duan , Wing-Ki Liu , Jian-Min Yuan , Lei Shi , Xiwen Zhu , Kelin Gao
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