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We study full counting statistics for classical heat transport through anharmonic/nonlinear molecular junctions formed by interacting oscillators. Analytical result of the steady state heat flux for an overdamped anharmonic junction with…

Statistical Mechanics · Physics 2013-03-13 Sha Liu , Bjiay Kumar Agarwalla , Jian-Sheng Wang , Baowen Li

Electronic current flowing in a molecular electronic junction dissipates significant amounts of energy to vibrational degrees of freedom, straining and rupturing chemical bonds and often quickly destroying the integrity of the molecular…

Mesoscale and Nanoscale Physics · Physics 2020-09-25 Riley J. Preston , Thomas D. Honeychurch , Daniel S. Kosov

Thermal transport through nanosystems is central to numerous processes in chemistry, material sciences, electrical and mechanical engineering, with classical molecular dynamics as the key simulation tool. Here we focus on thermal junctions…

Mesoscale and Nanoscale Physics · Physics 2020-08-31 Na'im Kalantar , Bijay Kumar Agarwalla , Dvira Segal

Controlling the direction and magnitude of both heat and electronic currents using rectifiers has significant implications for the advancement of molecular circuit design. In order to facilitate the implementation of new transport phenomena…

Mesoscale and Nanoscale Physics · Physics 2019-08-02 Galen T. Craven , Dahai He , Abraham Nitzan

Thermopower measurements of molecular junctions have recently gained interest as a characterization technique that supplements the more traditional conductance measurements. Here we investigate the electronic conductance and thermopower of…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 Troels Markussen , Chengjun Jin , Kristian S. Thygesen

We investigate the Joule expansion of an interacting quantum gas in an energy eigenstate. The Joule expansion occurs when two subsystems of different particle density are allowed to exchange particles. We demonstrate numerically that the…

Statistical Mechanics · Physics 2019-08-07 Jae Dong Noh , Eiki Iyoda , Takahiro Sagawa

We discuss inherent thermometry in a Superconductor - Normal metal - Superconductor tunnel junction. In this configuration, the energy selectivity of single-particle tunneling can provide a significant electron cooling, depending on the…

Superconductivity · Physics 2009-11-13 Hervé Courtois , Sukumar Rajauria , Philippe Gandit , Frank Hekking , Bernard Pannetier

We investigate the particle and heat transport in quantum junctions with the geometry of star graphs. The system is in a nonequilibrium steady state, characterized by the different temperatures and chemical potentials of the heat reservoirs…

Statistical Mechanics · Physics 2017-10-13 Mihail Mintchev , Luca Santoni , Paul Sorba

The thermopower of a Kondo-correlated gate-defined quantum dot is studied using a current heating technique. In the presence of spin correlations the thermopower shows a clear deviation from the semiclassical Mott relation between…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 R. Scheibner , H. Buhmann , D. Reuter , M. N. Kiselev , L. W. Molenkamp

We follow the nonequilibrium Green's function formalism to study time-dependent thermal transport in a linear chain system consisting of two semi-infinite leads connected together by a coupling that is harmonically modulated in time. The…

Mesoscale and Nanoscale Physics · Physics 2010-08-18 Eduardo C. Cuansing , Jian-Sheng Wang

Joule heating is a non-equilibrium dissipative process that occurs in a normal metal when an electric current flows, in an amount proportional to the metal's resistance. When it is induced by eddy currents resulting from a change in…

Superconductivity · Physics 2020-09-18 J. E. Hirsch

Thermal conductance of single molecular junctions at room temperature has been measured recently using picowatt-resolution scanning probes. However, fully understanding thermal transport in a much wider temperature range is needed for the…

Mesoscale and Nanoscale Physics · Physics 2022-02-15 Gen Li , Bing-Zhong Hu , Nuo Yang , Jing-Tao Lü

The interaction between electronic and nuclear degrees of freedom in single-molecule junctions is an essential mechanism, which may result in the current-induced rupture of chemical bonds. As such, it is fundamental for the stability of…

Mesoscale and Nanoscale Physics · Physics 2020-11-25 André Erpenbeck , Yaling Ke , Uri Peskin , Michael Thoss

Molecular electronics offers unique scientific and technological possibilities, resulting from both the nanometre scale of the devices and their reproducible chemical complexity. Two fundamental yet different effects, with no classical…

Mesoscale and Nanoscale Physics · Physics 2017-05-12 Andrew K. Mitchell , Kim G. L. Pedersen , Per Hedegaard , Jens Paaske

An integrated piecewise thermal equilibrium approach based on the first-principles calculation method has been developed to calculate bias dependent electronic structures and current- and differential conductance-voltage characteristics of…

Other Condensed Matter · Physics 2009-11-13 M. -H. Tsai , T. -H. Lu , Y. -H. Tang

In molecular devices electronic degrees of freedom are coupled to vibrational modes of the molecule, offering an opportunity to study fundamental aspects of this coupling between at the nanoscale. To this end we consider the nonequilibrium…

Strongly Correlated Electrons · Physics 2014-01-29 Yuval Vinkler-Aviv , Avraham Schiller , Natan Andrei

Vibrationally inelastic electron transport through a flexible molecular junction is investigated. The study is based on a mechanistic model for a biphenyl molecule between two metal electrodes. Employing methods from electron-molecule…

Mesoscale and Nanoscale Physics · Physics 2023-07-26 Martin Cizek , Michael Thoss , Wolfgang Domcke

Boiling heat transfer is the basis of many commonly used cooling techniques. In cooling of electronic devices, for example, it is desirable to further miniaturize heat exchangers to achieve higher heat transfer, and thus it is necessary to…

Fluid Dynamics · Physics 2023-08-25 Soumyadeep Paul , Yusuke Ito , Wei-Lun Hsu , Hirofumi Daiguji

The electrical conductance of molecular junctions may strongly depend on the temperature, and weakly on molecular length, under two distinct mechanisms: phase-coherent resonant conduction, with charges proceeding via delocalized molecular…

Mesoscale and Nanoscale Physics · Physics 2017-12-25 Hyehwang Kim , Dvira Segal

We investigate the thermopower of single molecules weakly coupled to metallic leads. We model the molecule in terms of the relevant electronic orbitals coupled to phonons corresponding to both internal vibrations and to oscillations of the…

Mesoscale and Nanoscale Physics · Physics 2009-09-29 Jens Koch , Felix von Oppen , Yuval Oreg , Eran Sela
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