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We numerically investigate the thermoelectric properties of a triangle quantum dot connected to metallic electrodes using the non-equilibrium Green's function method in the Anderson model. Exploiting the equation of motion method in the…

Mesoscale and Nanoscale Physics · Physics 2022-06-08 Ahmad Ahmadi Fouladi , Javad Vahedi

We investigate the heat conduction properties of molecular junctions comprising anharmonic interactions. We find that nonlinear interactions can lead to novel phenomena: it negative differential thermal conductance and heat rectification.…

Soft Condensed Matter · Physics 2009-11-11 Dvira Segal

We propose a possible route to achieve high thermoelectric efficiency in molecular junctions by combining a local chemical tuning of the molecular electronic states with the use of semiconducting electrodes. The former allows to control the…

Materials Science · Physics 2009-08-05 D. Nozaki , H. Sevinçli , W. Li , R. Gutierrez , G. Cuniberti

Understanding heating and cooling mechanisms in mesoscopic superconductor-semiconductor hybrid devices is crucial for their application in quantum technologies. Owing to the poor thermal conductivity of typical devices, heating effects can…

Mesoscale and Nanoscale Physics · Physics 2024-06-12 Angel Ibabe , Gorm O. Steffensen , Ignacio Casal , Mario Gomez , Thomas Kanne , Jesper Nygard , Alfredo Levy Yeyati , Eduardo J. H. Lee

We investigate the power dissipated by an electronic current flowing through a quantum point contact in a two-dimensional electron gas. Based on the Landauer-B\"uttiker approach to quantum transport, we evaluate the power that is dissipated…

Mesoscale and Nanoscale Physics · Physics 2022-03-30 Carmen Blaas-Anselmi , Félix Helluin , Rodolfo A. Jalabert , Guillaume Weick , Dietmar Weinmann

We report a theoretical study of the thermopower of single-molecule junctions, with focus on phenyl-based molecular junctions. In contrast to prior studies, thermal fluctuations of the torsional angle between the phenyl rings and variations…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 Yonatan Dubi

We investigate the problem of heat conduction across a molecular junction connecting two nanoparticles, both in vacuum and in a liquid environment, using classical molecular dynamics simulations. In vacuum, the well-known result of a length…

Materials Science · Physics 2011-11-04 Samy Merabia , Jean-Louis Barrat , Laurent J. Lewis

We consider several fundamental optical phenomena involving single molecules in biased metal-molecule-metal junctions. The molecule is represented by its highest occupied and lowest unoccupied molecular orbitals, and the analysis involves…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael Galperin , Abraham Nitzan

We report a method using scanning tunnelling microscope single molecular break junction to simultaneously measure and correlate the single-molecule thermopower and electrical conductance. In contrast to previously reported approaches, it…

Mesoscale and Nanoscale Physics · Physics 2021-09-24 Joseph M. Hamill , Christopher Weaver , Tim Albrecht

Understanding energy transport at the nanoscale is an open and fundamental challenge in the molecular sciences with direct implications for the design of new electronics, computing devices, and materials. While nanoscale energy transport…

Mesoscale and Nanoscale Physics · Physics 2025-10-15 Renai Chen , Galen T. Craven

We present a consistent theory of energy balance and conversion in a single-molecule junction with strong interactions between electrons on the molecular linker (dot) and phonons in the nuclear environment where the Marcus-type electron…

Mesoscale and Nanoscale Physics · Physics 2020-01-22 Natalya A. Zimbovskaya , Abraham Nitzan

We develop a general theory for thermal transport in anharmonic systems under the weak system-bath coupling approximation similar to the quantum master equation formalism. A current operator is derived, which is valid not only in the steady…

Mesoscale and Nanoscale Physics · Physics 2012-05-28 Juzar Thingna , J. L. García-Palacios , Jian-Sheng Wang

We analyze the heat current flowing across interacting quantum dots within the Coulomb blockade regime. Power can be generated by either voltage or temperature biases. In the former case, we find nonlinear contributions to the Peltier…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 Miguel A. Sierra , David Sanchez

We study heating and heat dissipation of a single \c60 molecule in the junction of a scanning tunneling microscope (STM) by measuring the electron current required to thermally decompose the fullerene cage. The power for decomposition…

Heating and heat conduction in molecular junctions are considered within a general NEGF formalism. We obtain a unified description of heating in current carrying molecular junctions as well as the electron and phonon contributions to the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael Galperin , Mark A. Ratner , Abraham Nitzan

We present an original method to estimate the conductivity of a single molecule anchored to nanometric-sized metallic electrodes, using a Mechanically Controlled Break Junction (MCBJ) operated at room temperature in liquid. We record the…

Mesoscale and Nanoscale Physics · Physics 2018-03-16 M. Gil , T. Malinowski , M. Iazykov , H. Klein

The thermoelectric transport through a molecular bridge is discussed, with an emphasis on the effects of inelastic processes of the transport electrons caused by the coupling to the vibrational modes of the molecule. In particular it is…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 O. Entin-Wohlman , Y. Imry , A. Aharony

To investigate the initial process of Joule heating in semiconductors microscopically and quantitatively, we developed a theoretical framework for the ab initio evaluation of the carrier energy relaxation in semiconductors under a high…

Materials Science · Physics 2021-08-25 Emi Minamitani

We discuss heat transport through a Josephson tunnel junction under various bias conditions. We first derive the formula for the cooling power of the junction valid for arbitrary time dependence of the Josephson phase. Combining it with the…

Mesoscale and Nanoscale Physics · Physics 2013-04-04 Dmitry Golubev , Timothé Faivre , Jukka P. Pekola

A first-principles approach is presented for the thermoelectricity in molecular junctions formed by a single molecule contact. The study investigates the Seebeck coefficient considering the source-drain electrodes with distinct temperatures…

Mesoscale and Nanoscale Physics · Physics 2009-05-07 Yu-Shen Liu , Yu-Chang Chen