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We present a basic framework for modeling collective mode effects in photocurrent measurements performed on two-dimensional materials using nano-optical scanned probes. We consider photothermal, photovoltaic, and bolometric contributions to…

Mesoscale and Nanoscale Physics · Physics 2023-12-04 A. Rikhter , D. N. Basov , M. M. Fogler

The effect of the local fields on the absorption spectra of silicon nanoclusters (NCs), freestanding or embedded in SiO2, is investigated in the DFT-RPA framework for different size and amorphization of the samples. We show that local field…

Mesoscale and Nanoscale Physics · Physics 2012-05-03 Roberto Guerra , Margherita Marsili , Olivia Pulci , Stefano Ossicini

We investigated the nucleation process at the molecular level. Controlled sticking of individual atoms onto mass selected clusters over a wide mass range has been carried out for the first time. We measured the absolute unimolecular…

Atomic and Molecular Clusters · Physics 2007-11-13 Fabien Chirot , Pierre Labastie , Sébastien Zamith , Jean-Marc L'Hermite

We present a simple model of collective plasmons in a dimerized chain of spherical metallic nanoparticles, an elementary example of a topologically nontrivial nanoplasmonic system. Taking into account long-range quasistatic dipolar…

Mesoscale and Nanoscale Physics · Physics 2018-10-23 Charles A. Downing , Guillaume Weick

Cryogenic cluster beam experiments have provided crucial insights into the evolution of the metallic state from the atom to the bulk. Surprisingly, one of the most fundamental metallic properties, the ability of a metal to efficiently…

Atomic and Molecular Clusters · Physics 2011-01-26 John Bowlan , Anthony Liang , Walt A. de Heer

A cluster consisting of many atoms or molecules may be considered, in some circustances, to be a single large molecule with a well defined polarizability. Once the polarizability of such a cluster is known, one can evaluate certain…

Materials Science · Physics 2009-11-11 Hye-Young Kim , Jorge O. Sofo , Darrell Velegol , Milton W. Cole , Gautam Mukhopadhyay

Skyrmions are topological defects belonging to nontrivial homotopy classes in particle theory. Their remarkably stable topology has recently been observed in electromagnetic waves. For the evanescent fields near a surface, this has been…

The temperature increase and temperature gradients induced by mid-infrared laser illumination of vertical gold nanoantenna arrays embedded into polymer layers was measured directly with a photothermal expansion nanoscope. Nanoscale thermal…

Gold nanoclusters are grown by 1.8 MeV Au^\sup{2+} implantation on c-Al\sub{2}O\sub{3}(0001)substrate and subsequent air annealing at temperatures 1273K. Post-annealed samples show plasmon resonance in the optical (561-579 nm) region for…

We report on the nanoparticle-size-dependent onset of quantum tunneling of electrons across the sub-nanometer gaps in three different sizes (30, 50, and 80 nm) of highly uniform gold nanosphere dimers. For precision plasmonics, the gap…

We use excited-state quantum chemistry techniques to investigate the intraband absorption of doped semiconductor nanoparticles as a function of doping density, nanoparticle radius, and material properties. The excess electrons are modeled…

Mesoscale and Nanoscale Physics · Physics 2019-07-29 Bryan T. G. Lau , Timothy C. Berkelbach

Plasmonic nanoantennas have proven to be efficient transducers of electromagnetic to mechanical energy and vice versa. The sudden thermal expansion of these structures after an ultrafast optical pulsed excitation leads to the emission of…

In experiments where ultraviolet light produces aerosols from trace amounts of ozone, sulphur dioxide, and water vapour, the number of additional small particles produced by ionization by gamma sources all grow up to diameters larger than…

Atomic and Molecular Clusters · Physics 2015-06-04 Henrik Svensmark , Martin B. Enghoff , Jens Olaf Pepke Pedersen

We have studied the structure and properties of potassium clusters containing even number of atoms ranging from 2 to 20 at the ab initio level. The geometry optimization calculations are performed using all-electron density functional…

Atomic and Molecular Clusters · Physics 2016-09-28 Arup Banerjee , Tapan K. Ghanty , Aparna Chakrabarti

The development of nanoplasmonic devices, such as plasmonic circuits and metamaterial superlenses in the visible to ultraviolet frequency range, is hampered by the lack of low-loss plasmonic media. Recently, strong plasmonic response was…

Plasmonic response in metals, defined as the ability to support subwavelength confinement of surface plasmon modes, is typically limited to a narrow frequency range below the metals' plasma frequency. This places severe limitations on the…

The lifetime of localized surface plasmon plays an important role in many aspects of plasmonics and its applications. In small metal nanostructures, the dominant mechanism restricting plasmon lifetime is size-dependent Landau damping. We…

Mesoscale and Nanoscale Physics · Physics 2016-10-18 A. S. Kirakosyan , M. I. Stockman , T. V. Shahbazyan

The flexibility and versatility of nanoassembled plasmonic structures provide platforms for mesoscale tunable optical modulation. Our recently developed model for these nanoassembled plasmonic structures is composed of a dielectric…

Optics · Physics 2024-12-31 Md. Imran Khan , Sayantani Ghosh , Arnold D. Kim

The local field approach and kinetic equation method is applied to calculate the surface plasmon radiative damping in a spheroidal metal nanoparticle embedded in any dielectric media. The radiative damping of the surface plasmon resonance…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 Nicolas I. Grigorchuk

Multilayer assemblies of metal nanoparticles can act as photonic structures, where collective plasmon resonances hybridize with cavity modes to create plasmon-polariton states. For sufficiently strong coupling, plasmon polaritons…