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It is a generally accepted idea that the particle size distribution strongly affects the optical spectra of colloidal plasmonic nanoparticles. It is often quoted as one of the main reasons while explaining the mismatch between the…

Optics · Physics 2022-02-14 Rituraj Borah , Sammy W. Verbruggen

We have performed large-scale Lennard-Jones molecular dynamics simulations of homogeneous vapor-to-liquid nucleation, with $10^9$ atoms. This large number allows us to resolve extremely low nucleation rates, and also provides excellent…

Chemical Physics · Physics 2014-04-07 Raymond Angélil , Jürg Diemand , Kyoko K. Tanaka , Hidekazu Tanaka

The localized surface plasmon resonance of metallic nanostructures produces strongly localized and enhanced near-field light, significantly contributing to nanophotonics research and applications. Plasmon nanofocusing represents another…

Polymer materials with low water uptake exhibit a highly heterogeneous interior, characterized by water clusters in the form of nanodroplets and nanochannels. Here, based on our recent insights from computer simulations, we argue that water…

Soft Condensed Matter · Physics 2022-06-16 Matej Kanduč , Rafael Roa , Won Kyu Kim , Joachim Dzubiella

The thermodynamics and kinetics of crystallization of nanoparticles, as opposed to bulk phases, may be influenced by surface and size effects. We investigate the importance of such factors in the crystallization process of gold, silver, and…

Statistical Mechanics · Physics 2024-07-09 Arthur France-Lanord , Sarath Menon , Julien Lam

We present an ab-initio study of the hybridization of localized surface plasmons in a metal nanoparticle dimer. The atomic structure, which is often neglected in theoretical studies of quantum nanoplasmonics, has a strong impact on the…

This paper provides new insights concerning the simulation of plasmon driven chemical reactions using real-time TDDFT based on the tight-binding electronic structure code DFTB+, with applications to the dissociation of H$_2$ on octahedral…

Chemical Physics · Physics 2023-03-21 Sajal Kumar Giri , George C. Schatz

A major challenge for plasmonics as an enabling technology for quantum information processing is the realization of active spatio-temporal control of light on the nanoscale. The use of phase-shaped pulses or beams enforces specific…

Optics · Physics 2015-06-03 Svetlana V. Boriskina , Bjoern M. Reinhard

The ability to engineer localized surface plasmon resonances at large scale usually relies on precise nanoscale patterning. Here, we demonstrate that mid-infrared plasmonic responses can instead emerge in unpatterned polysilicon films…

Understanding the dynamics of the micro-sized surface bubbles produced by plasmonic heating can benefit a wide range of applications like microfluidics, catalysis, micro-patterning and photo-thermal energy conversion. Usually, surface…

Fluid Dynamics · Physics 2022-01-19 Qiushi Zhang

Owing to their ability to concentrate light on nanometer scales, plasmonic surface structures are ideally suited for on-chip functionalization with nonlinear or gain materials. However, achieving a high effective quantum yield across a…

Surface plasmons on metals can concentrate light into sub-nanometric volumes and on these near atomic length scales the electronic response at the metal interface is smeared out over a Thomas-Fermi screening length. This nonlocality is a…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Yu Luo , A. I. Fernandez-Dominguez , Aeneas Wiener , S. A. Maier , J. B. Pendry

The random-phase-approximation semiclassical scheme for description of plasmon excitations in large metallic nanospheres (with radius 10--100 nm) is developed for a case of presence of dynamical electric field. The spectrum of plasmons in…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 W. Jacak , J. Krasnyj , J. Jacak , A. Chepok , L. Jacak , W. Donderowicz , D. Z. Hu , D. M. Schaadt

We study the plasmonic properties of coupled noble-metal nanochains in the case of different number of coupled chains and doping by different transition-metal (TM) atoms within the time-dependent density-functional theory (TDDFT) approach.…

Mesoscale and Nanoscale Physics · Physics 2014-09-12 Neha Nayyar , Volodymyr Turkowski , Talat S. Rahman

Nanoplasmonics exploits the coupling between light and collective electron density oscillations (plasmons) to bypass the stringent limits imposed by diffraction. This coupling enables confinement of light to sub-wavelength volumes and is…

We present an analysis of the temperature dependence of the optical response of small sodium clusters in a temperature range bracketing the melting phase transition. When the temperature increases, the mean excitation energy undergoes a red…

chem-ph · Physics 2009-10-28 Aurel Bulgac , Caio Lewenkopf

The elastic response of suspended NbSe3 nanowires is studied across the charge density wave phase transition. The nanoscale dimensions of the resonator lead to a large resonant frequency (10-100 MHz), bringing the excited phonon frequency…

We have studied the plasmonic properties of aperiodic arrays of identical nanoparticles (NPs) formed by two opposite and equal graded-chains (a chain where interactions change gradually). We found that these arrays concentrate the external…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 Natalia Esteves-López , Horacio M. Pastawski , Raúl A. Bustos-Marún

The temporal modulation of material parameters enables optical amplification within linear media. Here we consider the fundamental building block of plasmonics, a subwavelength metal nanoparticle, and study how temporal modulation alters…

Mesoscale and Nanoscale Physics · Physics 2025-08-29 Miguel Verde , Paloma A. Huidobro

Plasmon modes of a two-dimensional lattice of long conducting circular wires are investigated by using an embedding technique to solve Maxwell's equations rigorously. The frequency-dependent density of states is calculated for various…

Materials Science · Physics 2007-05-23 J. M. Pitarke , J. E. Inglesfield , N. Giannakis