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We study time-delays in atomic multiphoton ionization (MPI) using the phase-sensitive detection of photoelectron vortices. Photoelectron vortices are created by MPI with counter-rotating circularly polarized (CRCP) ultrashort double pulse…
An isolated attosecond vortex $\gamma$-ray pulse is generated by using a relativistic spatiotemporal optical vortex (STOV) laser in particle-in-cell simulations. A $\sim$ 300-attosecond electron slice with transverse orbital angular…
For tracing the spatiotemporal evolution of electronic systems, we suggest and analyze theoretically a setup that exploits the excellent spatial resolution based on scanning tunneling microscopy techniques combined with the temporal…
Field-emission of electrons underlies major advances in science and technology, ranging from imaging the atomic-scale structure of matter to signal processing at ever-higher frequencies. The advancement of these applications to their…
Interaction of a strong laser pulse with matter transfers not only energy but also linear momentum of the photons. Recent experimental advances have made it possible to detect the small amount of linear momentum delivered to the…
Measuring the time it takes to remove an electron from an atom or molecule during photoionization using newly developed attosecond spectroscopies has been a focus of many recent experiments. However, the outcome of such measurement depends…
Attosecond observations of coherent electron dynamics in molecules and nanostructures can be achieved by combining conventional scanning tunneling microscopy (STM) with ultrashort femtosecond laser pulses. While experimental studies in the…
First time-resolved photoemission experiments employing attosecond streaking of electrons emitted by an XUV pump pulse and probed by a few-cycle NIR pulse found a time delay of about 100 attoseconds between photoelectrons from the…
Transient grating spectroscopy has become a mainstay among metal and semiconductor characterization techniques. Here we extend the technique towards the shortest achievable timescales by using tabletop high-harmonic generation of attosecond…
Modern intense ultrafast pulsed lasers generate an electric field of sufficient strength to permit tunnel ionization of the valence electrons in atoms. This process is usually treated as a rapid succession of isolated events, in which the…
Measuring and controlling the ionization dynamics by intense laser fields has recently led to important breakthroughs, from the investigation of tunneling time delays to attosecond molecular imaging by electron holography. In these…
We illustrate how attosecond light pulses can be used to directly mapping out the time-dependence of the correlated motion of two excited atomic electrons, discuss how the two-electron correlations manifest themselves in realistic…
Strong field ionization provides a unique mean to address complex dynamics of an electron in competing Coulomb and laser fields. Recent streak camera experiment (K\"ubel, et al., Phys. Rev. Lett. 119, 183201) analyzed asymmetries in the…
Multi-electron dynamics in atoms and molecules very often occur on sub- to few-femtosecond timescales. The available intensities of extreme-ultraviolet (XUV) attosecond pulses have previously only allowed the time-resolved investigation of…
In this work, we study the coherent dynamics of an atomic Zeeman wave packet using a continuous pump--probe scheme. A polarized wave packet is generated via few-photon excitation by a femtosecond laser pulse, creating a state with a…
We present an innovative beamline for extreme ultraviolet (XUV)-infrared (IR) pump-probe reflection spectroscopy in solids with attosecond temporal resolution. The setup uses an actively stabilized interferometer, where attosecond pulse…
Photoionization from energetically distinct electronic states may have a relative time delay of tens of attoseconds. Here we demonstrate that pulses of optical vortices allow measuring such attoseconds delays from magnetic sublevels, even…
We present a theory of time-resolved photoionisation in the presence of a vortex beam. In a pump-probe setup, an extreme ultraviolet or an x-ray pump pulse triggers ionization, which is probed by a synchronized infrared pulse with non-zero…
We propose a new scenario to apply IR-pump-XUV-probe schemes to resolving strong field ionization induced and attosecond pulse driven electron-hole dynamics and coherence in real time. The coherent driving of both the infrared laser and the…
The recent development of Homochromatic Attosecond Streaking (HAS) has enabled a novel, highly precise method for ultrafast metrology of attosecond electron pulses as well as for real-time sampling of the instantaneous field waveforms of…