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The evolution of electron wavepackets determines the course of many physical and chemical phenomena and attosecond spectroscopy aims to measure and control such dynamics in real-time. Here, we investigate radial electron wavepacket motion…

Atomic Physics · Physics 2015-09-04 Niranjan Shivaram , Xiao-Min Tong , Henry Timmers , Arvinder Sandhu

Ionization of an atom or molecule presents surprising richness beyond our current understanding: strong-field ionization with low-frequency fields recently revealed unexpected kinetic energy structures (1, 2). A solid grasp on electron…

Attosecond transient absorption spectroscopy has thus far been lacking the capability to simultaneously characterize the intense laser pulses at work within a time-resolved quantum-dynamics experiment. However, precise knowledge of these…

We demonstrate a novel method to measure the temporal evolution of electric fields with optical frequencies. Our technique is based on the detection of transient currents in air plasma. These directional currents result from sub-cycle…

Resonance-enhanced multiphoton ionization (REMPI) in potassium atom is investigated within the strong coupling regime using photoelectron momentum imaging techniques. The kinetic energy distribution of the ionized electrons reveals the…

Atomic Physics · Physics 2025-03-10 Wankai Li , Yixuan Wang , Xing Li , Tao Yang , Dongdong Zhang , Dajun Ding

We introduce and experimentally demonstrate a method, where the two intrinsic time scales of a molecule, the slow nuclear motion and the fast electronic motion, are simultaneously measured in a photo-electron photo-ion coincidence…

We theoretically study time-resolved photoemission in atoms as probed by attosecond streaking. We review recent advances in the study of the photoelectric effect in the time domain and show that the experimentally accessible time shifts can…

Atomic Physics · Physics 2015-03-06 Stefan Nagele , Renate Pazourek , Michael Wais , Georg Wachter , Joachim Burgdörfer

We use three dimensional time-dependent Schr\"odinger equation (3D--TDSE) to calculate angular electron momentum distributions and photoelectron spectra of atoms driven by spatially inhomogeneous fields. An example for such inhomogeneous…

Atomic Physics · Physics 2013-06-26 M. F. Ciappina , J. A. Pérez-Hernández , T. Shaaran , L. Roso , M. Lewenstein

Velocity map imaging inside an electrostatic quadrupole guide is demonstrated. By switching the voltages that are applied to the rods, the quadrupole can be used for guiding Stark decelerated molecules and for extracting the ions. The…

Chemical Physics · Physics 2017-08-23 Marina Quintero Pérez , Paul Jansen , Hendrick L. Bethlem

Isochronous mass spectrometry (IMS) in storage rings is a powerful tool for mass measurements of exotic nuclei with very short half-lives down to several tens of microseconds, using a multicomponent secondary beam separated in-flight…

Intense 3-cycle pulses (10 fs) of 800 nm laser light are utilized to measure energy distributions of ions emitted following Coulomb explosion of Ar$_n$ clusters ($n$=400-900) upon their irradiation by peak intensitis of 5$\times$10$^{14}$ W…

Atomic and Molecular Clusters · Physics 2010-05-21 D. Mathur , F. A. Rajgara , A. R. Holkundkar , N. K. Gupta

This tutorial presents an introduction to the interaction of light and matter on the attosecond timescale. Our aim is to detail the theoretical description of ultra-short time-delays, and to relate these to the phase of extreme ultraviolet…

Atomic Physics · Physics 2012-07-20 J. M. Dahlström , A. L'Huillier , A. Maquet

We propose the scheme of temporal double-slit interferometer to precisely measure the electric field of shaped intense femtosecond laser pulse directly, and apply it to control the electron tunneling wave packets in attosecond precision. By…

Atomic Physics · Physics 2023-11-13 Xiaoyun Zhao , Mingqing Liu , Yizhang Yang , Zhou Chen , Xiaolei Hao , Chuncheng Wang , Weidong Li , Jing Chen

The attosecond streaking technique is normally utilized to characterize the attosecond pulses in extreme ultraviolet spectrum, while the pulse simulation and reconstruction schemes turn out to be unreliable for extremely short sub-100as…

Optics · Physics 2018-09-05 Renzhi Shao , Bin Li

Attosecond pulses, produced through high-order harmonic generation in gases, have been successfully used for observing ultrafast, sub-femtosecond electron dynamics in atoms, molecules and solid state systems. Today's typical attosecond…

Photoionization of matter is one of the fastest electronic processes in nature. Experimental measurements of photoionization dynamics have become possible through attosecond metrology. However, all experiments reported to date contain a…

Quantum Physics · Physics 2025-02-11 Meng Han , Jia-Bao Ji , Leung Chung Sum , Kiyoshi Ueda , Hans Jakob Wörner

Strong field ionization by circularly polarized laser fields from initial states with internal orbital momentum has interesting propensity rule: electrons counter-rotating with respect to the laser field can be liberated more easily than…

Atomic Physics · Physics 2015-12-16 Jivesh Kaushal , Felipe Morales , Olga Smirnova

To measure and control the electron motion in atoms and molecules by the strong laser field on the attosecond time scale is one of the research frontiers of atomic and molecular photophysics. It involves many new phenomena and processes and…

Atomic Physics · Physics 2022-03-30 Chao Chen , Jiayin Che , Shang Wang , Guoguo Xin , Yanjun Chen

We propose an attosecond XUV-pump IR-probe photoionization protocol that employs pairs of counter-rotating consecutive harmonics and angularly resolved photoelectron detection, thereby providing direct measurement of ionization phases. The…

Atomic Physics · Physics 2019-10-02 Stefan Donsa , Nicolas Douguet , Joachim Burgdörfer , Iva Březinová , Luca Argenti