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The existence of heterogeneity in the dynamics of supercooled liquids is believed to be one of the hallmarks of the glass transition. Intense research has been carried out in the past to understand the origin of this heterogeneity in…

Soft Condensed Matter · Physics 2020-07-01 Indrajit Tah , Smarajit Karmakar

The dynamical glass transition is typically taken to be the temperature at which a glassy liquid is no longer able to equilibrate on experimental timescales. Consequently, the physical properties of these systems just above or below the…

Soft Condensed Matter · Physics 2017-03-08 Samuel S. Schoenholz , Ekin D. Cubuk , Efthimios Kaxiras , Andrea J. Liu

We study multicomponent liquids by increasing the mass of $15\%$ of the particles in a binary Kob-Andersen model. We find that the heavy particles have dual effects on the lighter particles. At higher temperatures, there is a significant…

Soft Condensed Matter · Physics 2024-07-30 Ehtesham Anwar , Palak Patel , Mohit Sharma , Sarika Maitra Bhattacharyya

We discuss the relaxation dynamics of a simple lattice gas model for glass-forming systems and show that with increasing density of particles this dynamics slows down very quickly. By monitoring the trajectory of tagged particles we find…

Soft Condensed Matter · Physics 2010-05-07 Pinaki Chaudhuri , Ludovic Berthier , Srikanth Sastry , Walter Kob

We study the role of elasticity-induced facilitation on the dynamics of glass-forming liquids by a coarse-grained two-dimensional model in which local relaxation events, taking place by thermal activation, can trigger new relaxations by…

Disordered Systems and Neural Networks · Physics 2023-04-05 Misaki Ozawa , Giulio Biroli

We analyse, using Inhomogenous Mode-Coupling Theory, the critical scaling behaviour of the dynamical susceptibility at a distance epsilon from continuous second-order glass transitions. We find that the dynamical correlation length xi…

Disordered Systems and Neural Networks · Physics 2014-12-17 Saroj Kumar Nandi , Giulio Biroli , Jean-Philippe Bouchaud , Kunimasa Miyazaki , David R. Reichman

The origin of the dramatic changes in the behavior of liquids as they approach their vitreous state - increases of many orders of magnitude in transport properties and dynamic time scales - is a major unsolved problem in condensed matter.…

Soft Condensed Matter · Physics 2015-06-23 R. Casalini , D. Fragiadakis , C. M. Roland

We use a simple mode-coupling approach to investigate glassy dynamics of partially pinned fluid systems. Our approach is different from the mode-coupling theory developed by Krakoviack [Phys. Rev. Lett. 94, 065703 (2005), Phys. Rev. E 84,…

Disordered Systems and Neural Networks · Physics 2015-06-04 Grzegorz Szamel , Elijah Flenner

We report on zero field cooled magnetization relaxation experiments on a concen- trated frozen ferrofluid exhibiting a low temperature superspin glass transition. With a method initially developed for spin glasses, we investigate the field…

Disordered Systems and Neural Networks · Physics 2009-02-09 Elie Wandersman , V. Dupuis , Emmanuelle Dubois , Régine Perzynski , S. Nakamae , Eric Vincent

We present experimental confirmation of dynamic facilitation in monodisperse and bidisperse colloidal suspensions near the glass transition volume fraction. Correlations in particle dynamics are seen to exist not only in space (clusters and…

Soft Condensed Matter · Physics 2014-06-24 Scott V. Franklin , Eric R. Weeks

In this work we numerically investigate a new method for the characterization of growing length scales associated with spatially heterogeneous dynamics of glass-forming liquids. This approach, motivated by the formulation of the…

Disordered Systems and Neural Networks · Physics 2013-10-28 Kang Kim , Shinji Saito , Kunimasa Miyazaki , Giulio Biroli , David R. Reichman

By using fluid-kinetic simulations of confined and concentrated emulsion droplets, we investigate the nature of space non-homogeneity in soft-glassy dynamics and provide quantitative measurements of the statistical features of plastic…

Soft Condensed Matter · Physics 2014-02-19 R. Benzi , M. Sbragaglia , P. Perlekar , M. Bernaschi , S. Succi , F. Toschi

We use computer simulations to investigate the static properties of a simple glass-forming fluid in which the positions of a finite fraction of the particles has been frozen in. By probing the equilibrium distribution of the overlap between…

Disordered Systems and Neural Networks · Physics 2015-06-12 Walter Kob , Ludovic Berthier

Dynamic heterogeneity in glass-formers has been related to their static structure using the concept of dynamic propensity. We re-examine this relationship by analyzing dynamical fluctuations in two atomistic glass-formers and two…

Statistical Mechanics · Physics 2009-08-25 Ludovic Berthier , Robert L. Jack

We examine the phenomenon of dynamical heterogeneity in computer simulations of an equilibrium, glass-forming liquid. We describe several approaches to quantify the spatial correlation of single-particle motion, and show that spatial…

Soft Condensed Matter · Physics 2009-09-25 Sharon C. Glotzer , Claudio Donati

We use computer simulations to study the relaxation dynamics of a model for oil-in-water microemulsion droplets linked with telechelic polymers. This system exhibits both gel and glass phases and we show that the competition between these…

Soft Condensed Matter · Physics 2015-05-29 Pinaki Chaudhuri , Pablo I. Hurtado , Ludovic Berthier , Walter Kob

The dynamics of dense particle packings near the jamming transition is characterized by correlated particle motion. The growth of dynamical heterogeneities, or strong spatial variations in the motion of the particles constituting the…

Soft Condensed Matter · Physics 2024-09-12 Rajkumar Biswas , Anoop Mutneja , Smarajit Karmakar , Ranjini Bandyopadhyay

We investigate the spatio-temporal distribution of microscopic relaxation events, defined through particle hops, in a model polymer glass using molecular dynamics simulations. We introduce an efficient algorithm to directly identify hops…

Soft Condensed Matter · Physics 2013-08-30 Anton Smessaert , Jörg Rottler

The dynamical facilitation scenario, by which localized relaxation events promote nearby relaxation events in an avalanching process, has been suggested as the key mechanism connecting the microscopic and the macroscopic dynamics of…

Soft Condensed Matter · Physics 2015-11-03 Raffaele Pastore , Antonio Coniglio , Massimo Pica Ciamarra

We investigate the characteristic length scales associated with the glass transition phenomenon. By studying an atomic glass-forming liquid in negatively curved space, for which the local order is well identified and the amount of…

Statistical Mechanics · Physics 2010-02-10 François Sausset , Gilles Tarjus