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We study coherent energy transfer of a single excitation and quantum entanglement in a dimer, which consists of a donor and an acceptor modeled by two two-level systems. Between the donor and the acceptor, there exists a dipole-dipole…

Quantum Physics · Physics 2015-03-17 Jie-Qiao Liao , Jin-Feng Huang , Le-Man Kuang , C. P. Sun

Interplay of simultaneous creation, annihilation, propagation, and relaxation of an excitation in molecular condensates interacting with an ultrashort quantum optical pulse is studied in general and specialized to a dimer. A microscopic…

Quantum Physics · Physics 2012-08-27 J. Perina,

We study the direct incoherent energy transfer from an immobile excited donor molecule to acceptor molecules, which are all attached to polymer chains, randomly arranged in a viscous solvent. The decay forms are found explicitly, in terms…

Condensed Matter · Physics 2008-02-03 G. Oshanin , J. De Coninck , A. Blumen , S. F. Burlatsky , M. Moreau

We develop a mathematically rigorous theory for the quantum transfer processes in degenerate donor-acceptor dimers in contact with a thermal environment. We calculate explicitly the transfer rates and the acceptor population efficiency. The…

Quantum Physics · Physics 2020-07-15 Marco Merkli , Gennady P. Berman , Avadh Saxena

The roles of the vibration motions played in the excitation energy transfer process are studied. It is found that a strong coherent transfer in the hybrid system emerges when the detuning between the donor and the acceptor equals the…

Biological Physics · Physics 2014-12-18 Xin Wang , Hao Chen , Hong-rong Li

Absorption of electromagnetic energy by a material is a phenomenon that underlies many applied problems, including molecular sensing, photocurrent generation and photodetection. Commonly, the incident energy is delivered to the system…

Optics · Physics 2018-06-11 Denis G. Baranov , Alex Krasnok , Timur Shegai , Andrea Alù , Y. D. Chong

We study transfer of coherent nuclear oscillations between an excitation energy donor and an acceptor in a simple dimeric electronic system coupled to an unstructured thermodynamic bath and some pronounced vibrational intramolecular mode.…

Chemical Physics · Physics 2015-01-08 Tomáš Mančal , Jakub Dostál , Jakub Pšenčík , Donatas Zigmantas

The dynamics of a dimer coupled to two different environments each in a spin star configuration under the influence of decoherence is studied. The exact analytical expression for the transition probability in the dimer system is obtained…

Quantum Physics · Physics 2014-01-15 I. Sinayskiy , A. Marais , F. Petruccione , A. Ekert

We study the nature of the energy transfer process within a pair of coupled two-level systems (donor and acceptor) subject to interactions with the surrounding environment. Going beyond a standard weak-coupling approach, we derive a master…

Quantum Physics · Physics 2011-04-05 Dara P. S. McCutcheon , Ahsan Nazir

We characterize the coherent dynamics of a two-level quantum emitter driven by a pair of symmetrically-detuned phase-locked pulses. The promise of dichromatic excitation is to spectrally isolate the excitation laser from the quantum…

The non-equilibrium stationary coherences that form in donor-acceptor systems are investigated to determine their relationship to the efficiency of energy transfer to a neighboring reaction center. It is found that the effects of asymmetry…

Chemical Physics · Physics 2020-07-03 Kenneth A. Jung , Paul Brumer

The time-development of photoexcitations in molecular aggregates exhibits specific dynamics of electronic states and vibrational wavefunction. We discuss the dynamical formation of entanglement between electronic and vibrational degrees of…

Quantum Physics · Physics 2007-05-23 Dmitri S. Kilin , Jeffrey A. Cina , Oleg V. Prezhdo

Photochromic molecular structures constitute a unique platform for constructing molecular switches, sensors and memory devices. One of their most promising applications is as light-switchable electron acceptor or donor units. Here, we…

Chemical Physics · Physics 2020-07-21 Jakub K. Sowa , Emily A. Weiss , Tamar Seideman

We experimentally demonstrate the coherent control, i.e., phase-dependent enhancement and suppression, of the optical absorption in an array of metallic nanoantennas covered by a thin lu- minescent layer. The coherent control is achieved by…

Coherent control of femtosecond two-photon absorption in the intermediate-field regime is analyzed in detail in the powerful frequency domain using an extended 4th-order perturbative description. The corresponding absorption is coherently…

Atomic Physics · Physics 2008-01-24 Lev Chuntonov , Leonid Rybak , Andrey Gandman , Zohar Amitay

We theoretically show that energy absorption in crystalline silicon can be controlled by two-color femtosecond double-pulse irradiation, in which two temporally separated pulses with different wavelengths interact sequentially with the…

Materials Science · Physics 2026-04-29 Eiyu S. Gushiken , Mizuki Tani , Hiroki Katow , Kenichi L. Ishikawa

Dynamics of resonant energy transfer of a single excitation in a molecular dimer system is studied in the simultaneous presence of diagonal and off-diagonal exciton-phonon coupling. It is found that the off-diagonal coupling plays an…

Quantum Physics · Physics 2015-05-27 Ning Wu , Zhe Chang , Yang Zhao

Resonant transfer of energy between excited states in a system of two semiconductor quantum dots is studied theoretically. The model Hamiltonian has been formulated, which allowed describe the impact on the dynamics of the resonant laser…

Mesoscale and Nanoscale Physics · Physics 2013-06-03 P. A. Golovinski

Adsorption of dimers is modelled using random sequential adsorption algorithm. The interaction between molecules is given by screened electrostatic potential. The paper focuses on the properties of adsorbed monolayers as well as the…

Materials Science · Physics 2013-05-14 Michal Ciesla , Jakub Barbasz

We study inelastic collisions of counter-propagating self-induced transparency solitons in a homogeneously broadened two-level medium. The energy of the pulse can be almost totally absorbed in the medium due to asymmetric collision with a…

Optics · Physics 2012-04-11 Denis Novitsky
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