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The thermodynamic behavior of collapse transition in a fully flexible coarse-grained model of energy polydisperse polymer (EPP), a statistical model of random heteropolymer, is investigated in an implicit solvent by means of molecular…

Soft Condensed Matter · Physics 2025-03-04 Thoudam Vilip Singh , Lenin S. Shagolsem

A non-isothermal phase field model that captures both displacive and diffusive phase transformations in a unified framework is presented. The model is developed in a formal thermodynamic setting, which provides guidance on admissible…

Materials Science · Physics 2011-12-02 Mirko Maraldi , Garth N. Wells , Luisa Molari

The lattice cluster theory (LCT) for semiflexible linear telechelic melts, developed in paper I, is applied to examine the influence of chain stiffness on the average degree of self-assembly and the basic thermodynamic properties of linear…

Soft Condensed Matter · Physics 2015-06-29 Wen-Sheng Xu , Karl F. Freed

Alpha S8 is the most stable crystalline form, at ambient pressure and temperature (STP), of elemental sulfur. In this paper we analyze the zero pressure low temperature part of the phase diagram of this crystal, in order to test a simple…

Soft Condensed Matter · Physics 2009-10-31 C. Pastorino , Z. Gamba

Using non-equilibrium molecular dynamics simulations we study the yielding behaviour of a model cluster crystal formed by ultrasoft particles under shear. We investigate the evolution of stress as a function of strain for different shear…

Soft Condensed Matter · Physics 2020-05-26 G. P. Shrivastav , G. Kahl

Semicrystalline polymers (SCP) represent important class of materials used in many applications from packaging to transportation to electronics to pharmaceuticals. Understanding the structure and dynamics of the crystalline and amorphous…

Soft Condensed Matter · Physics 2025-04-28 Valeriy V. Ginzburg

We present a Bethe approximation to study lattice models of linear polymers. The approach is variational in nature and based on the cluster variation method (CVM). We focus on a model with $(i)$ a nearest neighbor attractive energy…

Statistical Mechanics · Physics 2009-10-31 Stefano Lise , Amos Maritan , Alessandro Pelizzola

The effect of finite temperature $T$ and finite strain rate $\dot\gamma$ on the statistical physics of plastic deformations in amorphous solids made of $N$ particles is investigated. We recognize three regimes of temperature where the…

Statistical Mechanics · Physics 2015-05-19 Smarajit Karmakar , Edan Lerner , Itamar Procaccia , Jacques Zylberg

We theoretically investigate the kinetics of the folding transition of a single semiflexible polymer. In the folding transition, the growth rate decrease with an increase in the number of monomers in a collapsed domain, suggesting that the…

Soft Condensed Matter · Physics 2009-11-13 Natsuhiko Yoshinaga

We present an extremely simplified model of multiple-domains polymer stretching in an atomic force microscopy experiment. We portray each module as a binary set of contacts and decompose the system energy into a harmonic term (the…

Biomolecules · Quantitative Biology 2008-01-20 Carlo Guardiani , Franco Bagnoli

We define a lattice model for the interaction of a polymer with water. We solve the model in a suitable approximation. In the case of a non-polar homopolymer, for reasonable values of the parameters, the polymer is found in a non-compact…

Statistical Mechanics · Physics 2009-10-31 Pierpaolo Bruscolini , Lapo Casetti

We describe some recent results concerning the statistical properties of a self-interacting polymer stretched by an external force. We concentrate mainly on the cases of purely attractive or purely repulsive self-interactions, but our…

Probability · Mathematics 2011-08-25 Dmitry Ioffe , Yvan Velenik

We model the flow behaviour of dense melts of flexible and semiflexible ring polymers in the presence of walls using a hybrid multiscale approach. Specifically, we perform molecular dynamics simulations and apply the Irving-Kirkwood formula…

Numerical Analysis · Mathematics 2026-05-25 Ranajay Datta , Mária Lukáčová-Medviďová , Andreas Schömer , Peter Virnau

We study the steady state resulting from instabilities in crystals driven through a dissipative medium, for instance, a colloidal crystal which is steadily sedimenting through a viscous fluid. The problem involves two coupled fields, the…

Statistical Mechanics · Physics 2009-10-31 Rangan Lahiri , Mustansir Barma , Sriram Ramaswamy

Relaxor ferroelectrics are difficult to study and understand. The experiment shows that at low energy scattering there is an acoustic mode, an optic mode, dynamic quasi-elastic scattering and strictly elastic scattering as well as Bragg…

Materials Science · Physics 2008-08-29 R. A. Cowley , S. N. Gvasaliya , B. Roessli

This report deals with phase transition in Bond Fluctuation Model (BFM) of a linear homo polymer on a two dimensional square lattice. Each monomer occupies a unit cell of four lattice sites. The condition that a lattice site can at best be…

Soft Condensed Matter · Physics 2012-04-16 Hima Bindu Kolli , K. P. N. Murthy

The time-dependent response of polystyrene and poly(methyl methacrylate) is studied in isothermal long-term shear creep tests at small strains and various temperatures in the vicinity of the glass transition point. A micromechanical model…

Soft Condensed Matter · Physics 2007-05-23 Aleksey D. Drozdov , Joachim Kaschta

The properties of a semiflexible polymer with fixed ends exposed to oscillatory shear flow are investigated by simulations. The two-dimensionally confined polymer is modeled as a linear bead-spring chain, and the interaction with the fluid…

Soft Condensed Matter · Physics 2021-12-14 Antonio Lamura , Roland G. Winkler

We model polydomain liquid-crystal elastomers by extending the neo-classical soft and semi-soft free energies used successfully to describe monodomain samples. We show that there is a significant difference between polydomains cross-linked…

Soft Condensed Matter · Physics 2014-07-09 J. S. Biggins , M. Warner , K. Bhattacharya

The recently developed Perturbed-Chain Statistical Associating Fluid Theory (PC-SAFT) is investigated for a wide range of model parameters including the parameter m representing the chain length and the thermodynamic temperature T and…

Soft Condensed Matter · Physics 2009-11-11 L. Yelash , M. Mueller , W. Paul , K. Binder
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