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The thermodynamic stability of the hard-sphere gas has been examined, using the formalism of scaled particle theory [SPT], and by applying explicitly the conditions of stability required by both the second and third laws of thermodynamics.…

Statistical Mechanics · Physics 2007-05-23 J. F. Kenney

We successfully extend a multiscale simulation (MSS) method to nonisothermal well-entangled polymer melt flows between two coaxial cylinders. In the multiscale simulation, the macroscopic flow system is connected to a number of microscopic…

Soft Condensed Matter · Physics 2020-07-30 Yuji Hamada , Takeshi Sato , Takashi Taniguchi

We study the finite-temperature dynamics of thin elastic sheets in a single-clamped cantilever configuration. This system is known to exhibit a tilt transition at which the preferred mean plane of the sheet shifts from horizontal to a plane…

Soft Condensed Matter · Physics 2023-12-27 Roberto Abril Valenzuela , Paul Z. Hanakata , Mark J. Bowick

We examine the phase transition of polymer adsorption as well as the underlying kinetics of polymer binding from dilute solutions on a structureless solid surface. The emphasis is put on the properties of regular multiblock copolymers,…

Soft Condensed Matter · Physics 2009-09-03 A. Milchev , V. Rostiashvili , S. Bhattacharya , T. Vilgis

Protein folding is analyzed using a replica variational formalism to investigate some free energy landscape characteristics relevant for dynamics. A random contact interaction model that satisfies the minimum frustration principle is used…

Disordered Systems and Neural Networks · Physics 2009-10-30 Shoji Takada , Peter G. Wolynes

We introduce a simple geometric model for a double-stranded and double-helical polymer. We study the statistical mechanics of such polymers using both analytical techniques and simulation. Our model has a single energy-scale which…

Soft Condensed Matter · Physics 2007-05-23 Alvise De Col , Tanniemola B. Liverpool

Kinetics of conformational change of a semiflexible polymer under mechanical external field were investigated with Langevin dynamics simulations. It is found that a semiflexible polymer exhibits large hysteresis in mechanical…

Soft Condensed Matter · Physics 2009-11-10 Natsuhiko Yoshinaga , Kenichi Yoshikawa , Takao Ohta

Through a combination of rheological characterization and temperature-variable imaging methods, a novel gelation pathway in dilute solutions of a semiconducting polymer to achieve interconnected, crystalline networks with hierarchical…

Applied Physics · Physics 2018-11-26 Jing He , Xiaoqing Kong , Yuhao Wang , Michael Delaney , Dilhan M. Kalyon , Stephanie S. Lee

We consider the Peierls model for closed polyactetylene chains with an even number of carbon atoms as well as infinite chains, in the presence of temperature. We prove the existence of a critical temperature below which the chain is…

Mathematical Physics · Physics 2023-10-13 David Gontier , Adéchola Kouande , Eric Séré

Modelling elastocaloric effect (eCE) is crucial for the design of environmentally friendly and energy-efficient eCE based solid-state cooling devices. Here, a thermodynamically consistent non-isothermal phase-field model (PFM) coupling…

Materials Science · Physics 2023-03-10 Wei Tang , Qihua Gong , Min Yi , Bai-Xiang Xu , Long-Qing Chen

Within the framework of Lorentz model for description of viscoelastic medium the influence of deformational defect of the shear modulus is studied on melting of ultrathin lubricant film confined between the atomically flat solid surfaces.…

Statistical Mechanics · Physics 2009-11-11 A. V. Khomenko , I. A. Lyashenko

Two series of uniaxial tensile tests are performed on isotactic polypropylene with the strain rates ranging from 5 to 200 mm/min. In the first series, injection-molded specimens are used without thermal pre-treatment, whereas in the other…

Materials Science · Physics 2007-05-23 A. D. Drozdov , J. deC. Christiansen

The present contribution deals with the thermomechanical modeling of the strain-induced crystallization in unfilled polymers. This phenomenon significantly influences mechanical and thermal properties of polymers and has to be taken into…

Soft Condensed Matter · Physics 2020-11-11 Serhat Aygün , Sandra Klinge

Syndiotactic polystyrene (sPS) exhibits complex polymorphic behavior upon crystallization. Computational modeling of polymer crystallization has remained a challenging task because the relevant processes are slow on the molecular time…

Soft Condensed Matter · Physics 2018-05-28 Chan Liu , Kurt Kremer , Tristan Bereau

We investigate the dynamics and the pathways of the collapse of a single, semiflexible polymer in a poor solvent via 3-D Brownian Dynamics simulations. Earlier work indicates that the condensation of semiflexible polymers generically…

Soft Condensed Matter · Physics 2009-11-10 Alberto Montesi , Matteo Pasquali , F. C. MacKintosh

We investigate a reversible polymerization process in which individual polymers aggregate and fragment at a rate proportional to their molecular weight. We find a nonequilibrium phase transition despite the fact that the dynamics are…

Statistical Mechanics · Physics 2008-06-24 E. Ben-Naim , P. L. Krapivsky

We present using simple scaling arguments and one step replica symmetry breaking a theory for the localization of semiflexible polymers in a quenched random environment. In contrast to completely flexible polymers, localization of…

Soft Condensed Matter · Physics 2009-11-10 Arti Dua , Thomas A. Vilgis

Polymer blends consisting of two or more polymers are important for a wide variety of industries and processes, but, the precise mechanism of their thermomechanical behaviour is incompletely understood. In order to understand clearly, it is…

Soft Condensed Matter · Physics 2021-01-12 Pashupati Pokharel , Feng Wei , Jianyi Shi , Yingmin Wang , Dequan Xiao

The non-equilibrium structural and dynamical properties of semiflexible polymers confined to two dimensions are investigated by molecular dynamics simulations. Three different scenarios are considered: The force-extension relation of…

Soft Condensed Matter · Physics 2013-01-08 A. Lamura , R. G. Winkler

We derive a continuum-level plasticity model for polycrystalline materials in the high energy density regime, based on a single dislocation density and single mobility mechanism, with an evolution model for the dislocation density. The…

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