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The phase separation of a simple binary mixture of incompatible linear polymers in solution is investigated using an extension of the sedimentation equilibrium method, whereby the osmotic pressure of the mixture is extracted from the…

Soft Condensed Matter · Physics 2009-09-29 Chris I. Addison , Pierre-Arnaud Artola , Jean-Pierre Hansen , Ard A. Louis

Bilayer graphene has been a subject of intense study in recent years. We extend a structural phase field crystal method to include an external potential from adjacent layer(s), which is generated by the corresponding phase field and changes…

Materials Science · Physics 2020-12-24 Kai Liu

The phase diagram of a system of monodispersed hard rectangles of size $m\times m k$ on a square lattice is numerically determined for $m=2,3$ and aspect ratio $k= 1,2,\ldots, 7$. We show the existence of a disordered phase, a nematic phase…

Statistical Mechanics · Physics 2014-05-19 Joyjit Kundu , R. Rajesh

We study theoretically the effect of a gravitational field on the equilibrium behaviour of a colloidal suspension of rods with different length-to-width aspect ratios. The bulk phases of the system are described with analytical equations of…

Soft Condensed Matter · Physics 2023-03-10 Tobias Eckert , Matthias Schmidt , Daniel de las Heras

During the intercalation of lithium in layered host materials such as graphite, lithium atoms can move within the plane between two neighboring graphene sheets, but cannot cross the sheets. Repulsive interactions between atoms in different…

Materials Science · Physics 2024-09-06 Antoine Cordoba , Marion Chandesris , Mathis Plapp

Using a geometry-based fundamental measure density functional theory, we calculate bulk fluid phase diagrams of colloidal mixtures of vanishingly thin hard circular platelets and hard spheres. We find isotropic-nematic phase separation with…

Soft Condensed Matter · Physics 2015-06-11 Daniel de las Heras , Matthias Schmidt

A mesoscopic continuum model is employed to analyse the transport mechanisms and structure formation during the redistribution stage of deposition experiments where organic molecules are deposited on a solid substrate with periodic…

Mesoscale and Nanoscale Physics · Physics 2018-07-24 Christoph Honisch , Te-Sheng Lin , Andreas Heuer , Uwe Thiele , Svetlana Gurevich

We discuss mixing/segregation phenomena in a schematic hard spheres lattice model for binary mixtures of granular media, by analytical evaluation, within Bethe-Peierls approximation, of Edwards' partition function. The presence of…

Statistical Mechanics · Physics 2007-05-23 M. Tarzia , A. Fierro , M. Nicodemi , M. Pica Ciamarra , A. Coniglio

We show that one can employ well-established numerical continuation methods to efficiently calculate the phase diagram for thermodynamic systems. In particular, this involves the determination of lines of phase coexistence related to first…

Soft Condensed Matter · Physics 2021-01-22 Max Philipp Holl , Andrew J. Archer , Uwe Thiele

We study the phase behavior of mixtures of monodisperse colloidal spheres with a depletion agent which can have arbitrary shape and can possess a polydisperse size or shape distribution. In the low concentration limit, considered here, we…

Soft Condensed Matter · Physics 2009-11-11 C. Grodon , R. Roth

We theoretically study sedimentation-diffusion equilibrium of dilute binary, ternary, and polydisperse mixtures of colloidal particles with different buoyant masses and/or charges. We focus on the low-salt regime, where the entropy of the…

Soft Condensed Matter · Physics 2009-11-11 Jos Zwanikken , rene van Roij

Phase diagrams are essential tools of the materials scientist, showing which phases are at equilibrium under a set of applied thermodynamic conditions. Essentially all phase diagrams today are two dimensional, typically constructed with…

Mathematical Physics · Physics 2024-04-10 Wenhao Sun , Matthew J. Powell-Palm , Jiadong Chen

A model predicting the structure of repulsive, spherically symmetric, monodisperse particles confined between two walls is presented. We study the buckling transition of a single flat layer as the double layer state develops. Experimental…

Condensed Matter · Physics 2009-10-22 T Chou , David R. Nelson

The equilibrium phase behaviour of hard spheres with size polydispersity is studied theoretically. We solve numerically the exact phase equilibrium equations that result from accurate free energy expressions for the fluid and solid phases,…

Soft Condensed Matter · Physics 2007-05-23 M. Fasolo , P. Sollich

Phase separation of multicomponent liquid mixtures plays an integral part in many processes ranging from industry to cellular biology. In many cases the morphology of coexisting phases is crucially linked to the function of the separated…

Soft Condensed Matter · Physics 2020-11-25 Sheng Mao , Milena S. Chakraverti-Wuerthwein , Hunter Gaudio , Andrej Kosmrlj

We compute phase diagrams for $A_nB_m$ starblock copolymers in the strong-segregation regime as a function of volume fraction $\phi$, including bicontinuous phases related to minimal surfaces (G, D, and P surfaces) as candidate structures.…

Soft Condensed Matter · Physics 2009-10-31 Peter D. Olmsted , Scott T. Milner

Colloidal particles that are confined to an interface such as the air-water interface are an example of a two-dimensional fluid. Such dispersions have been observed to spontaneously form cluster and stripe morphologies in certain systems…

Soft Condensed Matter · Physics 2008-09-17 A. J. Archer

The binodals and the non-ergodicity lines of a binary mixture of hard sphere-like particles with large size ratio are computed for studying the interplay between dynamic arrest and phase separation in depletion-driven colloidal mixtures.…

Soft Condensed Matter · Physics 2009-11-13 Ph. Germain , S. Amokrane

A first principle prediction of the binary nanoparticle phase diagram assembled by solvent evaporation has eluded theoretical approaches. In this paper, we show that a binary system interacting through Lennard-Jones (LJ) potential contains…

Soft Condensed Matter · Physics 2020-11-06 Shang Ren , Yang Sun , Feng Zhang , Alex Travesset , Cai-Zhuang Wang , Kai-Ming Ho

Phase transformations can be difficult to characterize at the microscopic level due to the inability to directly observe individual atomic motions. Model colloidal systems, by contrast, permit the direct observation of individual particle…

Soft Condensed Matter · Physics 2015-04-21 Ye Yang , Lin Fu , Catherine Marcoux , Joshua E. S. Socolar , Patrick Charbonneau , Benjamin B. Yellen