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Low temperature measurements of the ac magnetic susceptibility along the [110] direction of a single crystal of the dipolar spin ice material Ho2Ti2O7, in zero static field, are presented. While behavior that is qualitatively consistent…

Materials Science · Physics 2015-05-27 J. A. Quilliam , L. R. Yaraskavitch , H. A. Dabkowska , B. D. Gaulin , J. B. Kycia

We have studied the field-dependent ac magnetic susceptibility of single crystals of Dy2Ti2O7 spin ice along the [111] direction in the temperature range 1.8 K - 7 K. Our data reflect the onset of local spin ice order in the appearance of…

Strongly Correlated Electrons · Physics 2015-06-12 M. J. Matthews , C. Castelnovo , R. Moessner , S. A. Grigera , D. Prabhakaran , P. Schiffer

We report a study of the low temperature bulk magnetic properties of the spin ice compound Dy2Ti2O7 with particular attention to the (T < 4 K) spin freezing transition. While this transition is superficially similar to that in a spin glass,…

Materials Science · Physics 2007-05-23 J. Snyder , B. G. Ueland , J. S. Slusky , H. Karunadasa , R. J. Cava , P. Schiffer

The residual entropy of spin ice and other frustrated magnets is a property of considerable interest, yet the usual way of determining it, by integrating the heat capacity, is generally ambiguous. Here we note that a straightforward…

Strongly Correlated Electrons · Physics 2013-08-07 L. Bovo , S. T. Bramwell

We report vibrating coil magnetometry of the spin ice system Ho2Ti2O7 down to ~0.04 K for magnetic fields up to 5 T applied parallel to the [111] axis. History dependent behavior emerges below T*_0 ~ 0.6 K near zero magnetic field, in…

Strongly Correlated Electrons · Physics 2012-06-25 C. Krey , S. Legl , S. R. Dunsiger , M. Meven , J. S. Gardner , J. M. Roper , C. Pfleiderer

Elastic and inelastic neutron scattering studies have been carried out on the pyrochlore magnet Ho2Ti2O7. Measurements in zero applied magnetic field show that the disordered spin ice ground state of Ho2Ti2O7 is characterized by a pattern…

Strongly Correlated Electrons · Physics 2016-08-05 J. P. Clancy , J. P. C. Ruff , S. R. Dunsiger , Y. Zhao , H. A. Dabkowska , J. S. Gardner , Y. Qiu , J. R. D. Copley , T. Jenkins , B. D. Gaulin

We present a parametric study of the diffuse magnetic scattering at (1/2,1/2,1/2) positions in reciprocal space, ascribed to a frozen antiferromagnetic spin ice state in single crystalline Tb2Ti2O7. Our high-resolution neutron scattering…

Strongly Correlated Electrons · Physics 2015-06-18 K. Fritsch , E. Kermarrec , K. A. Ross , Y. Qiu , J. R. D. Copley , D. Pomaranski , J. B. Kycia , H. A. Dabkowska , B. D. Gaulin

We have studied the thermodynamics of the stuffed spin ice material, Dy2(DyxTi2-x)O7-x/2, in which additional Dy3+ replace Ti4+ in the pyrochlore Dy2Ti2O7. Heat capacity measurements indicate that these materials lose the spin ice zero…

Strongly Correlated Electrons · Physics 2008-04-26 B. G. Ueland , G. C. Lau , R. S. Freitas , J. Snyder , M. L. Dahlberg , B. D. Muegge , E. L. Duncan , R. J. Cava , P. Schiffer

The magnetocaloric effect of polycrystalline samples of pure and Y-doped dipolar spin ice Dy2Ti2O7 was investigated at temperatures from nominally 0.3 K to 6 K and in magnetic fields of up to 2 T. As well as being of intrinsic interest, it…

Soft Condensed Matter · Physics 2015-06-25 M. Orendac , J. Hanko , E. Cizmar , A. Orendacova , M. Shirai , S. T. Bramwell

At low temperatures, a spin ice enters a Coulomb phase - a state with algebraic correlations and topologically constrained spin configurations. In Ho2Ti2O7, we have observed experimentally that this process is accompanied by a non-standard…

The spin ice materials Ho2Ti2O7 and Dy2Ti2O7 are experimental and theoretical exemplars of highly frustrated magnetic materials. However, the effects of an applied uniaxial pressure are not well studied, and here we report magnetization…

Magnetization and susceptibility studies on single crystals of the pyrochlore Ho$_{2}$Ti$_{2}$O$_{7}$ are reported for the first time. Magnetization isotherms are shown to be qualitatively similar to that predicted by the nearest neighbor…

Disordered Systems and Neural Networks · Physics 2009-11-07 A. L. Cornelius , J. S. Gardner

We report magnetization and ac susceptibility of single crystals of the spin ice compound Dy2Ti2O7. Saturated moments at 1.8 K along the charasteristic axes [100] and [110] agree with the expected values for an effective ferromagnetic…

Strongly Correlated Electrons · Physics 2016-08-31 H. Fukazawa , R. G. Melko , R. Higashinaka , Y. Maeno , M. J. P. Gingras

Systematic measurements of the magnetic susceptibility were performed on single crystals of lightly doped La2-xSrxCuO4 (x=0.03, 0.04 and 0.05). For all samples the temperature dependence of the in-plane magnetic susceptibility shows typical…

Superconductivity · Physics 2009-10-31 S. Wakimoto , S. Ueki , Y. Endoh , K. Yamada

Dy2Ti2O7 has been advanced as an ideal spin ice. We present a neutron scattering investigation of a sample of 162Dy2Ti2O7. The scattering intensity has been mapped in zero applied field in the hhl and hk0 planes at temperatures between 0.05…

Disordered Systems and Neural Networks · Physics 2009-11-10 T. Fennell , O. A. Petrenko , B. Fak , S. T. Bramwell , M. Enjalran , T. Yavors'kii , M. J. P. Gingras , R. G. Melko , G. Balakrishnan

Experimental data of the frequency-dependent ac susceptibility for the dipolar spin ice Dy2Ti2O7 has been analyzed by Monte Carlo simulations on the basis of the single-spin-flip Metropolis algorithm. We have directly evaluated the ac…

Strongly Correlated Electrons · Physics 2013-10-15 Hiroshi Takatsu , Kazuki Goto , Hiromi Otsuka , Ryuji Higashinaka , Kazuyuki Matsubayashi , Yoshiya Uwatoko , Hiroaki Kadowaki

We have performed AC susceptibility and DC magnetic relaxation measurements on the spin ice system Dy$_2$Ti$_2$O$_7$ down to 0.08 K. The relaxation time of the magnetization has been estimated below 2 K down to 0.08 K. The spin dynamics of…

Strongly Correlated Electrons · Physics 2012-02-07 K. Matsuhira , C. Paulsen , E. Lhotel , C. Sekine , Z. Hiroi , S. Takagi

We study single crystals of Dy$_2$Ti$_2$O$_7$ and Ho$_2$Ti$_2$O$_7$ under magnetic field and stress applied along their [001] direction. We find that many of the features that the emergent gauge field of spin ice confers to the macroscopic…

Dy2Ti2O7 is a geometrically frustrated magnetic material with a strongly correlated spin ice regime that extends from 1 K down to as low as 60 mK. The diffuse elastic neutron scattering intensities in the spin ice regime can be remarkably…

Statistical Mechanics · Physics 2008-08-02 Taras Yavors'kii , Tom Fennell , Michel J. P. Gingras , Steven T. Bramwell

Intensity distribution of the neutron magnetic scattering has been taken in the reciprocal space of a single crystal of the "spin ice" system Ho2Ti2O7 at the elastic energy position in the temperature (T) region between 0.4 K and 50 K. The…

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