English

Dynamics and thermodynamics of a topological transition in spin ice materials under strain

Statistical Mechanics 2021-05-18 v1 Other Condensed Matter

Abstract

We study single crystals of Dy2_2Ti2_2O7_7 and Ho2_2Ti2_2O7_7 under magnetic field and stress applied along their [001] direction. We find that many of the features that the emergent gauge field of spin ice confers to the macroscopic magnetic properties are preserved in spite of the finite temperature. The magnetisation vs. field shows an upward convexity within a broad range of fields, while the static and dynamic susceptibilities present a peculiar peak. Following this feature for both compounds, we determine a single experimental transition curve: that for the Kasteleyn transition in three dimensions, proposed more than a decade ago. Additionally, we observe that compression up to 0.8%-0.8\% along [001] does not significantly change the thermodynamics. However, the dynamical response of Ho2_2Ti2_2O7_7 is quite sensitive to changes introduced in the Ho3+{\rm Ho}^{3+} environment. Uniaxial compression can thus open up experimental access to equilibrium properties of spin ice at low temperatures.

Keywords

Cite

@article{arxiv.2105.07977,
  title  = {Dynamics and thermodynamics of a topological transition in spin ice materials under strain},
  author = {L. Pili and A. Steppke and M. E. Barber and F. Jerzembeck and C. W. Hicks and P. C. Guruciaga and D. Prabhakaran and R. Moessner and A. P. Mackenzie and S. A. Grigera and R. A. Borzi},
  journal= {arXiv preprint arXiv:2105.07977},
  year   = {2021}
}